Related papers: Time-resolved THz Stark spectroscopy
Nonlinear terahertz (THz) spectroscopy relies on the interaction of matter with few-cycle THz pulses of electric field amplitudes up to megavolts/centimeter (MV/cm). In condensed-phase molecular systems, both resonant interactions with…
We bring together the advantages of terahertz (THz) and optical spectroscopies to introduce TACOS (Terahertz-Assisted Chiro-Optical Spectroscopy), a novel approach for ultrafast and highly efficient imaging of molecular chirality and…
We report a comprehensive theoretical analysis of the instability achievable by using phase modulation spectroscopy to lock a terahertz local oscillator to an absorptive reference consisting of the rotational transition of molecules at room…
Slow motion movies are not only fascinating to watch, they also allow us to see intricate details of the mechanical dynamics of complex phenomena. If the images in each frame are replaced by terahertz (THz) waves, such movies can monitor…
We report on the measurement of terahertz electric-field vector waveforms by using a system that contains no mechanical moving parts. It is known that two phase-locked femtosecond lasers with different repetition rates can be used to…
Speckle patterns observed in coherent optical imaging reflect important characteristic information of the scattering object. To capture speckle patterns, angular resolved or oblique illumination geometries are usually employed in…
Lightwave-driven terahertz scanning tunnelling microscopy (THz-STM) is capable of exploring ultrafast dynamics across a wide range of materials with angstrom resolution. In contrast to scanning near-field optical microscopy, where photons…
In conventional optical Stark-shift spectroscopy, molecules are exposed to spatially homogeneous static electric fields that shift the energies of their spectral lines. These shifts are attributed to the molecular electronic properties,…
In this work, the detection of terahertz (THz) pulse via different schemes of THz time-domain spectroscopy (THz-TDS), including electro-optic sampling (EOS) and photoconductive sampling (PCS), has been reviewed by insisting on its…
Coupling phase-stable single-cycle terahertz (THz) pulses to scanning tunneling microscope (STM) junctions enables spatio-temporal imaging with femtosecond temporal and \r{A}ngstrom spatial resolution. The time resolution achieved in such…
Electro-optic sampling allows the electric field of THz, mid-infrared and visible light pulses to be measured directly as a function of time, with data analysis often performed in the frequency domain after fast Fourier transform. Here we…
The Terahertz frequency range bears intriguing opportunities, beyond very advanced applications in spectroscopy and matter control. Peculiar quantum phenomena are predicted to lead to light emission by non-trivial mechanisms. Typically,…
We propose and demonstrate a Terahertz (THz) oscilloscope for recording time information of an ultrashort electron beam. By injecting a laser-driven THz pulse with circular polarization into a dielectric tube, the electron beam is swept…
We demonstrate how dynamic Stark control (DSC) can be achieved on molecular photodissociation in the dipole limit, using single-cycle (FWHM) laser pulses in the terahertz (THz) regime. As the laser-molecule interaction follows the…
Single molecule spectroscopy aims at unveiling often hidden but potentially very important contributions of single entities to a system's ensemble response. Albeit contributing tremendously to our ever growing understanding of molecular…
THz spectroscopy is an emerging tool for detection of microorganisms and harmful compounds in the food industry, the study of proteins in biomedicine and the development of electron-beam X-ray sources for molecular imaging and lithography.…
Terahertz (THz) waves have been significantly developed in the last fifteen years because of their great potential for applications in industrial and scientific communities1,2. The unique properties of THz waves as transparency for numerous…
In Terahertz (THz) technology, one of the long-standing challenges has been the formation of intense pulses covering the hard-to-access frequency range of 1-15 THz (so-called THz gap). This frequency band, lying between the electronically…
The time-resolved detection of ultrashort pulsed THz-band electric field temporal profiles without an ultrashort laser probe is demonstrated. A non-linear interaction between a narrow-bandwidth optical probe and the THz pulse transposes the…
Transmission through photoexcited semiconductors is used to temporally and spectrally shape a Terahertz pulse. By adjusting the optical pump-THz probe delay, we experimentally introduce a polar asymmetry in the pulse profile as high as 92%.…