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This review discusses how low-energy, valence excitations created by swift electrons can render information on the optical response of structured materials with unmatched spatial resolution. Electron microscopes are capable of focusing…

Materials Science · Physics 2012-11-13 F. J. Garcia de Abajo

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

We study the nonlocal response of a confined electron gas within the hydrodynamical Drude model. We address the question whether plasmonic nanostructures exhibit nonlocal resonances that have no counterpart in the local-response Drude…

Mesoscale and Nanoscale Physics · Physics 2011-09-30 Søren Raza , Giuseppe Toscano , Antti-Pekka Jauho , Martijn Wubs , N. Asger Mortensen

Recently synthesized 3D materials with Dirac spectrum exhibit peculiar electric transport qualitatively different from its 2D analogue, graphene. Neglecting impuritiy scattering, the real part of the conductivity is strongly frequency…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 B. Rosenstein , H. C. Kao , M. Lewkowicz

We develop a microscopic large-$N$ theory of electron-electron interaction corrections to multi-legged Feynman diagrams describing second- and third-order nonlinear response functions. Our theory, which reduces to the well-known random…

Materials Science · Physics 2017-01-25 Habib Rostami , Mikhail I. Katsnelson , Marco Polini

The dynamics of electrons and atoms interacting with intense and ultrashort optical pulses presents an important problem in physics that cuts across different materials such as semiconductors and metals. The currently available laser…

Condensed Matter · Physics 2009-10-31 I. E. Perakis , T. V. Shahbazyan

We perform a study of the achievable field enhancement of plasmonic cascade nanolenses in the quantum and classical regimes, and explore the limits enforced at larger sizes by retardation and at smaller sizes by nonlocality and other…

Optics · Physics 2017-12-25 Jamie M. Fitzgerald , Vincenzo Giannini

We use quantum electrodynamics and the confinement-induced nonlocal dielectric response model based on the Keldysh-Rytova electron interaction potential to study the epsilon-near-zero modes of metallic films in the transdimensional regime.…

Mesoscale and Nanoscale Physics · Physics 2020-01-27 Igor V. Bondarev , Hamze Mousavi , Vladimir M. Shalaev

We study the effect of nonlocal optical response on the optical properties of metallic nanowires, by numerically implementing the hydrodynamical Drude model for arbitrary nanowire geometries. We first demonstrate the accuracy of our…

Mesoscale and Nanoscale Physics · Physics 2012-02-07 Giuseppe Toscano , Søren Raza , Antti-Pekka Jauho , N. Asger Mortensen , Martijn Wubs

Cathodoluminescence (CL) microscopy has emerged as a powerful tool for investigating the optical properties of materials at the nanoscale, offering unique insights into the behavior of photonic and plasmonic materials under electron…

Quantum plasmonics is a rapidly growing field of research that involves the study of the quantum properties of light and its interaction with matter at the nanoscale. Here, surface plasmons - electromagnetic excitations coupled to electron…

Quantum Physics · Physics 2013-12-25 M. S. Tame , K. R. McEnery , S. K. Ozdemir , J. Lee , S. A. Maier , M. S. Kim

We develop a theoretical model of the surface plasmon resonance of metallic nanospheres in the size range down to the single nanometer size. Within this model we explicitly show how different microscopic mechanisms, namely quantization due…

Optics · Physics 2013-08-26 R. Carmina Monreal , Tomasz J. Antosiewicz , S. Peter Apell

Within the MNPBEM toolbox, we show how to simulate electron energy loss spectroscopy (EELS) of plasmonic nanoparticles using a boundary element method approach. The methodology underlying our approach closely follows the concepts developed…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Ulrich Hohenester

Scanning transmission electron microscopy (STEM) combined with electron energy loss spectroscopy (EELS) has become a standard technique to map localized surface plasmon resonances with a nanometer spatial and a sufficient energy resolution…

Mesoscale and Nanoscale Physics · Physics 2020-06-02 Michal Horák , Tomáš Šikola

We report on reflection spectra of caesium atoms in close vicinity of a nanostructured metallic meta-surface. We show that the hyperfine sub-Doppler spectrum of the $6S_{1/2} - 6P_{3/2}$ resonance transition at 852 nm is strongly affected…

Mesoscale and Nanoscale Physics · Physics 2016-03-29 Syed Abdullah Aljunid , Eng Aik Chan , Giorgio Adamo , Martial Ducloy , David Wilkowski , Nikolay I. Zheludev

An accurate description of the optical response of subwavelength metallic particles and nanogap structures is a key problem of plasmonics. Quantum hydrodynamic theory (QHT) has emerged as a powerful method to calculate the optical response…

Mesoscale and Nanoscale Physics · Physics 2021-03-17 Henrikh M. Baghramyan , Fabio Della Sala , Cristian Ciracì

We develop a novel approach to ultrafast optical modulation of quantum-mechanical phenomena at the interface of plasmonic metals. Focusing on efficient and versatile nanoparticle-on-mirror plasmonic nanocavities, we discuss indirect control…

Optics · Physics 2026-03-17 Artur Avdizhiyan , Ilya Razdolski , Anton Yu. Bykov

In Yang et al. [Nature 576, 248 (2019)], the authors introduced a general theoretical framework for nanoscale electromagnetism based on Feibelman parameters. Here quantum effects of the optically excited electrons at the interface between…

Mesoscale and Nanoscale Physics · Physics 2022-03-08 Ulrich Hohenester , Gerhard Unger

Geometrical singularities in plasmonic metasurfaces have recently been proposed for the enhancement of light-matter interactions, owing to their broadband light-harvesting properties and extreme plasmon confinement. However, the large…

Mesoscale and Nanoscale Physics · Physics 2020-03-03 Fan Yang , Emanuele Galiffi , Paloma Arroyo Huidobro , John Pendry

We investigate an interplay between quantum geometrical effects and surface plasmons through surface plasmonic structures, based on an electron hydrodynamic theory. First we demonstrate that the quantum nonlinear Hall effect can be…

Mesoscale and Nanoscale Physics · Physics 2022-11-23 Riki Toshio , Norio Kawakami
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