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Related papers: Rapid Scan White Light Pump-Probe Spectroscopy wit…

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We demonstrate an approach to two-dimensional electronic spectroscopy (2DES) that combines the benefits of shot-to-shot detection at high-repetition rates with the simplicity of a broadband white light continuum input and conventional…

Optics · Physics 2023-10-03 Asha S. Thomas , Vivek N. Bhat , Vivek Tiwari

We demonstrate femtosecond pump-probe transient absorption spectroscopy using a programmable dispersive filter as an ultra-fast delay line. Combined with fast synchronous detection this delay line allows for recording of 6 ps decay traces…

Optics · Physics 2018-06-22 Xavier Audier , Naveen Balla , Herve Rigneault

We report here an experimental setup to perform three-pulse pump-probe measurements over a wide wavelength and temperature range. By combining two pump pulses in the visible (650-900 nm) and mid-IR (5-20 $\mu$m) range, with a broadband…

A major limitation of transient optical spectroscopy is that relatively high laser fluences are required to enable broadband, multichannel detection with acceptable signal-to-noise levels. Under typical experimental conditions, many…

Optics · Physics 2023-05-03 Siedah J. Hall , Peter J. Budden , Anne Zats , Matthew Y. Sfeir

Standard optical pump-probe methods analyze a system's temporal response to a laser pulse within sub-femtoseconds to several nanoseconds, constrained by the optical delay line's length. While resistance is a sensitive detector in various…

Instrumentation and Detectors · Physics 2024-04-26 M. I. Blumenau , A. Yu. Kuntsevich

Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction,…

We have developed a single-shot imaging technique that can capture ultrafast events occurring on femtosecond to picosecond time scales. The technique is based on an optical pump-probe method, in which multiple time-delayed femtosecond…

Instrumentation and Detectors · Physics 2018-11-14 Sarang Yeola , Donghoon Kuk , Ki-Yong Kim

We describe an ultrafast time resolved pump-probe spectroscopy setup aimed at studying the switching of nanophotonic structures. Both fs pump and probe pulses can be independently tuned over broad frequency range between 3850 and 21050…

Optics · Physics 2010-11-02 Tijmen G. Euser , Philip J. Harding , Willem L. Vos

Femtosecond optical pump-probe technique is used to study charge carrier dynamics in few-layer MoS2 samples fabricated by mechanical exfoliation. An ultrafast pump pulse excites carriers and differential reflection of a probe pulse tuned to…

Mesoscale and Nanoscale Physics · Physics 2011-11-01 Rui Wang , Brian A. Ruzicka , Nardeep Kumar , Matthew Z. Bellus , Hsin-Ying Chiu , Hui Zhao

The paper describes a new concept of visible pump/X-ray probe/slow detector experiments that could be performed at third-generation synchrotron light sources. We propose a technique that would allow time resolution up to femtosecond…

Instrumentation and Detectors · Physics 2009-11-07 E. L. Saldin , E. A. Schneidmiller , M. V. Yurkov

An experimental continuous-wave (cw) pump-probe scheme is demonstrated by investigating the population and photoionization dynamics of an atomic system. Specifically, $^6$Li atoms are initially prepared in optically pumped $2^{2}S_{1/2}$…

We propose and demonstrate pump-probe spectroscopy of rubidium absorption which reveals the sub-Doppler hyperfine structure of the $^{5}$S$_{1/2} \leftrightarrow$ $^{5}$P$_{3/2}$ (D2) transitions. The counter propagating pump and probe…

Femtosecond spectroscopy is an important tool for tracking rapid photoinduced processes in a variety of materials. To spatially map the processes in a sample would substantially expand the capabilities of the method. This is, however,…

Optics · Physics 2019-05-01 Ondřej Denk , Kaibo Zheng , Donatas Zigmantas , Karel Žídek

Combined microwave-optical pump-probe methods are emerging to study the quantum state of spin qubit centers and the charge dynamics in semiconductors. A major hindrance is the limited bandwidth of microwave irradiation/detection circuitry…

Applied Physics · Physics 2020-10-27 S. Kollarics , A. Bojtor , K. Koltai , B. G. Márkus , K. Holczer , J. Volk , G. Klujber , M. Szieberth , F. Simon

Background-free fluorescence detection in multidimensional electronic spectroscopy promises high sensitivity compared to conventional approaches. Here we explore the sensitivity limits of multidimensional electronic spectroscopy. We present…

Chemical Physics · Physics 2022-10-18 Amitav Sahu , Vivek N. Bhat , Sanjoy Patra , Vivek Tiwari

Optical pump-probe spectroscopy is a powerful tool to directly probe the carrier dynamics in materials down to sub-femtosecond resolution. To perform such measurement, while keeping the pump induced perturbation to the sample as small as…

Recording of transient absorption microscopy images requires fast detection of minute optical density changes, which is typically achieved with high-repetition-rate laser sources and lock-in detection. Here, we present a highly flexible and…

Light scattering detection in the near field, a rapidly expanding family of scattering techniques, has recently proved to be an appropriate procedure for performing dynamic measurements. Here we report an innovative algorithm, based on the…

We present a simple method and its experimental implementation to completely determine the characteristics of the pump-and-probe pulse and the Stokes pulse in a coherent anti-Stokes Raman scattering microscope at sample level without…

We demonstrate a pump-probe strobe light spectroscopy for sensitive detection of magneto-optical dynamics in the context of hybrid magnonics. The technique uses a combinatorial microwave-optical pump-probe scheme, leveraging both the…

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