Related papers: Quantum tunneling of magnetization in molecular sp…
We explore dissipative quantum tunnelling, a phenomenon central to various physical and chemical processes, using a double-well potential model. This paper aims to bridge gaps in understanding the crossover from thermal activation to…
This chapter takes a microscopic view of quantum tunneling of magnetization (QTM) in single-molecule magnets (SMMs), focusing on the interplay between exchange and anisotropy. Careful consideration is given to the relationship between…
We demonstrate that transport spectroscopy of single molecular magnets shows signatures of quantum tunneling at low temperatures. We find current and noise oscillations as function of bias voltage due to a weak violation of spin selection…
An effective Hamiltonian, describing quantum tunneling in ferrimagnetic nanoparticles which includes interactions between the electronic spins of nanoparticle and microscopic environmental spins (like nuclear spins or paramagnetic…
We study the magnetic relaxation of a system of localized spins interacting through weak dipole interactions, at a temperature large with respect to the ordering temperature but low with respect to the crystal field level splitting. The…
We give a further step in the quantum mechanical description of engineered atomic spin structures by deriving a master equation of the Redfield type that governs the dynamics of the atomic spin density matrix. By generalizing this approach…
It is shown that a single molecular magnet placed in a rapidly oscillating magnetic field displays the phenomenon of quenching of tunneling processes. The results open a way to manipulate the quantum states of molecular magnets by means of…
Quantum mechanical objects or nanoobjects have been proposed as bits for information storage. While time-averaged properties of magnetic, quantum-mechanical particles have been extensively studied experimentally and theoretically,…
The spin relaxation in the molecular magnet \Mn12 is investigated by a novel type of high-frequency magnetic spectroscopy. By reversing the external magnetic field the intensities of the $|\pm 10>\to |\pm 9>$ transitions within the ground…
We consider transport through a single-molecule magnet strongly coupled to metallic electrodes. We demonstrate that for half-integer spin of the molecule electron- and spin-tunneling \emph{cooperate} to produce both quantum tunneling of the…
The first measurements of magnetization hysteresis loops on diluted single crystal of [(Pc)2Ho]-TBA+ (Pc: phthalocyaninato, TBA: tetrabutylammonium) in the subkelvin temperature range are reported. Characteristic staircase-like structure…
The description of the tunneling of a macroscopic variable in the presence of a bath of localized spins is a subject of great fundamental and practical interest, and is relevant for many solid-state qubit designs. Instead of focusing on the…
The quantum tunneling of the magnetization vector are studied theoretically in single-domain ferromagnetic nanoparticles placed in an external magnetic field at an arbitrarily directed angle in the $ZX$ plane. We consider the…
This article takes a broad view of the understanding of magnetic bistability and magnetic quantum tunneling in single-molecule magnets (SMMs), focusing on three families of relatively simple, low-nuclearity transition metal clusters: spin S…
The spin-reversal in dilute Li$_2$(Li$_{1-x}$Fe$_{x}$)N with $x < 1$ % is dominated by resonant quantum tunneling of spatially well-separated states. We report on the effect of finite couplings between those states that give rise to…
The crossover between thermally assisted and pure quantum tunneling has been studied in single crystals of high spin (S=10) uniaxial molecular magnet Mn12 using micro-Hall-effect magnetometry. Magnetic hysteresis and relaxation experiments…
We study entanglement between quantum states of multi level spin system of a single particle considering a nucleus with spin 3/2 in both the internal electric field gradient and the external magnetic field. It was shown that entanglement is…
Quantum tunneling of domain walls out of an impurity potential in a mesoscopic ferromagnetic sample is investigated. Using improved expressions for the domain wall mass and for the pinning potential, we find that the cross-over temperature…
We investigate quantum entanglement in two-spin-1/2 NMR systems at thermal equilibrium under external magnetic fields. We derive closed-form analytical expressions for the entanglement of the system and show how the entanglement depends on…
Quantum tunneling was observed in the decay of metastable spin domains in gaseous Bose-Einstein condensates. A mean-field description of the tunneling was developed and compared with measurement. The tunneling rates are a sensitive probe of…