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Quantum control techniques play an important role in manipulating and harnessing the properties of different quantum systems, including isolated atoms. Here, we propose to achieve quantum control over a single on-surface atomic spin using…

Performing nanoscale scanning electron paramagnetic resonance (EPR) requires three essential ingredients. First, a static magnetic field together to field gradients to Zeeman split the electronic energy levels with spatial resolution.…

Mesoscale and Nanoscale Physics · Physics 2024-01-16 Carlos A. González-Gutiérrez , David García-Pons , David Zueco , María José Martínez-Pérez

We propose a method based on optically detected magnetic resonance (ODMR) to measure the decoherence time $T_{2}$ of a single electron spin in a semiconductor quantum dot. The electron spin resonance (ESR) of a single excess electron on a…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Oliver Gywat , Hans-Andreas Engel , Daniel Loss , R. J. Epstein , F. M. Mendoza , D. D. Awschalom

Shrinking spintronic devices to the nanoscale ultimately requires localized control of individual atomic magnetic moments. At these length scales, the exchange interaction plays important roles, such as in the stabilization of…

Nuclear electric resonance (NER) spectroscopy is currently experiencing a revival as a tool for nuclear spin-based quantum computing. Compared to magnetic or electric fields, local electron density fluctuations caused by changes in the…

Quantum Physics · Physics 2025-01-30 Johannes K. Krondorfer , Andreas W. Hauser

Recent advances in increasing the spectroscopic energy resolution in scanning tunneling microscopy (STM) have been achieved by integrating electron spin resonance (ESR) with STM. Here, we demonstrate the design and performance of a…

Quantum dot arrays provide a promising platform for quantum information processing. For universal quantum simulation and computation, one central issue is to demonstrate the exhaustive controllability of quantum states. Here, we report the…

The rapidly rising fields of spintronics and quantum information science have led to a strong interest in developing the ability to coherently manipulate electron spins. Electron spin resonance (ESR) is a powerful technique to manipulate…

Materials Science · Physics 2009-11-13 M. Pioro-Ladriere , T. Obata , Y. Tokura , Y. -S. Shin , T. Kubo , K. Yoshida , T. Taniyama , S. Tarucha

The ability to manipulate coherently individual quantum objects organized in arrays is a prerequisite to any scalable quantum information platform. For electron spin qubits, it requires the fine tuning of large arrays of tunnel-coupled…

Molecular systems can exhibit a complex, chemically tailorable inner structure which allows for targeting of specific mechanical, electronic and optical properties. At the single-molecule level, two major complementary ways to explore these…

Mesoscale and Nanoscale Physics · Physics 2017-04-05 Rocco Gaudenzi , Maciej Misiorny , Enrique Burzurí , Maarten R. Wegewijs , Herre S. J. van der Zant

Controlling the motion of macroscopic oscillators in the quantum regime has been the subject of intense research in recent decades. In this direction, opto-mechanical systems, where the motion of micro-objects is strongly coupled with laser…

Quantum Physics · Physics 2021-06-03 Maxime Perdriat , Clément Pellet-Mary , Paul Huillery , Loïc Rondin , Gabriel Hétet

Electrons in atoms and molecules move on attosecond time scales. Deciphering their quantum dynamics in space and time calls for high-resolution microscopy at this speed. While scanning tunnelling microscopy (STM) driven with terahertz…

Optically addressed atomic defects in the solid-state are widely used as single-photon sources and memories for quantum network applications. The solid-state environment allows for a high density of electron and nuclear spins with the…

Spin squeezing has been explored in atomic systems as a tool for quantum sensing, improving experimental sensitivity beyond the spin standard quantum limit for certain measurements. To optimize absolute metrological sensitivity, it is…

High Energy Physics - Phenomenology · Physics 2025-02-21 Eric Boyers , Garry Goldstein , Alexander O. Sushkov

The ability to coherently control and read out qubits with long coherence times in a scalable system is a crucial requirement for any quantum processor. Nuclear spins in the solid state have shown great promise as long-lived qubits. Control…

The ability to determine precisely the separation of two frequencies is fundamental to spectroscopy, yet the resolution limit poses a critical challenge: distinguishing two incoherent signals becomes impossible when their frequencies are…

Quantum Physics · Physics 2025-12-29 Qingyun Cao , Genko T. Genov , Yaoming Chu , Jianming Cai , Yu Liu , Alex Retzker , Fedor Jelezko

Quantum metrology experiments in atomic physics and quantum optics have demonstrated measurement accuracy beyond the shot-noise limit via multi-particle entanglement. At the same time, electron microscopy, an essential tool for…

A single atom is the prototypical quantum system, and a natural candidate for a quantum bit - the elementary unit of a quantum computer. Atoms have been successfully used to store and process quantum information in electromagnetic traps, as…

Mesoscale and Nanoscale Physics · Physics 2013-05-21 Jarryd J. Pla , Kuan Y. Tan , Juan P. Dehollain , Wee H. Lim , John J. L. Morton , David N. Jamieson , Andrew S. Dzurak , Andrea Morello

We review the problem of spin decoherence of magnetic atoms deposited on a surface. Recent breakthroughs in scanning tunnelling microscopy (STM) make it possible to probe the spin dynamics of individual atoms, either isolated or integrated…

Mesoscale and Nanoscale Physics · Physics 2017-02-14 F. Delgado , J. Fernández-Rossier

The recent development of all-electrical electron spin resonance (ESR) in a scanning tunneling microscope (STM) setup has opened the door to vast applications. Despite the fast growing number of experimental works on STM-ESR, the…

Mesoscale and Nanoscale Physics · Physics 2019-07-17 J. Reina Gálvez , C. Wolf , F. Delgado , N. Lorente