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By means of Dynamical Mean-Field Theory we investigate the spin response function of a model for correlated materials with d- or f-electrons hybridized with more delocalized ligand orbitals. We point out the existence of two different…

Strongly Correlated Electrons · Physics 2013-10-14 A. Amaricci , N. Parragh , M. Capone , G. Sangiovanni

The near nucleus behavior of the exchange-correlation potential $v_{xc}({\bf r})$ in Hohenberg-Kohn-Sham density functional theory is investigated. It is shown that near the nucleus the linear term of $O(r)$ of the spherically averaged…

Materials Science · Physics 2009-11-13 Zhixin Qian

The reconstruction of the exchange-correlation potential from accurate ab initio electron densities can provide insights into the limitations of the currently available approximate functionals and provide guidance for devising improved…

Strongly Correlated Electrons · Physics 2013-02-05 Katharina Boguslawski , Christoph R. Jacob , Markus Reiher

We propose a method to determine the magnetic exchange interaction and on-site anisotropy tensors of extended Heisenberg spin models from density functional theory including relativistic effects. The method is based on the…

We introduce a new class of exchange-correlation potentials for a static and time-dependent Density Functional Theory of strongly correlated systems in 3D. The potentials are obtained via Dynamical Mean Field Theory and, for strong enough…

Strongly Correlated Electrons · Physics 2015-05-18 Daniel Karlsson , Antonio Privitera , Claudio Verdozzi

The dynamics of magnetization in the presence of spin-transfer torque was studied. We derived the equation for the motion of magnetization in the presence of a spin current by using the local equilibrium assumption in non-equilibrium…

Mesoscale and Nanoscale Physics · Physics 2008-08-07 Kazuhiko Seki , Hiroshi Imamura

The polarization-dependence of the exchange-correlation (XC) energy functional of periodic insulators within Kohn-Sham (KS) density-functional theory requires a ${\cal O} (1/q^2)$ divergence in the XC kernel for small vectors q. This…

Materials Science · Physics 2009-10-30 Ph. Ghosez , X. Gonze , R. W. Godby

A spin angular gradient approximation for the exchange correlation magnetic field in the density functional formalism is proposed. The usage of such corrections leads to a consistent spin dynamical approach beyond the local approximation.…

Strongly Correlated Electrons · Physics 2009-11-07 M. I. Katsnelson , V. P. Antropov

A description of non-collinear magnetism in the framework of spin-density functional theory is presented for the exact exchange energy functional which depends explicitly on two-component spinor orbitals. The equations for the effective…

We utilize simulations of electron scattering by a chain of dynamical quantum spins, to analyze the interplay between the spin transfer effect and the magnetization dynamics. We show that the complex interactions between the spin-polarized…

Materials Science · Physics 2021-04-21 Neil Tramsen , Alexander Mitrofanov , Sergei Urazhdin

The density functional theory (DFT) is a remarkably successful theory of electronic structure of matter. At the foundation of this theory lies the Kohn-Sham (KS) equation. In this paper, we describe the long-time behaviour of the…

Analysis of PDEs · Mathematics 2021-05-11 Fabio Pusateri , Israel Michael Sigal

The influence of correlation effects on the orbital moments for transition metals and their alloys is studied by first-principle relativistic Density Functional Theory in combination with the Dynamical Mean-Field Theory. In contrast to the…

Strongly Correlated Electrons · Physics 2009-11-13 S. Chadov , J. Minár , M. I. Katsnelson , H. Ebert , D. Ködderitzsch , A. I. Lichtenstein

A well-known connection between the magnetic susceptibility and the effective exchange parameter is analyzed. It is shown that all current computational schemes use a long-wave approximation which is suitable only for localized moments…

Strongly Correlated Electrons · Physics 2009-11-07 V. P. Antropov

We introduce a new functional for simulating ground-state and time-dependent electronic systems within density-functional theory. The functional combines an expression for the exact Kohn-Sham (KS) potential in the limit of complete electron…

Mesoscale and Nanoscale Physics · Physics 2021-01-15 M. J. P. Hodgson , J. D. Ramsden , T. R. Durrant , R. W. Godby

A brief survey of the author's works on the quantum theory of magnetism. Theoretical foundation and applications of the generalized spin-fermion (sp-d) exchange lattice model to various magnetic systems, e.g., rare-earth metals and…

Strongly Correlated Electrons · Physics 2007-05-23 A. L. Kuzemsky

For more than three decades, clear discrepancies have existed between spin densities in momentum space revealed by Magnetic Compton scattering experiments and theoretical calculations based on density functional theory (DFT). Here by making…

Strongly Correlated Electrons · Physics 2024-02-02 A. D. N. James , E. I. Harris-Lee , S. B. Dugdale

A fundamental weakness of density functional theory (DFT) is the difficulty in making systematic improvements to approximations for the exchange and correlation functionals. In this paper, we follow a wave-function-based approach [N.I.…

Chemical Physics · Physics 2018-10-05 Timothy J. Callow , Nikitas I. Gidopoulos

We discuss an efficient scheme for obtaining spin-polarized quasi-particle excitation energies within the general framework of the density functional theory (DFT). Our approach is to correct the DFT eigenvalues via the electrostatic energy…

Strongly Correlated Electrons · Physics 2007-10-11 B. Barbiellini , A. Bansil

A new electronic structure principle, viz. the minimum magnetizability principle (MMP) has been proposed and also has been verified through ab initio calculations, to extend the domain of applicability of the conceptual density functional…

Chemical Physics · Physics 2009-11-11 Akhilesh Tanwar , Debesh Ranjan Roy , Sourav Pal , Pratim Kumar Chattaraj

This work builds a bridge between density functional theory (DFT) and model interpretations of Anderson's superexchange theory by constructing a $f$-$d$-$p$ model with DFT Wannier functions to enable a direct quantum many-body solution…

Materials Science · Physics 2020-11-03 Dian-Teng Chen , Jia Chen , Xiang-Guo Li , George Christou , Xiao-Guang Zhang , Hai-Ping Cheng
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