Related papers: Relation Between Photoionisation Cross Sections an…
Attosecond interferometry in a two-color field is central to attosecond metrology and spectroscopy. In this technique, a photoelectron wave packet is released when a single photon from an extreme ultraviolet comb is absorbed. The wave…
We present a robust, ab initio method for addressing atom-light interactions and apply it to photoionization of argon. We use a close-coupling ansatz constructed on a multi-configurational Hartree-Fock description of localized states and…
We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…
To measure and control the electron motion in atoms and molecules by the strong laser field on the attosecond time scale is one of the research frontiers of atomic and molecular photophysics. It involves many new phenomena and processes and…
We present fully ab initio simulations of attosecond streaking for ionization of helium accompanied by shake-up of the second electron. This process represents a prototypical case for strongly correlated electron dynamics on the attosecond…
In this study, we have investigated the photoionization cross section of an on-center hydrogenic impurity in a multi-layered spherical quantum dot. The electronic energy levels and their wave functions have been determined fully numerically…
Photoionization cross sections and rate coefficients have been calculated for all bound vibrational levels of the 1s$\sigma_{\mathrm{g}}$ state of H$_{2}^{+}$, HD$^{+}$, and D$_{2}^{+}$. The Born-Oppenheimer approximation is employed in our…
A graphical presentation of the timing of avalanche photodiode events in the datasets from the experiment of Weihs et al. [Phys. Rev. Lett. 81, 5039 (1998)] makes manifest the existence of two types of signal delay: (1) The introduction of…
Attosecond dynamics in strong-field tunnel ionization are encoded in intricate holographic patterns in the photoelectron momentum distributions (PMDs). These patterns show the interference between two or more superposed quantum electron…
The generation of a streaking spectrogram is based on energy absorption from the streaking laser. Investigating this absorption we show rigorously under which condition the measured time shift is independent of properties of the streaking…
Attosecond interferometry (AI) is an experimental technique based on ionizing a system with an attosecond pulse train in the presence of an assisting laser. This assisting laser provides multiple pathways for the photoelectron wave packet…
The phasing problem of heterodyne-detected nonlinear spectroscopy states that the relative time delay between the exciting pulses and a local oscillator must be known with subcycle precision to separate absorptive and dispersive…
Angular dependence of photoemission time delay for the valence $np_{3/2}$ and $np_{1/2}$ subshells of Ar, Kr and Xe is studied in the dipole relativistic random phase approximation. Strong angular anisotropy of the time delay is reproduced…
Coherent processing of quantum information and attosecond science had so far little in common. We here show that recent data in high harmonic emission reveal quantum information processing at the attosecond timescale. By observing the…
We solve the time-dependent Schr\"odinger equation describing a water molecule driven by a superposition of the XUV and IR pulses typical for a RABBITT experiment. This solution is obtained by a combination of the time-dependent coordinate…
A clear consensus on how long it takes a particle to tunnel through a potential barrier has never been so urgently required, since the electron dynamics in strong-field ionization can be resolved on attosecond time-scale in experiment and…
Tunneling ionization is characterized by a negative time delay, observed asymptotically as a specific shift of the photoelectron momentum distribution, which is caused by the interference of the sub-barrier recolliding and direct ionization…
The implementation of attosecond photoelectron-photoion coincidence spectroscopy for the investigation of atomic and molecular dynamics calls for a high-repetition-rate driving source combined with experimental setups characterized by…
We consider the general expressions for the time delay of photons of different energies in the framework of multi-dimensional cosmological models. In models with compactified extra-dimensions (Kaluza-Klein type models), the main source of…
In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…