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Using temperature dependent Raman spectroscopy we address the question of how the transition from bulk to few atomic layers affects the charge density wave (CDW) phases in 1T-TaS2. We find that for crystals with thickness larger than approx…

Mesoscale and Nanoscale Physics · Physics 2019-10-30 Adina Luican-Mayer , Jeffrey R. Guest , Saw-Wai Hla

We employ low-frequency Raman spectroscopy to study the nearly commensurate (NC) to commensurate (C) charge density wave (CDW) transition in 1T-TaS2 ultrathin flakes protected from oxidation. We identify new modes originating from C phase…

We use scanning tunneling microscopy to study the domain structure of the nearly-commensurate charge density wave (NC-CDW) state of 1T-TaS$_2$. In our sub-angstrom characterization of the state, we find a continual evolution of the CDW…

Strongly Correlated Electrons · Physics 2022-08-31 Manoj Singh , Boning Yu , James Huber , Bishnu Sharma , Ghilles Ainouche , Ling Fu , Jasper van Wezel , Michael C. Boyer

Recent experiments have shown that the high temperature incommensurate (I) charge density wave (CDW) phase of 1T-TaS2 can be photoinduced from the lower temperature, nearly commensurate (NC) CDW state. Here we report a time-resolved x-ray…

Strongly Correlated Electrons · Physics 2017-12-13 G. Lantz , C. Laulhé , S. Ravy , M. Kubli , M. Savoini , K. Tasca , E. Abreu , V. Esposito , M. Porer , A. Ciavardini , L. Cario , J. Rittmann , P. Beaud , S. L. Johnson

The capability to isolate one to few unit-cell thin layers from the bulk matrix of layered compounds opens fascinating prospects to engineer novel electronic phases. However, a comprehensive study of the thickness dependence and of…

Strongly Correlated Electrons · Physics 2017-09-06 Árpád Pásztor , Alessandro Scarfato , Céline Barreteau , Enrico Giannini , Christoph Renner

We use scanning tunneling microscopy to study the temperature evolution of the atomic-scale properties of the nearly-commensurate charge density wave (NC-CDW) state of the low-dimensional material, 1T-TaS$_2$. Our measurements at 203 K, 300…

Strongly Correlated Electrons · Physics 2023-04-28 Boning Yu , Ghilles Ainouche , Manoj Singh , Bishnu Sharma , James Huber , Michael C. Boyer

Transport studies of atomically thin 1T-TaS2 have demonstrated the presence of intermediate resistance states across the nearly commensurate (NC) to commensurate (C) charge density wave (CDW) transition, which can be further switched…

Materials Science · Physics 2020-09-29 Tarun Patel , Junichi Okamoto , Tina Dekker , Bowen Yang , Jingjing Gao , Xuan Luo , Wenjian Lu , Yuping Sun , Adam W. Tsen

Lower thermal stability due to thinning often leads to unprecedented hidden phases in low-dimensional materials. Such hidden phases can coexist or compete with preexisting electronic phases. We investigate hidden phases observed in…

Materials Science · Physics 2023-02-09 Wooin Yang , Dowook Kim , Hyoung Kug Kim , Tae-Hwan Kim

Ultra-thin 2D materials have shown complete paradigm shift of understanding of physical and electronic properties because of confinement effects, symmetry breaking and novel phenomena at nanoscale. Bulk 2H-TaS2 undergoes an incommensurate…

Mesoscale and Nanoscale Physics · Physics 2023-07-18 Divya Rawat , Aksa Thomas , Ajay Soni

Due to their anisotropy, layered materials are excellent candidates for studying the interplay between the in-plane and out-of-plane entanglement in strongly correlated systems. A relevant example is provided by 1T-TaS2, which exhibits a…

The commensurate charge density wave (CDW) in the layered compound $1T$-TaS$_2$ has hitherto mostly been treated as a quasi two-dimensional phenomenon. Recent band structure calculations have, however, predicted that the CDW coexists with a…

The transition metal dichalcogenide 1T-TaS$_2$ is well known to harbor a rich variety of charge density wave (CDW) distortions which are correlated with underlying lattice atom modulations. The long range CDW phases extend throughout the…

Materials Science · Physics 2017-05-24 Xiaochen Zhu , Ang J. Li , G. R. Stewart , Arthur F. Hebard

The impact of variable Ti self-doping on the 1T-TiSe2 charge density wave (CDW) is studied by scanning tunneling microscopy. Supported by density functional theory we show that agglomeration of intercalated-Ti atoms acts as preferential…

We report measurements of anisotropic triple-$q$ charge density wave (CDW) fluctuations in the transition metal dichalcogenide 1$T$-TiSe$_2$ over a large volume of reciprocal space with X-ray diffuse scattering. Above the transition…

We report on depinning of nearly-commensurate charge-density waves in 1T-TaS2 thin-films at room temperature. A combination of the differential current-voltage measurements with the low-frequency noise spectroscopy provide unambiguous means…

Mesoscale and Nanoscale Physics · Physics 2024-06-19 A. Mohammadzadeh , A. Rehman , F. Kargar , S. Rumyantsev , J. M. Smulko , W. Knap , R. K. Lake , A. A. Balandin

The charge density wave (CDW) state in van der Waals systems shows interesting scaling phenomena as the number of layers can significantly affect the CDW transition temperature, $T_{CDW}$. However, it is often difficult to use conventional…

Charge density wave (CDW) phases are symmetry-reduced states of matter in which a periodic modulation of the electronic charge frequently leads to drastic changes of the electronic spectrum, including the emergence of energy gaps. We…

Mesoscale and Nanoscale Physics · Physics 2017-06-30 Bahadur Singh , Chuang-Han Hsu , Wei-Feng Tsai , Vitor M. Pereira , Hsin Lin

CuTe is a two-dimensional (2D) layered material, yet forming a quasi-one-dimensional (quasi-1D) charge-density-wave (CDW) along the a-axis in the ab-plane at high transition temperature $T_{CDW}=335$ K. However, the anisotropic properties…

Strongly Correlated Electrons · Physics 2022-03-03 R. S. Li , L. Yue , Q. Wu , S. X. Xu , Q. M. Liu , Z. X. Wang , T. C. Hu , X. Y. Zhuo , L. Y. Shi , S. J. Zhang , D. Wu , T. Dong , N. L. Wang

We report experimental evidence of charge density wave (CDW) transition in monolayer 1T-VTe$_2$ film. 4$\times$4 reconstruction peaks are observed by low energy electron diffraction below the transition temperature $T_{CDW}$ = 186 K.…

Materials Science · Physics 2019-12-18 Yuan Wang , Junhai Ren , Jiaheng Li , Yujia Wang , Huining Peng , Pu Yu , Wenhui Duan , Shuyun Zhou

Most metallic transition metal dichalcogenides undergo charge density wave (CDW) instabilities with similar or identical ordering vectors in bulk and in single layer, albeit with different critical temperatures. Metallic 1T-TiTe$_2$ is a…

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