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Two-dimensional (2D) materials are categorized into van der Waals (vdW) and non-vdW types. However, no relevant descriptors have been proposed for identifying the latter. Here, we identify the non-vdW 2D materials by calculating the…

Materials Science · Physics 2025-08-05 Shota Ono

Control over the optical properties of atomically thin two-dimensional (2D) layers, including those of transition metal dichalcogenides (TMDs), is needed for future optoelectronic applications. Remarkable advances have been achieved through…

The nanoscale periodic potentials introduced by moir\'{e} patterns in semiconducting van der Waals (vdW) heterostructures provide a new platform for designing exciton superlattices. To realize these applications, a thorough understanding of…

Van der Waals heterostructures (vdWHs) allow the assembly of high-crystalline two-dimensional (2D) materials in order to explore dimensionality effects in strongly correlated systems and the emergence of potential new physical scenarios. In…

Strongly Correlated Electrons · Physics 2021-07-13 Carla Boix-Constant , Samuel Mañas-Valero , Rosa Córdoba , Eugenio Coronado

Excitons are spin integer particles that are predicted to condense into a coherent quantum state at sufficiently low temperature, and exciton condensates can be realized at much higher temperature than condensates of atoms because of strong…

Optical dynamics in van der Waals heterobilayers is of fundamental scientific and practical interest. Based on a time-dependent adiabatic GW approach, we discover a new many-electron (excitonic) channel for converting photoexcited…

Materials Science · Physics 2023-05-30 Chen Hu , Mit H. Naik , Yang-Hao Chan , Steven G. Louie

We explore the flatness of conduction and valence bands of interlayer excitons in MoS$_2$/WSe$_2$ van der Waals heterobilayers, tuned by interlayer twist angle, pressure, and external electric field. We employ an efficient continuum model…

Mesoscale and Nanoscale Physics · Physics 2023-11-20 Sara Conti , Andrey Chaves , Tribhuwan Pandey , Lucian Covaci , François M. Peeters , David Neilson , Milorad V. Milošević

Coulomb bound electron-hole pairs, excitons, govern the optical properties of semi-conducting transition metal dichalcogenides like MoS$_2$ and WSe$_2$. We study optical transitions at the K-point for 2H homobilayer MoS$_2$ in Density…

We present a theory of bilayer two-dimensional electron systems that host a spatially indirect exciton condensate when in thermal equilibrium. Equilibrium bilayer exciton condensates (BXCs) are expected to form when two nearby semiconductor…

Mesoscale and Nanoscale Physics · Physics 2017-01-31 Feng-Cheng Wu , Fei Xue , A. H. MacDonald

Interlayer excitons in van der Waals heterostructures offer rich collective phases, prospective optoelectronic applications, and versatile tunability, where control by electronic means is particularly relevant and practical. Here, in the…

Mesoscale and Nanoscale Physics · Physics 2025-02-20 Cem Sevik , Engin Torun , Milorad V. Milosevic , Fulvio Paleari

Van der Waals (vdW) heterobilayers formed by two-dimensional (2D) transition metal dichalcogenides (TMDCs) created a promising platform for various electronic and optical properties. ab initio band results indicate that the band offset of…

Materials Science · Physics 2020-09-04 Yuanyuan Wang , Fengping Li , Wei Wei , Baibiao Huang , Ying Dai

The excitonic insulator, a quantum mechanical state arising from exciton condensation, was proposed theoretically many years ago but has yet to be experimentally confirmed. The discovery of correlated transition metal oxides based on $4d$…

Strongly Correlated Electrons · Physics 2024-10-18 Hidemaro Suwa , Shang-Shun Zhang , Cristian D. Batista

Dielectric structures can support low-absorption optical modes, which are attractive for engineering light-matter interactions with excitonic resonances in two-dimensional (2D) materials. However, the coupling strength is often limited by…

The discovery of new families of exfoliatable 2D crystals that have diverse sets of electronic, optical, and spin-orbit coupling properties, enables the realization of unique physical phenomena in these few-atom thick building blocks and in…

Observation of interlayer, charge-transfer (CT) excitons in van der Waals heterostructures (vdWHs) based on 2D-2D systems has been well investigated. While conceptually interesting, these charge transfer excitons are highly delocalized and…

The van der Waals heterostructures are a fertile frontier for discovering emergent phenomena in condensed matter systems. They are constructed by stacking elements of a large library of two-dimensional materials, which couple together…

Mesoscale and Nanoscale Physics · Physics 2020-05-22 William Dorrell , Harris Pirie , S. Minhal Gardezi , Nathan C. Drucker , Jennifer E. Hoffman

Semiconductor heterostructures provide a powerful platform for the engineering of excitons. Here we report the excitonic properties of two-dimensional (2D) heterostructures that consist of monolayer MoS2 and WS2 stacked epitaxially or…

Excitons in monolayer transition-metal-dichalcogenides (TMDs) dominate their optical response and exhibit strong light-matter interactions with lifetime-limited emission. While various approaches have been applied to enhance light-exciton…

Two dimensional (2D) van der Waals heterostructures from transition metal dichalcogenide (TMDC) semiconductors show a new class of spatially separate excitons with extraordinary properties. The interlayer excitons (XI) have been studied…

Materials Science · Physics 2021-03-02 Jaehoon Ji , Jong Hyun Choi

Coupled two-dimensional electron-hole bilayers provide a unique platform to study strongly correlated Bose-Fermi mixtures in condensed matter. Electrons and holes in spatially separated layers can bind to form interlayer excitons, composite…

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