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High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

We show that optical second-harmonic generation (SHG) can be observed from individual single-walled carbon nanotubes (SWCNTs) and, furthermore, allows imaging of individual tubes. Detailed analysis of our results suggests that the…

Nanoparticles of Ferric Chloride doped ZnS has been synthesized by simple chemical precipitation method and characterized by XRD, SEM, UV-Vis analysis, Differential Thermal Analysis, Thermo Gravimetric Analysis and Differential Scanning…

Chemical Physics · Physics 2013-03-12 T. Theivasanthi , N. Kartheeswari , M. Alagar

We study the second harmonic generation (SHG) in a suspension of small spherical particles confined within a slab, assuming undepleted pump and applying (i) single scattering approximation and (ii) diffusion approximation. In the case (i),…

Optics · Physics 2007-05-23 E. V. Makeev , S. E. Skipetrov

We demonstrate the first achievement of continuous-wave (CW) pumped second harmonic generation (SHG) in few- and mono-layer gallium selenide (GaSe) flakes, which are coated on silicon photonic crystal (PC) cavities. Because of ultrahigh…

We report calculated substantial enhancement of the second harmonic generation (SHG) in cuprous oxide crystals resonantly hybridized with an appropriate organic material (DCM2:CA:PS 'solid-state solvent'). The quadrupole origin of the…

Materials Science · Physics 2009-11-13 Oleksiy Roslyak , Joseph L. Birman

Optical spectroscopy based on second-order nonlinearity is a critical technique for characterizing two-dimensional (2D) crystals as well as bioimaging and quantum optics. It is generally believed that second-harmonic generation (SHG) in…

Mesoscale and Nanoscale Physics · Physics 2026-01-14 Haoning Tang , Zhitong Ding , Tianyi Ruan , Zeyu Hao , Kenji Watanabe , Takashi Taniguchi , Haozhe Wang , Ali Javey , Feng Wang , Yuan Cao

Recent experiments and calculations in topological semimetals have observed anomalously strong second-order optical nonlinearity, but yet whether the enhancement also occurs at surfaces of topological semimetals in general remains an open…

Second harmonic generation in a two dimensional nonlinear quasi-crystal is demonstrated for the first time. Temperature and wavelength tuning of the crystal reveal the uniformity of the pattern while angle tuning reveals the dense nature of…

Optics · Physics 2007-05-23 Neil Broderick , Anna Peacock , Katia Gallo , Ruth Lewen , Radu Bratfalean

Optical coating, an integral part of many optical systems, is prone to damage from environmental exposure and laser irradiation. This underscores the need for reliable and sensitive coating diagnostics. We introduce second harmonic…

Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…

We conduct a theoretical and numerical study on the second-harmonic (SH) optical response of a nano-structured metamaterial composed of a periodic array of inclusions. Both the inclusions and their surrounding matrix are made of…

Mesoscale and Nanoscale Physics · Physics 2019-03-13 Ulises R. Meza , Bernardo S. Mendoza , W. Luis Mochán

We demonstrate enhanced second harmonic generation in a gallium phosphide photonic crystal waveguide with a measured external conversion efficiency of 5$\times10^{-7}$/W. Our results are promising for frequency conversion of on-chip…

Optics · Physics 2015-05-28 Kelley Rivoire , Sonia Buckley , Fariba Hatami , Jelena Vuckovic

We investigate the generation of ultraviolet (UV) second-harmonic radiation on the boundary of a UV transparent crystal, which is derived from the automatic partial phase matching of the incident wave and the total internal reflection. By…

Optics · Physics 2016-12-19 Xiaohui Zhao , Yuanlin Zheng , Huaijin Ren , Ning An , Xuewei Deng , Xianfeng Chen

We analytically investigate the effect of a non-centrosymmetric geometry in the optical second harmonic (SH) generation from a particle made of a centrosymmetric material, in the interior of which quadratic optical processes are suppressed.…

Optics · Physics 2019-03-27 Raksha Singla , W. Luis Mochán

We show that the lack of inversion symmetry in monolayer MoS2 allows strong optical second harmonic generation. Second harmonic of an 810-nm pulse is generated in a mechanically exfoliated monolayer, with a nonlinear susceptibility on the…

Materials Science · Physics 2015-06-15 Nardeep Kumar , Sina Najmaei , Qiannan Cui , Frank Ceballos , Pulickel M. Ajayan , Jun Lou , Hui Zhao

Nano-resonator integrated with two-dimensional materials (e.g. transition metal dichalcogenides) have recently emerged as a promising nano-optoelectronic platform. Here we demonstrate resonatorenhanced second-harmonic generation (SHG) in…

The crystal structure of La 4 Ge 3S 12 has been known to be noncentrosymmetric for almost four decades. This characteristic inversion symmetry breaking suggests the presence of nonlinear optical properties. Yet only recently have nonlinear…

Materials Science · Physics 2026-02-19 Hiroya Ohtsuki , Suguru Nakata , Yu Yamane , Ryunosuke Takahashi , Koichi Kusakabe , Hiroki Wadati

We present a comprehensive tensorial characterization of second-harmonic generation from silicon nitride films with varying composition. The samples were fabricated using plasma-enhanced chemical vapor deposition, and the material…

Hydrogen sulfide (H2S) is a prototype molecular system and a sister molecule of water. The phase diagram of solid H2S at high pressures remains largely unexplored arising from the challenges in dealing with the looser S-H bond and larger…

Superconductivity · Physics 2015-03-26 Yinwei Li , Jian Hao , Yanling Li , Yanming Ma