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Recent studies have demonstrated that the polarization states of high harmonics from solids can differ from those of the driving pulses. To gain insights on the microscopic origin of this behavior, we perform one-particle intraband-only…

We apply the theory of high-order harmonic generation by low-frequency laser fields in the strong field approximation to the study of the spatial and temporal coherence properties of the harmonics. We discuss the role of dynamically induced…

Quantum Physics · Physics 2007-05-23 Pascal Salières , Anne L'Huillier , Philippe Antoine , Maciej Lewenstein

High-order harmonic generation (HHG) in aligned linear molecules can offer valuable information about strong-field interactions in lower-lying molecular orbitals, but extracting this information is difficult for three-dimensional molecular…

We theoretically investigate the interference effect of high-order harmonics generated from molecules at different alignment angles. It is shown that the interference of the harmonic emissions from molecules aligned at different angles can…

Optics · Physics 2015-02-27 Meiyan Qin , Xiaosong Zhu , Yang Li , Qingbin Zhang , Pengfei Lan , Peixiang Lu

The present work reports on the generation of short-pulse coherent extreme ultraviolet radiation of controlled polarization. The proposed strategy is based on high-order harmonics generated in pre-aligned molecules. Field-free molecular…

Two different induced effects of a laser falling edge on high-order harmonic generation are resolved by solving numerically full-dimensional electronic time-dependent Schr\"{o}dinger equation beyond the Born-Oppenheimer approximation. The…

Atomic Physics · Physics 2017-02-01 M. Vafaee , H. Ahmadi , A. Maghari

High-order harmonic generation via single-slit diffraction of relativistic laser pulses is investigated. Using fully kinetic 2D and 3D particle-in-cell simulations, we show that interesting optical phenomena emerge, including the generation…

Plasma Physics · Physics 2025-05-07 Longqing Yi

In this work using three-dimensional particle-in-cell simulations and analytical considerations we demonstrate intense high-order plasma surface harmonics carrying a time-varying orbital angular momentum (OAM) -- the self-torque. We show…

Plasma Physics · Physics 2022-01-03 Jingwei Wang , Matt Zepf , Yuxin Leng , Ruxin Li , Sergey G. Rykovanov

We study ionization of atoms in strong elliptically-polarized laser fields numerically and analytically. We focus on effects of laser ellipticity on the offset angle in photoelectron momentum distribution. This angle is considered to encode…

Atomic Physics · Physics 2023-04-26 J. Y. Che , J. Y. Huang , F. B. Zhang , C. Chen , G. G. Xin , Y. J. Chen

We study theoretically the two-center interferences occurring in high harmonic generation from diatomic molecules. By solving the time-dependent Schroedinger equation, either numerically or with the molecular strong-field approximation, we…

We investigate the polarization properties of high harmonics generated with the bichromatic counterrotating circularly polarized (BCCP) laser fields by numerically solving time-dependent Schr\"odinger equation (TDSE). It is found that, the…

Atomic Physics · Physics 2016-12-21 Xiaofan Zhang , Liang Li , Xiaosong Zhu , Xi Liu , Qingbin Zhang , Pengfei Lan , Peixiang Lu

We present a theoretical analysis of high-order harmonic generation from ion-atom collisions in the presence of linearly polarized intense laser pulses. Photons with frequencies significantly higher than in standard atomic high-harmonic…

Atomic Physics · Physics 2009-11-10 Manfred Lein , Jan M. Rost

Electromagnetic radiation at higher harmonics of the plasma frequency ($\omega \sim n\omega_{pe}, n > 2$) has been occasionally observed in type II and type III solar radio bursts, yet the underlying mechanism remains undetermined. Here we…

Solar and Stellar Astrophysics · Physics 2023-12-22 Chuanyang Li , Yao Chen , Zilong Zhang , Hao Ning , TangMu Li

We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic…

Recent reports on intense-field pump-probe experiments for high harmonic generation from coherently rotating linear molecules, have revealed remarkable characteristic effects of the simultaneous variation of the polarization geometry and…

Atomic and Molecular Clusters · Physics 2009-11-13 F. H. M. Faisal , A. Abdurrouf

We consider the formation of RbCs by an elliptically polarized laser pulse. By varying the ellipticity of the laser for sufficiently large laser intensity, we see that the formation probability presents a strong dependence, especially…

Atomic Physics · Physics 2019-02-06 J. Pablo Salas , Cristel Chandre , J Salas

We present a theoretical model of high-harmonic generation from diatomic molecules. The theory includes effects of alignment as well as nuclear motion and is used to predict results for N$_2$, O$_2$, H$_2$ and D$_2$. The results show that…

Atomic Physics · Physics 2007-05-23 Christian Bruun Madsen , Lars Bojer Madsen

Based upon our previous works (Eur.Phys.J.D 6, 319(1999); Chin.Phys.Lett. 18, 236(2001)), we develop a classical approach to calculate the high-order harmonic generation of the laser driven atoms and molecules. The Coulomb singularities in…

Atomic Physics · Physics 2007-05-23 Chaohong Lee , Yiwu Duan , Wing-Ki Liu , Jian-Min Yuan , Lei Shi , Xiwen Zhu , Kelin Gao

The generation of high-order harmonics in a medium of chiral molecules driven by intense bi-elliptical laser fields can lead to strong chiroptical response in a broad range of harmonic numbers and ellipticities [D. Ayuso et al, J. Phys. B…

Optics · Physics 2018-07-04 David Ayuso , Piero Decleva , Serguei Patchkovskii , Olga Smirnova

We investigate the effect on high-order harmonic generation of the distortion of molecular orbitals by the driving laser field. Calculations for high-order harmonic generation including orbital distortion are performed for N2. Our results…

Atomic Physics · Physics 2015-06-15 Maciej Dominik Śpiewanowski , Adam Etches , Lars Bojer Madsen