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Photon bunching in incoherent cathodoluminescence (CL) spectroscopy originates from the fact that a single high-energy electron can generate multiple photons when interacting with a material, thus revealing key properties of electron-matter…

Frequency-filtered photon correlations have been proven to be extremely useful in grasping how the detection process alters photon statistics. Harnessing the spectral correlations also permits refinement of the emission and unraveling of…

A common challenge in quantum information processing with photons is the limited ability to manipulate and measure correlated states. An example is the inability to measure picosecond scale temporal correlations of a multi-photon state,…

Single-photon detectors are ``blind" after the detection of a photon, and thereafter display a characteristic recovery in efficiency, during which the number of undetected photons depends on the statistics of the incident light. We show how…

Photons in a nonlinear medium can repel or attract each other, resulting in a strongly correlated quantum many-body system. Typically, such strongly correlated states of light arise from the extreme nonlinearity granted by quantum emitters…

We report on the implementation of a time-multiplexed click detection scheme to probe quantum correlations between different spatial optical modes. We demonstrate that such measurement setups can uncover nonclassical correlations in…

Quantum Physics · Physics 2015-07-08 J. Sperling , M. Bohmann , W. Vogel , G. Harder , B. Brecht , V. Ansari , C. Silberhorn

We demonstrate the generation of Coulomb-correlated pair, triple and quadruple states of free electrons by femtosecond photoemission from a nanoscale field emitter inside a transmission electron microscope. Event-based electron spectroscopy…

Mesoscale and Nanoscale Physics · Physics 2023-11-28 Rudolf Haindl , Armin Feist , Till Domröse , Marcel Möller , John H. Gaida , Sergey V. Yalunin , Claus Ropers

We demonstrate paired generation of a single photo-electron in a quantum dot and a single photon from a single polarization-entangled photon pair that is generated by spontaneous parametric down conversion. The electron is reated in a GaAs…

Transmission electron microscopes (TEMs) enable atomic-scale imaging and characterisation, driving advances across fields from materials science to biology. Quantum correlations, specifically entanglement, may provide a basis for novel…

We propose an alternative formulation of the sensor method presented in [Phys. Rev. Lett 109, 183601 (2012)] for the calculation of frequency-filtered and time-resolved photon correlations. Our approach is based on an algebraic expansion of…

Quantum Physics · Physics 2018-12-26 David I. H. Holdaway , Valentina Notararigo , Alexandra Olaya-Castro

Compact silicon integrated devices, such as micro-ring resonators, have recently been demonstrated as efficient sources of quantum correlated photon pairs. The mass production of integrated devices demands the implementation of fast and…

We demonstrate the generation of quantum-correlated photon-pairs combined with the spectral filtering of the pump field by more than 95dB using Bragg reflectors and electrically tunable ring resonators. Moreover, we perform demultiplexing…

Quantum light is increasingly recognized as a promising resource for developing optical measurement techniques. Particular attention has been paid to enhancing the precision of the measurements beyond classical techniques by using…

Chemical Physics · Physics 2023-10-03 Yuta Fujihashi , Kuniyuki Miwa , Masahiro Higashi , Akihito Ishizaki

Spontaneous processes triggered in a sample by free electrons are commonly regarded as incoherent, and therefore unable to interfere with external light sources. Here, we challenge this concept by showing through first-principles theory…

Classical physics is often a good approximation for quantum systems composed of many interacting particles, although wavepacket dispersion and scattering processes continuously induce delocalization and entanglement. According to…

Nonlinear optical phenomena such as parametric amplification and frequency conversion are typically driven by external optical fields. Free electrons can also act as electromagnetic sources, offering unmatched spatial precision. Combining…

Mesoscale and Nanoscale Physics · Physics 2025-08-04 Leila Prelat , Eduardo J. C. Dias , F. Javier García de Abajo

While the spontaneous emission from independent emitters provides spatially uncorrelated photons - a typical manifestation of quantum randomness, the interference of the coherent scattering leads to a well-defined intensity pattern - a…

Quantum Physics · Physics 2025-12-04 K. Singh , A. Cidrim , A. Kovalenko , T. Pham , O. Číp , L. Slodička , R. Bachelard

Entangling microwave and optical photons is one of the promising ways to realize quantum transduction through quantum teleportation. This paper investigates the entanglement of microwave-optical photon pairs generated from an…

Quantum Physics · Physics 2024-07-30 Changchun Zhong , Fangxin Li , Srujan Meesala , Steven Wood , David Lake , Oskar Painter , Liang Jiang

The emerging field of free-electron quantum optics enables electron-photon entanglement and holds the potential for generating nontrivial photon states for quantum information processing. Although recent experimental studies have entered…

Quantum Physics · Physics 2024-04-04 Zetao Xie , Zeling Chen , Hao Li , Qinghui Yan , Hongsheng Chen , Xiao Lin , Ido Kaminer , Owen D. Miller , Yi Yang

Energy-time entangled photons are critical in many quantum optical phenomena and have emerged as important elements in quantum information protocols. Entanglement in this degree of freedom often manifests itself on ultrafast timescales…

Quantum Physics · Physics 2018-02-07 Jean-Philippe W. MacLean , John M. Donohue , Kevin J. Resch