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The process of reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) reveals the target atom electronic structure when one of the transitions proceeds from below the ionization threshold. Such an…

Atomic Physics · Physics 2021-09-14 Anatoli Kheifets

We calculate the transient absorption of an isolated attosecond pulse by helium atoms subject to a delayed infrared (\ir) laser pulse. With the central frequency of the broad attosecond spectrum near the ionization threshold, the absorption…

Atomic Physics · Physics 2015-06-12 Shaohao Chen , Mengxi Wu , Mette B. Gaarde , Kenneth J. Schafer

We present R-Matrix with time dependence (RMT) calculations for the photoionization of helium irradiated by an EUV laser pulse and an overlapping IR pulse with an emphasis on the anisotropy parameters of the sidebands generated by the…

Atomic Physics · Physics 2015-06-23 H. F. Rey , H. W. van der Hart

We employ Reconstruction of Attosecond Beating By Interference of Two-photon Transitions with an advanced energy resolution (rainbow RABBITT) to resolve under-threshold discrete excitations and above-threshold auto-ionizing states in the He…

Atomic Physics · Physics 2025-02-14 Vladislav Serov , Anatoli Kheifets

Following up on a recent paper [Bharti et al., Phys. Rev. A 109 (2024) 023110], we compare the predictions from severalR-matrix with time-dependence calculations for a modified three-sideband version of the "reconstruction of attosecond…

Atomic Physics · Physics 2024-04-05 A. T. Bondy , J. C. del Valle , S. Saha , K. R. Hamilton , D. Bharti , A. Harth , K. Bartschat

Angular dependence of photoemission time delay for the valence $np_{3/2}$ and $np_{1/2}$ subshells of Ar, Kr and Xe is studied in the dipole relativistic random phase approximation. Strong angular anisotropy of the time delay is reproduced…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets , Ankur Mandal , P. C. Deshmukh , V. K. Dolmatov , S. T. Manson

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach due to the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we…

Time delays of electrons emitted from an isotropic initial state and leaving behind an isotropic ion are assumed to be angle-independent. Using an interferometric method involving XUV attosecond pulse trains and an IR probe field in…

We investigate theoretically the relative time delay of photoelectrons originating from different atomic subshells of noble gases. This quantity was measured via attosecond streaking and studied theoretically by Schultze et al. [Science…

Atomic Physics · Physics 2015-06-22 Jonas Wätzel , Andrey Moskalenko , Yaroslav Pavlyukh , Jamal Berakdar

Focused laser fields with textured polarization on a sub-wavelength scale allow extracting information on electronic processes which are not directly accessible by homogeneous fields. Here, we consider photoionization in radially and…

Atomic Physics · Physics 2021-06-30 Jonas Wätzel , Jamal Berakdar

After photon absorption, electrons from a dispersive band of a solid require a finite time in the photoemission process before being photoemitted as free particles, in line with recent attosecondresolved photoemission experiments. According…

Mesoscale and Nanoscale Physics · Physics 2017-02-15 Mauro Fanciulli , Henrieta Volfová , Stefan Muff , Jürgen Braun , Hubert Ebert , Jan Minár , Ulrich Heinzmann , J. Hugo Dil

We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…

Atomic Physics · Physics 2015-03-06 Stefan Nagele , Renate Pazourek , Michael Wais , Georg Wachter , Joachim Burgdörfer

A technique for measuring photoionization time delays with attosecond precision is combined with calculations of photoionization matrix elements to demonstrate how multi-electron dynamics affect photoionization time delays in carbon…

We propose a new scheme to control the shape of the Autler-Townes (AT) doublet in the photoelectron spectrum from atomic resonance-enhanced multiphoton ionization (REMPI). The scheme is based on the interference of two AT doublets created…

Atomic Physics · Physics 2025-07-01 T. Bayer , K. Eickhoff , D. Köhnke , M. Wollenhaupt

We theoretically study the photoelectron angular distributions (PADs) from two-color two-photon near-threshold ionization of hydrogen and noble gas (He, Ne, and Ar) atoms by a combined action of femtosecond extreme ultraviolet (EUV) and…

Atomic Physics · Physics 2015-06-22 Kenichi L. Ishikawa , A. K. Kazansky , N. M. Kabachnik , Kiyoshi Ueda

Photoionization from energetically distinct electronic states may have a relative time delay of tens of attoseconds. Here we demonstrate that pulses of optical vortices allow measuring such attoseconds delays from magnetic sublevels, even…

Atomic Physics · Physics 2016-10-03 Jonas Wätzel , Jamal Berakdar

We revisit the time-resolved photoemission in neon atoms as probed by attosecond streaking. We calculate streaking time shifts for the emission of 2p and 2s electrons and compare the relative delay as measured in a recent experiment by…

Ab initio simulations of a range of interferometric experiments are used to identify a strong dependence on multiphoton phase shifts in above-threshold ionization. A simple rule of thumb for interaction phase shifts is derived to explain…

Atomic Physics · Physics 2021-03-31 Mattias Bertolino , Jan Marcus Dahlström

We solve the time-dependent Schr\"odinger equation describing a water molecule driven by a superposition of the XUV and IR pulses typical for a RABBITT experiment. This solution is obtained by a combination of the time-dependent coordinate…

Atomic Physics · Physics 2018-01-17 Vladislav V. Serov , A. S. Kheifets

The attosecond high harmonic pulses obtained from a long Ar-filled gas cell were characterized by two techniques - the reconstruction of attosecond beating by interference of two-photon transition (RABITT) and frequency-resolved optical…