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We report the synthesis of an ilmenite-type polymorph of Ca$_x$IrO$_3$ distinct from the known post-perovskite and perovskite phases, via low-temperature topochemical Ca$^{2+}$/2Na$^+$ exchange from Na$_2$IrO$_3$. Powder X-ray diffraction…

Materials Science · Physics 2026-02-17 Haruki Kira , Yuya Haraguchi , Wataru Yokoshima , Daisuke Nishio-Hamane , Hiroko Aruga Katori

Octahedral tilting is most common distortion process observed in centrosymmetric perovskite compounds (ABO$_{3}$). Indeed, crucial physical properties of this oxide stem from the tilts of BO$_{6}$ rigid octahedra. In microwave ceramics with…

Materials Science · Physics 2017-10-11 J. E. Rodrigues , D. M. Bezerra , R. C. Costa , P. S. Pizani , A. C. Hernandes

We show with first-principles molecular dynamics the persistence of intrinsic $\langle111\rangle$ Ti off-centerings for BaTiO$_3$ in its cubic paraelectric phase. Intriguingly, these are inconsistent with the Pm$\bar 3$m space group often…

Materials Science · Physics 2022-04-01 Michele Kotiuga , Samed Halilov , Boris Kozinsky , Marco Fornari , Nicola Marzari , Giovanni Pizzi

Ultrasonic attenuation and phase velocity measurements have been carried out in the ferromagnetic perovskites La_{2/3}Ca_{1/3}MnO_3 and La_{2/3}Sr_{1/3}MnO_3. Data show that the transition at the Curie temperature, T_C, changes from first-…

Strongly Correlated Electrons · Physics 2009-11-10 J. Mira , J. Rivas , A. Moreno-Gobbi , M. Perez-Macho , F. Rivadulla

Despite important breakthroughs in the last decade, the calculation of temperature dependent properties of solids still remains a challenging task, especially in the vicinity of structural phase transitions. We show that the combination of…

Materials Science · Physics 2022-06-20 Quintin N. Meier , Natalio Mingo , Ambroise van Roekeghem

Nanostructured proton-conducting ceramics (PCCs) have attracted considerable interest as moderate-temperature proton conductors. Structure dynamics during proton conduction, particularly at grain boundaries, are crucial for stability and…

Density-functional simulations are used to calculate structural properties and high-symmetry phonons of the hypothetical cubic phase, the stable orthorhombic phase and an intermediate tetragonal phase of magnesium silicate perovskite. We…

mtrl-th · Physics 2016-09-07 M. C. Warren , G. J. Ackland

Perovskite material such as BCZT (Ba$_{0.875}$Ca$_{0.125}$(Zr$_{0.125}$Ti$_{0.875}$)O$_{3}$) is well known for its high value of piezoceramic properties and Curie temperature which has potential applications in sensors, actuators,…

Materials Science · Physics 2025-03-27 Debidutta Pradhan , Jagadish Kumar

We carry out a completely first-principles study of the ferroelectric phase transitions in BaTiO$_3$. Our approach takes advantage of two features of these transitions: the structural changes are small, and only low-energy distortions are…

mtrl-th · Physics 2016-09-07 W. Zhong , David Vanderbilt , K. M. Rabe

We report a detailed high-temperature powder neutron diffraction investigation of the structural behavior of the multiferroic GaFeO3 between 296 and 1368 K. Temperature dependent neutron diffraction patterns do not show any appreciable…

Materials Science · Physics 2015-06-12 S. K. Mishra , R. Mittal , R. Singh , M. Zbiri , T. Hansen , H. Schober

The magnetic, electric and thermal properties of the ($Ln_{1-y}$Y$_{y}$)$_{0.7}$Ca$_{0.3}$CoO$_3$ perovskites ($Ln$~=~Pr, Nd) were investigated down to very low temperatures. The main attention was given to a peculiar metal-insulator…

Strongly Correlated Electrons · Physics 2015-05-18 J. Hejtmánek , E. Šantavá , K. Knížek , M. Maryško , Z. Jirák T. Naito , H. Sasaki , H. Fujishiro

The phase transition behaviour of PbTiO3 and BaTiO3 under (111) epitaxial strain is investigated using density-functional theory calculations. From tensile strains of +0.015 to compressive strains of -0.015, PbTiO3 undergoes phase…

Materials Science · Physics 2009-11-13 Riku Oja , Karen Johnston , Johannes Frantti , Risto M. Nieminen

The perovskite-like ferroelectric system PbZr(1-x)Ti(x)O3 (PZT) has a nearly vertical morphotropic phase boundary (MPB) around x=0.45-0.50. Recent synchrotron x-ray powder diffraction measurements by Noheda et al. [Appl. Phys. Lett. 74,…

Materials Science · Physics 2009-10-31 B. Noheda , J. A. Gonzalo , L. E. Cross , R. Guo , S-E. Park , D. E. Cox , G. Shirane

Perovskite structure SrMnO$_3$ is a rare example of a multiferroic material where strain-tuning and/or cation substitution could lead to coinciding magnetic and ferroelectric ordering temperatures, which would then promise strong…

Materials Science · Physics 2018-10-24 Alexander Edström , Claude Ederer

We utilize single-crystal neutron diffraction to study the $C2/m$ structure of potassium hydrogen carbonate (KHCO$_3$) and macroscopic quantum entanglement above the phase transition at $T_c = 318$ K. Whereas split atom sites could be due…

Other Condensed Matter · Physics 2008-07-10 François Fillaux , Alain Cousson , Matthias J. Gutmann

The bilayer perovskite La$_3$Ni$_2$O$_7$ has recently been found to enter a superconducting state under hydrostatic pressure at temperatures as high as 80 K. The onset of superconductivity is observed concurrent with a structural transition…

Superconductivity · Physics 2024-04-15 Luke C. Rhodes , Peter Wahl

The structure and microstrucutre of fully-strained BiCrO3 thin films have been investigated by X-rays diffraction and transmission electron microscopy, at room temperature. Interestingly, three structural variants are simultaneously…

Materials Science · Physics 2010-06-04 Adrian David , Philippe Boullay , Vengadesh Mangalam , Nicolas Barrier , Wilfrid Prellier

We present the results of pressure-dependent far-infrared reflectivity measurements on the multiferroic perovskite BiFeO3 at room temperature. The observed behavior of the infrared-active phonon modes as a funtion of pressure clearly…

Other Condensed Matter · Physics 2007-12-06 A. Pashkin , K. Rabia , S. Frank , C. A. Kuntscher , R. Haumont , R. Saint-Martin , J. Kreisel

Nitride perovskites are supposed to exhibit excellent properties as oxide analogues and may even have better performance in specific fields for their more covalent characters. However, till now, very limited nitride perovskites have been…

Materials Science · Physics 2020-12-02 Churen Gui , Shuai Dong

Structural phase transitions in the organic inorganic metal halide perovskites are driven via rearrangement of methylammonium cation and distortion in the PbX6 octahedra. Compositional tuning is usually incorporated for suppression of the…