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BaFe$_2$S$_3$ is a quasi one-dimensional Mott insulator that orders antiferromagnetically below 117(5)\,K. The application of pressure induces a transition to a metallic state, and superconductivity emerges. The evolution of the magnetic…

Transition metal phosphorous trichalcogenides, $M{\rm P}X_3$ ($M$ and $X$ being transition metal and chalcogen elements respectively), have been the focus of substantial interest recently because of their possible magnetism in the…

Strongly Correlated Electrons · Physics 2019-12-05 Heung-Sik Kim , David Vanderbilt , Kristjan Haule

The pressure-induced insulator to metal transition (IMT) of layered magnetic nickel phosphorous tri-sulfide NiPS3 was studied in-situ under quasi-uniaxial conditions by means of electrical resistance (R) and X-ray diffraction (XRD)…

Strongly Correlated Electrons · Physics 2021-11-23 Takahiro Matsuoka , Amanda Haglund , Rui Xue , Jesse S. Smith , Maik Lang , Antonio M. dos Santos , David Mandrus

We present the observation of an isostructural Mott insulator-metal transition in van-der-Waals honeycomb antiferromagnet V$_{0.9}$PS$_3$ through high-pressure x-ray diffraction and transport measurements. The MPX$_3$ family of magnetic…

Strongly Correlated Electrons · Physics 2019-03-27 M. J. Coak , S. Son , D. Daisenberger , H. Hamidov , C. R. S. Haines , P. L. Alireza , A. R. Wildes , C. Liu , S. S. Saxena , J. -G. Park

Layered van-der-Waals 2D magnetic materials are of great interest in fundamental condensed-matter physics research, as well as for potential applications in spintronics and device physics. We present neutron powder diffraction data using…

Two-dimensional materials have proven to be a prolific breeding ground of new and unstudied forms of magnetism and unusual metallic states, particularly when tuned between their insulating and metallic phases. In this paper we present work…

Strongly Correlated Electrons · Physics 2019-01-02 C. R. S. Haines , M. J. Coak , G. I. Lampronti , C. Liu , H. Hamidov , A. R. Wildes , D. Daisenberger , P. Nahai-Williamson , S. S. Saxena

Recently discovered class of 2D materials based on transition metal phosphorous trichalcogenides exhibit antiferromagnetic ground state, with potential applications in spintronics. Amongst them, FePS$ _{3} $ is a Mott insulator with a band…

The engineering of magnetic order and electronic states in two-dimensional (2D) materials is pivotal for advanced spintronic technologies. Despite their potential, the scarcity of intrinsic 2D ferromagnets remains a critical challenge.…

Mesoscale and Nanoscale Physics · Physics 2025-03-17 Dong Liu , Sike Zeng , Ji-Hai Liao , Yu-Jun Zhao

We present a detailed NMR study of the insulator to metal transition induced by an applied pressure $p$ in the A15 phase of Cs$_{3}$C$_{60}$. We evidence that the insulating antiferromagnetic (AF) and superconducting (SC) phases only…

Strongly Correlated Electrons · Physics 2017-06-14 H. Alloul , P. Wzietek , T. Mito , D. Pontiroli , M. Aramini , M. Riccò , J. P. Itié , E. Elkaim

Layered magnetic transition-metal thiophosphate NiPS3 has unique two-dimensional (2D) magnetic properties and electronic behavior. The electronic band structure and corresponding magnetic state are expected to sensitive to the interlayer…

Strongly Correlated Electrons · Physics 2020-09-30 Xiaoli Ma , Yimeng Wang , Yunyu Yin , Binbin Yue , Jianhong Dai , Jianting Ji , Feng Jin , Fang Hong , Jian-Tao Wang , Qingming Zhang , Xiaohui Yu

We study the Mott transition, antiferromagnetism and superconductivity in layered organic conductors using Cellular Dynamical Mean Field Theory for the frustrated Hubbard model. A d-wave superconducting phase appears between an…

Strongly Correlated Electrons · Physics 2009-11-11 B. Kyung , A. -M. S. Tremblay

A new compound with a quasi-two-dimensional array of FeSe3O tetrahedra and an orthorombic structure, namely BaFe2Se2O, has been successfully fabricated. Experimental results show that this compound is an insulator and has an…

Strongly Correlated Electrons · Physics 2015-06-05 Fei Han , Xiangang Wan , Bing Shen , Hai-Hu Wen

We use elastic and inelastic neutron scattering (INS) to study the antiferromagnetic (AF) phase transitions and spin excitations in the two-dimensional (2D) zig-zag antiferromagnet FePSe$_3$. By determining the magnetic order parameter…

Strongly Correlated Electrons · Physics 2024-02-28 Lebing Chen , Xiaokun Teng , Ding Hu , Feng Ye , Garrett E. Granroth , Ming Yi , Jae-Ho Chung , Robert J. Birgeneau , Pengcheng Dai

The pressure effects on the antiferromagentic orders in iron-based ladder compounds CsFe$_2$Se$_3$ and BaFe$_2$S$_3$ have been studied using neutron diffraction. With identical crystal structure and similar magnetic structures, the two…

All the iron-based superconductors identified to date share a square lattice composed of Fe atoms as a common feature, despite having different crystal structures. In copper-based materials, the superconducting phase emerges not only in…

The one-third monolayer Sn layer on Si(111) has long been considered a benchmark system for exploring two-dimensional Mott physics, owing to its narrow bandwidth and sizable on-site Coulomb repulsion. Previous experiments suggested the…

NiPS3 is an exfoliable van-der-Waals intralayer antiferromagnet with zigzag-type spin arrangement. It is distinct from other TMPS3 (TM: transition metal) materials by optical excitations into a strongly correlated state that is tied to the…

Intrinsic magnetic topological insulators provide an ideal platform to achieve various exciting physical phenomena. However, this kind of materials and related research are still very rare. In this work, we reported the electronic and…

BaFe2Se3 is a potential superconductor material exhibiting transition at 11 K and ambient pressure. Here we extended the structural and performed electrical resistivity measurements on this compound up to 51 GPa and 20 GPa, respectively, in…

Temperature dependence of resistivity under high pressures with magnetic fields parallel and perpendicular to the FeSe planes are measured in FeSe single crystals. It is found that the structural transition (nematic) temperature is…

Superconductivity · Physics 2019-03-06 Guan-Yu Chen , Enyu Wang , Xiyu Zhu , Hai-Hu Wen
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