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In this work, we demonstrate experimentally the efficient generation and tunability of energetic highly-elliptical high-harmonics in Ar gas, driven by intense two-color counter rotating laser electric fields. A bi-chromatic beam tailored by…

We report on a compact and spectrally intense extreme-ultraviolet (XUV) source, which is based on high-harmonic generation (HHG) driven by 395 nm pulses. In order to minimize the XUV virtual source size and to maximize the XUV flux, HHG is…

Optics · Physics 2021-07-01 M. Kretschmar , M. J. J. Vrakking , B. Schütte

Spectrally-tunable quantum-light sources are key elements for the realization of long-distance quantum communication. A deterministically fabricated single-photon source with a photon-extraction efficiency of {\eta}=(20 +- 2) % and a tuning…

Mesoscale and Nanoscale Physics · Physics 2018-05-29 S. Fischbach , M. v. Helversen , M. Schmidt , A. Kaganskiy , R. Schmidt , A. Schliwa , T. Heindel , S. Rodt , S. Reitzenstein

High harmonic generation (HHG) in solids has emerged as a powerful spectroscopic method for resolving ultrafast electron dynamics and band structure properties across a wide range of materials. However, quantitative HHG studies require…

Optics · Physics 2025-12-16 S. Mandal , P. Kumar , Z. Pi , H. Y. Kim , M. Zhan , E. Goulielmakis

Time- and angle-resolved photoemission spectroscopy (TrARPES) is a powerful technique for capturing the ultrafast dynamics of charge carriers and revealing photo-induced phase transitions in quantum materials. However, the lack of widely…

Mesoscale and Nanoscale Physics · Physics 2022-01-05 Changhua Bao , Haoyuan Zhong , Shaohua Zhou , Runfa Feng , Yuan Wang , Shuyun Zhou

We describe a setup to study ultrafast dynamics in gas-phase molecules using time-resolved photoelectron and photoion spectroscopy. The vacuum ultraviolet (VUV) probe pulses are generated via strong field high-order harmonic generation from…

Atomic and Molecular Clusters · Physics 2014-04-14 Markus Koch , Thomas J. A. Wolf , Jakob Grilj , Emily Sistrunk , Markus Gühr

High-harmonic generation (HHG) normally requires a careful adjustment of the driving laser intensity (typically $10^{14} - 10^{15}$ W/cm$^2$) and gas medium parameters to enable good phase matching conditions. In contrast with conventional…

Brilliant X-ray sources are of great interest for many research fields from biology via medicine to material research. The quest for a cost-effective, brilliant source with unprecedented temporal resolution has led to the recent realization…

Plasma Physics · Physics 2014-06-26 K. Khrennikov , J. Wenz , A. Buck , J. Xu , M. Heigoldt , L. Veisz , S. Karsch

We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…

We report generation of spectrally bright vacuum ultraviolet (VUV) and deep UV (DUV) coherent radiations driven by quantum coherence in tunnel-ionized carbon monoxide (CO) molecules. Our technique allows us to switch between multiple…

High harmonics generation (HHG) of coherent extreme ultraviolet (EUV) radiation enables ultrafast pump-probe spectroscopy with attosecond-scale timing resolutions. Yet beam control of generated EUV radiation remains a major challenge for…

We report on the realization of a solid-state-based vacuum ultraviolet frequency comb, using multi-harmonic generation in an external enhancement cavity. Optical conversions in such arrangements were so-far reported only using gaseous…

Optics · Physics 2019-03-27 J. Seres , E. Seres , C. Serrat , Erin C. Young , James S. Speck , T. Schumm

On-chip ultraviolet sources are of great interest for building compact and scalable atomic clocks, quantum computers, and spectrometers; however, few material platforms are suitable for integrated ultraviolet light generation. Of these…

A frequency-stabilized ultraviolet laser system, locked to the thallium resonant transition of 377.5 nm, was demonstrated using a novel bichromatic spectroscopy technique for tuning the zero-crossing laser-lock point. The atomic thallium…

Atomic Physics · Physics 2016-12-09 Tzu-Ling Chen , Chang-Yi Lin , Jow-Tsong Shy , Yi-Wei Liu

A continuous-wave laser source at 148.4 nm based on second-harmonic generation in randomly quasi-phase matched strontium tetraborate, SrB4O7, is demonstrated. It provides (1.3-0.6+0.7) nW of VUV power in a single pass for an incident UV…

Optical modulation of high-harmonics generation in solids enables the detection of material properties such as the band structure and promising new applications such as super-resolution imaging in semiconductors. Various recent studies have…

Sources of quantum light, in particular correlated photon pairs that are indistinguishable in all degrees of freedom, are the fundamental resource that enables continuous-variable quantum computation and paradigms such as Gaussian boson…

The ideal laser source for the emerging research field of nonlinear Terahertz (THz) spectroscopy should offer radiation with a large versatility and deliver both ultra-intense multi-octave spanning single-cycle pulses and user-selectable…

Attosecond photoelectron spectroscopy is often performed with interferometric experimental setups that require outstanding stability. We demonstrate and characterize in detail an actively stabilized, versatile, high spectral resolution…

We report on the generation of intense extreme ultraviolet (EUV) supercontinuum with photon energies spanning from 35 eV to 50 eV (i. e., supporting an isolated attosecond pulse with a duration of ~271 as) by loosely focusing 35 fs, 11 mJ…

Optics · Physics 2015-05-30 Bin Zeng , Wei Chu , Guihua Li , Jinping Yao , Jielei Ni , Haisu Zhang , Ya Cheng , Zhizhan Xu