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Edge/surface states often appear in a topologically nontrivial phase, when the system has a boundary. The edge state of a one-dimensional topological insulator is one of the simplest examples. Electron Spin Resonance (ESR) is an ideal probe…

Strongly Correlated Electrons · Physics 2017-11-21 Yuan Yao , Masahiro Sato , Tetsuya Nakamura , Nobuo Furukawa , Masaki Oshikawa

Electron Spin Resonance (ESR) describes a suite of techniques for characterising electronic systems, with applications in physics, materials science, chemistry, and biology. However, the requirement for large electron spin ensembles in…

Quantum Physics · Physics 2015-03-04 L. T. Hall , P. Kehayias , D. A. Simpson , A. Jarmola , A. Stacey , D. Budker , L. C. L. Hollenberg

Electron paramagnetic resonance (EPR) spectroscopy is widely employed to characterize paramagnetic complexes. Recently, EPR combined with scanning tunneling microscopy (STM) achieved single-spin sensitivity with sub-angstrom spatial…

Mesoscale and Nanoscale Physics · Physics 2020-10-09 Tom S. Seifert , Stepan Kovarik , Dominik M. Juraschek , Nicola A. Spaldin , Pietro Gambardella , Sebastian Stepanow

We present a general method to realize resonant coupling between spins even though their energies are of different scales. Applying the method to the electron and nuclear spin systems such as a nitrogen-vacancy (NV) center with its nearby…

Quantum Physics · Physics 2023-11-20 Sichen Xu , Chanying Xie , Zhen-Yu Wang

Electron spin resonance (ESR) spectroscopy is the method of choice for characterizing paramagnetic impurities, with applications ranging from chemistry to quantum computing, but it gives access only to ensemble-averaged quantities due to…

Electron paramagnetic resonance (EPR) performed with a scanning tunneling microscope (STM) allows for probing the spin excitation of single atomic species with MHz energy resolution. One of the basic applications of conventional EPR is the…

Mesoscale and Nanoscale Physics · Physics 2021-11-10 Tom S. Seifert , Stepan Kovarik , Pietro Gambardella , Sebastian Stepanow

Quantum spin networks having engineered geometries and interactions are eagerly pursued for quantum simulation and access to emergent quantum phenomena such as spin liquids. Spin-1/2 centers are particularly desirable because they readily…

We report on electron spin resonance (ESR) measurements of phosphorus donors localized in a 200 square micron area below the inductive wire of a lumped element superconducting resonator. By combining quantum limited parametric amplification…

Mesoscale and Nanoscale Physics · Physics 2017-02-10 C. Eichler , A. J. Sigillito , S. A. Lyon , J. R. Petta

Scaling up qubits is a necessary step to realize useful systems of quantum computation. Here we demonstrate coherent manipulations of four individual electron spins using a micro-magnet method in a quadruple quantum dot - the largest number…

Electron spin resonance with a scanning tunneling microscope (ESR-STM) combines the high energy resolution of spin resonance spectroscopy with the atomic scale control and spatial resolution of STM. Here we describe the upgrade of a…

Instrumentation and Detectors · Physics 2019-01-30 Fabian D. Natterer , François Patthey , Tobias Bilgeri , Patrick R. Forrester , Nicolas Weiss , Harald Brune

Electron spin resonance spectroscopy (ESR) of a single electron in planar Si-MOS quantum dot is reported in the vicinity of a valley level anti-crossing. A number of one and two-photon resonances are observed due to mixing of magnetic…

Quantum dots patterned by atomically precise placement of phosphorus donors in single crystal silicon have long spin lifetimes, advantages in addressability, large exchange tunability, and are readily available few-electron systems. To be…

Mesoscale and Nanoscale Physics · Physics 2016-07-06 Yu Wang , Chin-Yi Chen , Gerhard Klimeck , Michelle Y. Simmons , Rajib Rahman

Quantum control techniques play an important role in manipulating and harnessing the properties of different quantum systems, including isolated atoms. Here, we propose to achieve quantum control over a single on-surface atomic spin using…

Spin-orbit (SO) interaction critically influences electron spin dynamics and spin transport in bulk semiconductors and semiconductor microstructures. This interaction couples electron spin to dc and ac electric fields. Spin coupling to ac…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Emmanuel I. Rashba

Hyperfine interactions between electron and nuclear spins have been widely used in material science, organic chemistry, and structural biology as a sensitive probe to the local chemical environment through spatial identification of nuclear…

Mesoscale and Nanoscale Physics · Physics 2022-12-28 Jinkyung Kim , Kyungju Noh , Yi Chen , Fabio Donati , Andreas J. Heinrich , Christoph Wolf , Yujeong Bae

The spintronic properties of magnetic molecules have attracted significant scientific attention. Special emphasis has been placed on the qubit for quantum information processing. The single molecule magnet, bis(phthalocyaninato (Pc))…

By comparing the signals of electron spin resonance (ESR) from two crystals of a diamond (spin-labels) the demagnetizing field of the Co, Fe, and Ni samples in the shape of strongly elongated ellipsoids of revolution (disks) has been…

Materials Science · Physics 2010-06-30 N. A. Poklonski , T. M. Lapchuk , N. I. Gorbachuk

We propose a general scheme for inducing resonant exchange between spins or pseudo-spins of unmatched levels via periodic driving. The basic idea is illustrated for a system of two heteronuclear atoms, for which analytical results are…

Quantum Gases · Physics 2018-08-08 Jun-Jie Chen , Zhi-Fang Xu , Li You

The sub-nanometer distance between tip and sample in a scanning tunneling microscope (STM) enables the application of very large electric fields with a strength as high as ~ 1 GV/m. This has allowed for efficient electrical driving of Rabi…

Mesoscale and Nanoscale Physics · Physics 2024-01-30 Hong T. Bui , Christoph Wolf , Yu Wang , Masahiro Haze , Arzhang Ardavan , Andreas J. Heinrich , Soo-hyon Phark

We consider an electronic spin, such as a nitrogen-vacancy (NV) center in diamond, weakly coupled to a large number (bath) of nuclear spins, and subjected to the Rabi driving with a periodically alternating phase (multiple rotary echo). We…

Mesoscale and Nanoscale Physics · Physics 2015-03-25 V. V. Mkhitaryan , F. Jelezko , V. V. Dobrovitski