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Based on the Elastically Collective Nonlinear Langevin Equation theory of bulk relaxation in glass-forming liquids, and our recent ideas of how interface-nucleated modification of caging constraints are spatially transferred into the…

Soft Condensed Matter · Physics 2020-07-01 Anh D. Phan , Kenneth S. Schweizer

We develop the Elastically Collective Nonlinear Langevin Equation theory to investigate, for the first time, glassy dynamics in capped metallic glass thin films. Finite-size effects on the spatial gradient of structural relaxation time and…

Soft Condensed Matter · Physics 2022-02-02 Anh D. Phan

We report on the first micro-scale observation of the velocity field imposed by a non-uniform heat content along the solid/liquid boundary. We determine both radial and vertical velocity components of this thermo-osmotic flow field by…

Fluid Dynamics · Physics 2016-05-11 Andreas Bregulla , Alois Würger , Katrin Günther , Michael Mertig , Frank Cichos

Shearing transitions of multi-layer molecularly thin-film lubrication systems in variations of the film-substrate coupling strength and the load are studied by using a multiscale method. Three kinds of the interlayer slips found in…

Chemical Physics · Physics 2017-06-07 Zuo-Bing Wu , X. C. Zeng

We analyze the displacements of the particles of a glass-forming molecular liquid perpendicular to a confining solid surface, using extensive molecular dynamics simulations with atomistic models. In the vicinity of an attractive surface,…

Soft Condensed Matter · Physics 2024-10-15 Alireza F. Behbahani , Vagelis Harmandaris

Free interfaces of liquid crystals tend to minimise both capillarity and anchoring forces. Here we study nematic films in planar and radial geometries with antagonistic anchoring boundary conditions and one deformable interface. Assuming a…

Soft Condensed Matter · Physics 2014-06-17 O V Manyuhina

A droplet of a classical liquid surrounded by a cold gas placed on a hot substrate is accompanied by unremitting internal circulations, while the droplet remains immobile. Two identical cells with opposite sense of circulation form in the…

Fluid Dynamics · Physics 2023-12-12 Aaveg Aggarwal , Eleftherios Kirkinis , Monica Olvera de la Cruz

This work reports a systematic study of the evolution of charge transport mechanism in granular ultra-thin films of palladium of thickness varying between 6nm and 2nm. While the films with thickness > 4nm exhibit metallic behaviour, that at…

Entropy stabilization has garnered significant attention as a new approach to designing novel materials. Much of the work in this area has focused on bulk ceramic processing, leaving entropy-stabilized thin films relatively underexplored.…

Materials Science · Physics 2020-06-29 Valerie Jacobson , Dave Diercks , Bobby To , Andriy Zakutayev , Geoff Brennecka

Many physical systems give rise to dynamical behavior leading to cuspidal shapes which represent a singularity of the governing equation. The cusp tip often exhibits self-similarity as well, indicative of scaling symmetry invariant in time…

Fluid Dynamics · Physics 2019-03-22 Chengzhe Zhou , Sandra M. Troian

In this work, we study the deformation behavior of thin films of various soft glassy materials that are simultaneously subjected to two creep flow fields, rotational shear flow by applying torque and elongational flow by applying normal…

Soft Condensed Matter · Physics 2012-09-21 Asima Shaukat , Manish Kaushal , Ashutosh Sharma , Yogesh M. Joshi

We extend the force-level ECNLE theory to treat the spatial gradients of the alpha relaxation time and glass transition temperature, and the corresponding film-averaged quantities, to the geometrically asymmetric case of finite thickness…

Soft Condensed Matter · Physics 2024-01-15 Anh D. Phan , Kenneth S. Schweizer

Plants and insects use slender conical structures to transport and collect small droplets, which are propelled along the conical structures due to capillary action. These droplets can deposit a fluid film during their motion, but despite…

The use of ultra-thin, i.e., monolayer films plays an important role for the emerging field of nano-fluidics. Since the dynamics of such films is governed by the interplay between substrate-fluid and fluid-fluid interactions, the transport…

Other Condensed Matter · Physics 2009-11-11 M. N. Popescu , S. Dietrich , G. Oshanin

We examine the structural and dynamic properties of confined binary hard-sphere mixtures designed to mimic realizable colloidal thin films. Using computer simulations, governed by either Newtonian or overdamped Langevin dynamics, together…

Soft Condensed Matter · Physics 2015-05-01 Jonathan A. Bollinger , Avni Jain , James Carmer , Thomas M. Truskett

The $\alpha$-process (segmental motion) of thin polystyrene films supported on glass substrate has been investigated in a wider frequency range from 10$^{-3}$ Hz to 10$^4$ Hz using dielectric relaxation spectroscopy and thermal expansion…

Soft Condensed Matter · Physics 2009-10-31 Koji Fukao , Yoshihisa Miyamoto

Superspreading wetting is traditionally attributed to surfactant-driven mechanisms. However, recent observations of superspreading in surfactant-free nanofluids defy standard theoretical explanations. This study considers a data-driven…

Fluid Dynamics · Physics 2026-01-06 Kai Fukami , Eita Shoji

We present an analysis of heterogeneous dynamics in molecular dynamics simulations of a thin polymeric film, supported by an absorbing structured surface. Near the glass transition "immobile" domains occur throughout the film, yet the…

Soft Condensed Matter · Physics 2009-11-10 Arlette R. C. Baljon , Joris Billen , Rajesh Khare

The displacement of a more viscous fluid by a less viscous immiscible fluid in confined geometries is a fundamental problem in multiphase flows. Recent experiments have shown that such fluid-fluid displacement in micro-capillary tubes can…

Fluid Dynamics · Physics 2025-12-01 Sthavishtha R. Bhopalam , Ruben Juanes , Hector Gomez

The glass transition temperature and its connection to statistical properties of confined and free-standing polymer films of varying thickness containing unentangled to highly entangled bead-spring chains are studied by molecular dynamics…

Soft Condensed Matter · Physics 2023-09-21 Hsiao-Ping Hsu , Kurt Kremer