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In recent years, ultrafast pump-probe spectroscopy has provided insightful information about nonequilibrium dynamics of excitations in materials. In a typical experiment of time-resolved x-ray absorption spectroscopy, the systems are…

Strongly Correlated Electrons · Physics 2019-05-29 Chen-Yen Lai , Jian-Xin Zhu

The electronic and structural properties of a material are strongly determined by its symmetry. Changing the symmetry via a photoinduced phase transition offers new ways to manipulate material properties on ultrafast timescales. However, in…

Strongly Correlated Electrons · Physics 2015-09-25 Simon Wall , Daniel Wegkamp , Laura Foglia , Joyeeta Nag , Richard F. Haglund , Julia Staehler , Martin Wolf

Floquet engineering of electronic systems is a promising way of controlling quantum material properties on an ultrafast time scale. So far, the energy structure of Floquet states in solids has been observed through time and angle-resolved…

Other Condensed Matter · Physics 2023-05-02 Kento Uchida , Satoshi Kusaba , Kohei Nagai , Tatsuhiko N. Ikeda , Koichiro Tanaka

The femtosecond optical pump-probe technique was used to study dynamics of photoexcited electrons and coherent optical phonons in transition metals Zn and Cd as a function of temperature and excitation level. The optical response in time…

Strongly Correlated Electrons · Physics 2009-11-11 Muneaki Hase , Kunie Ishioka , Jure Demsar , Kiminori Ushida , Masahiro Kitajima

The heating of the electronic distribution of a copper photocathode due to an intense drive laser pulse is calculated under the two-temperature model using fluences and pulse lengths typical in RF photoinjector operation. Using the finite…

Accelerator Physics · Physics 2018-03-14 J. Maxson , P. Musumeci , L. Cultrera , S. Karkare , H. Padmore

Time-resolved pump-probe measurements were made at variable heat accumulation in Co/Pd superlattices. Heat accumulation increases the baseline temperature and decreases the equilibrium magnetization. Transient ultrafast demagnetization…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 F. Hoveyda , E. Hohenstein , R. Judge , S. Smadici

Ultrafast spectroscopies constitute a fundamental tool to investigate the dynamics of non-equilibrium many-body states in correlated materials. Two-pulses (pump-probe) experiments have shed new light on the interplay between high-energy…

Strongly Correlated Electrons · Physics 2016-09-01 Claudio Giannetti

Experiments on superconducting materials have unveiled unique emergent properties when they are driven far from equilibrium. However, a quantitative first-principles treatment that describes experimental observations is lacking. In this…

The study of photoexcited strongly correlated materials is attracting growing interest since their rich phase diagram often translates into an equally rich out-of-equilibrium behavior, including non-thermal phases and photoinduced phase…

Ultrafast electronic dynamics are typically studied using pulsed lasers. We demonstrate a complementary experimental approach: quantum simulation of ultrafast dynamics using trapped ultracold atoms. Counter-intuitively, this technique…

Ultrafast laser excitation of a metal causes correlated, highly nonequilibrium dynamics of electronic and ionic degrees of freedom, which are however only poorly captured by the widely-used two-temperature model. Here we develop an…

Materials Science · Physics 2017-12-06 Pablo Maldonado , Karel Carva , Martina Flammer , Peter M. Oppeneer

We study the generation of coherent phonons in a superconductor by ultrafast optical pump pulses. The nonequilibrium dynamics of the coupled Bogoliubov quasiparticle-phonon system after excitation with the pump pulse is analyzed by means of…

Superconductivity · Physics 2011-12-14 Andreas P. Schnyder , Dirk Manske , Adolfo Avella

Tilted lattice potentials with periodic driving play a crucial role in the study of artificial gauge fields and topological phases with ultracold quantum gases. However, driving-induced heating and the growth of phonon modes restrict their…

We investigate the low-temperature thermodynamics of the unitary Fermi gas by introducing a model based on the zero-temperature spectra of both bosonic collective modes and fermonic single-particle excitations. We calculate the Helmholtz…

Quantum Gases · Physics 2011-07-08 Luca Salasnich

A positive rate of entropy production at steady state is a distinctive feature of truly non-equilibrium processes. Exact results, while being often limited to simple models, offer a unique opportunity to explore the thermodynamic features…

Statistical Mechanics · Physics 2022-06-29 Henry Alston , Luca Cocconi , Thibault Bertrand

The rate of entropy production by a stochastic process quantifies how far it is from thermodynamic equilibrium. Equivalently, entropy production captures the degree to which detailed balance and time-reversal symmetry are broken. Despite…

Statistical Mechanics · Physics 2020-12-02 Luca Cocconi , Rosalba Garcia-Millan , Zigan Zhen , Bianca Buturca , Gunnar Pruessner

In the last two decades, non-equilibrium spectroscopies have evolved from avant-garde studies to crucial tools for expanding our understanding of the physics of strongly correlated materials. The possibility of obtaining simultaneously…

Pump-probe spectroscopy is central for exploring ultrafast dynamics of fundamental excitations, collective modes and energy transfer processes. Typically carried out using conventional diffraction-limited optics, pump-probe experiments…

High-harmonic generation in solids has emerged as a powerful probe of ultrafast electron dynamics and lattice motion, and recent theoretical work has suggested that thermally driven lattice fluctuations can act as an effective source of…

In past decades, ultrafast spin dynamics in magnetic systems have been associated with heat deposition from high energy laser pulses, limiting the selective access to spin order. Here we use a long wavelength terahertz pump optical probe…

Materials Science · Physics 2021-06-04 Hovan Lee , Cedric Weber , Manfred Fähnle , Mostafa Shalaby