Related papers: Interrogating Quantum Nonlocal Effects in Nanoplas…
We experimentally demonstrate that the interaction between plasma and nanometer-sized semiconductor quantum dots (QDs) is directly connected to a change in their photoluminescence (PL) spectrum. This is done by taking in-situ, high…
In the last decades, the blossoming of experimental breakthroughs in the domain of electron energy loss spectroscopy (EELS) has triggered a variety of theoretical developments. Those have to deal with completely different situations, from…
Electron energy loss spectroscopy (EELS) has emerged as a powerful tool for the investigation of plasmonic nanoparticles, but the interpretation of EELS results in in terms of optical quantities, such as the photonic local density of…
Analysis of Bell-EPR nonlocal correlations in microscopic measurement theory framework indicates that novel quantum nonlocality effects can exist. In particular, it can result in distant correlations between the systems of elementary…
Plasmon-exciton polaritons provide exciting possibilities to control light-matter interactions at the nanoscale by enabling closer investigation of quantum optical effects and facilitating novel technologies based, for instance, on…
We investigate the excitation of electrostatic wakefields in metallic nanostructures (nanowires) due to the propagation of a short electron pulse. For that purpose, a dispersive (nonlocal) dielectric response of the system is considered,…
We present a hydrodynamic model, grounded in Madelung's formalism, to describe collective electronic motion in anisotropic materials. This model incorporates nonlocal contributions from the Thomas-Fermi quantum pressure and quantum effects…
In the context of electromagnetism and nonlinear optical interactions damping is generally introduced as a phenomenological, viscous term that dissipates energy, proportional to the temporal derivative of the polarization. Here, we follow…
Surface effects on the electronic energy loss of charged particles entering a metal surface are investigated within linear-response theory, in the framework of time-dependent density functional theory. Interesting phenomena occur in the…
Symmetry breaking at surfaces and interfaces and the capability to support large strain gradients in nanoscale systems enable new forms of electromechanical coupling. Here we introduce the concept of quantum flexoelectricity, a phenomenon…
The dielectric properties of metallic nanoclusters in the presence of an applied electromagnetic field are investigated using non-local linear response theory. In the quantum limit we find a non-trivial dependence of the induced field and…
Strong-field photoemission from metal nanostructures enabled fundamental discoveries recently. Here, we deliver theoretical demonstration of the electric field control of electrons in the closest nanoscale vicinity of plasmonic…
We present a variant of the recently developed quantum corrected model (QCM) for plasmonic nanoparticles [Nature Commun. 3, 825 (2012)] using non-local boundary conditions. The QCM accounts for electron tunneling in narrow gap regions of…
Metamaterials are fascinating tools that can structure not only surface plasmons and electromagnetic waves but also electromagnetic vacuum fluctuations. The possibility of shaping the quantum vacuum is a powerful concept that ultimately…
The electronic environment causes decoherence and dissipation of the collective surface plasmon excitation in metallic nanoparticles. We show that the coupling to the electronic environment influences the width and the position of the…
Plasmon resonance, with strong coupling of light to electrons at a metal-dielectric interface, allows light confinement and control at subwavelength scale. It's fundamentally limited by the inherent mobility of the electrons, leading to the…
Cathodoluminescence (CL) enables optical-frequency analysis of samples with nanometer resolutions, originating from the interaction of a focused electron beam with radiative electronic states, or directly with the optical modes of the…
Cathodoluminescence spectroscopy has recently emerged as a novel platform for nanoscale control of nonclassical features of light. Here, we propose a theoretical model for cathodoluminescence from a multi-level quantum emitter. Employing a…
Nonlinear metasurfaces based on coupling a locally enhanced plasmonic response to intersubband transitions of n-doped multi-quantum-wells (MQWs) have recently provided second-order susceptibilities orders of magnitude larger than any other…
Quantum simulations of metal surfaces are critical for catalytic innovation. Yet existing methods face a cost-accuracy dilemma: density functional theory is efficient but system-dependent in accuracy, while wavefunction-based theories are…