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In all theoretical treatments of electron transport through single molecules between two metal electrodes, a clear distinction has to be made between a coherent transport regime with a strong coupling throughout the junction and a Coulomb…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Robert Stadler , Jerome Cornil , Victor Geskin

The Hartree-Fock based diagonalization is a computational method for the investigation of the low-energy properties of correlated electrons in disordered solids. The method is related to the quantum-chemical configuration interaction…

Disordered Systems and Neural Networks · Physics 2007-05-23 Michael Schreiber , Thomas Vojta

This is a follow-up of our recently proposed work on pseudopotential calculation (Ref. [21]) of atoms and molecules within DFT framework, using cartesian coordinate grid. Detailed results are presented to demonstrate the usefulness,…

Chemical Physics · Physics 2015-05-18 Amlan K. Roy

The single-particle spectral properties near the Mott transition in the two-dimensional Hubbard model with next-nearest-neighbor hopping are investigated by using cluster perturbation theory. Complicated spectral features of this model are…

Strongly Correlated Electrons · Physics 2014-07-14 Masanori Kohno

The design of better exchange-correlation functionals for Density Functional Theory (DFT) is a central challenge of modern electronic structure theory. However, current developments are limited by the mathematical form of the functional,…

Chemical Physics · Physics 2024-08-19 Kyle Bystrom , Boris Kozinsky

The dynamical density-matrix renormalization group technique is used to calculate spin and charge excitation spectra in the one-dimensional (1D) Hubbard model at quarter filling with nearest-neighbor $t$ and next-nearest-neighbor $t'$…

Strongly Correlated Electrons · Physics 2009-11-13 S. Nishimoto , T. Shirakawa , Y. Ohta

We present a formulation and implementation of the DFT+\textit{U} method within the framework of linear combination of numerical atomic orbitals (NAO). Our implementation not only enables single-point total energy and electronic-structure…

Materials Science · Physics 2022-06-29 Xin Qu , Peng Xu , Hong Jiang , Lixin He , Xinguo Ren

We suggest measuring one-particle density matrix of a trapped ultracold atomic cloud by scattering fast atoms in a pure momentum state off the cloud. The lowest-order probability of the inelastic process, resulting in a pair of outcoming…

Soft Condensed Matter · Physics 2009-10-31 A. B. Kuklov , B. V. Svistunov

Interferences in multi-path systems for single and multiple particles are theoretically analyzed. A holistic method is presented, which allows to construct the unitary transition matrix describing interferometers for any port number d and…

Quantum Physics · Physics 2019-12-10 Bülent Demirel

We analyze the low-energy spectrum of a two-electron double quantum dot under a potential bias in the presence of an external magnetic field. We focus on the regime of spin blockade, taking into account the spin orbit interaction and…

Mesoscale and Nanoscale Physics · Physics 2013-05-30 Dimitrije Stepanenko , Mark Rudner , Bertrand I. Halperin , Daniel Loss

We show that an array of polar molecules interacting with Rydberg atoms is a promising hybrid system for scalable quantum computation. Quantum information is stored in long-lived hyperfine or rotational states of molecules which interact…

Quantum Physics · Physics 2022-06-07 Chi Zhang , M. R. Tarbutt

We present a non-perturbative expression for the scattering matrix of $N$ particles interacting inside a quantum dot. Characterizing the dot by its resonances, we find a compact form for the scattering matrix in a real-time representation.…

Mesoscale and Nanoscale Physics · Physics 2008-06-10 A. V. Lebedev , G. B. Lesovik , G. Blatter

We present a variational solution of the T-matrix integral equation within a local approximation. This solution provides a simple form for the T matrix similar to Hubbard models but with the local interaction depending on momentum and…

Other Condensed Matter · Physics 2007-05-23 I. A. Nechaev , E. V. Chulkov

The Hamaker constants, which are coefficients providing quantitative information on intermolecular forces, were calculated for a number of different materials according to the Lifshitz theory via simple DFT calculations without any…

Computational Physics · Physics 2020-08-20 Hideyuki Takagishi , Takashi Masuda , Tatsuya Shimoda , Ryo Maezono , Kenta Hongo

Hydrodynamic interactions in a suspension of spherical particles confined between two parallel planar walls are studied under creeping-flow conditions. The many-particle friction matrix in this system is evaluated using our novel numerical…

Fluid Dynamics · Physics 2009-11-11 S. Bhattacharya , J. Blawzdziewicz , E. Wajnryb

We establish a link between quantum mechanical molecular simulations and the transfer matrix of a molecule. The transfer matrix (T-matrix) of an object provides a complete description of its electromagnetic response. Once the T-matrices of…

Chemical Physics · Physics 2020-04-21 Ivan Fernandez-Corbaton , Carsten Rockstuhl , Wim Klopper

A program to calculate the three-particle hyperspherical brackets is presented. Test results are listed and it is seen that the program is well applicable up to very high values of the hypermomentum and orbital momenta. The listed runs show…

Computational Physics · Physics 2020-06-16 Victor D. Efros

The interaction within a hybrid system consisting of a spherical metal nanoparticle and a nearby organic dye molecule is formulated in a combined quantum-classical approach. Whereas the nanoparticle's polarization field is treated in…

Chemical Physics · Physics 2019-09-04 Xiaomeng Liu , Lennart Seiffert , Thomas Fennel , Oliver Kühn

Quantum--Mechanical methods that are both computationally fast and accurate are not yet available for electronic excitations having charge transfer character. In this work, we present a significant step forward towards this goal for those…

Chemical Physics · Physics 2015-06-12 Michele Pavanello , Troy Van Voorhis , Lucas Visscher , Johannes Neugebauer

We investigate the Mott transitions in the two-orbital Hubbard model with different bandwidths. By combining dynamical mean field theory with the exact diagonalization, we discuss the stability of itinerant quasi-particle states in each…

Strongly Correlated Electrons · Physics 2009-11-10 Akihisa Koga , Norio Kawakami , T. M. Rice , Manfred Sigrist