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We demonstrate the possibility of engineering the optical properties of transition metal dichalcogenide heterobilayers when one of the constitutive layers has a Janus structure. This has important consequences for the charge separation…

Mesoscale and Nanoscale Physics · Physics 2023-05-10 Engin Torun , Fulvio Paleari , Milorad V. Milosevic , Ludger Wirtz , Cem Sevik

Vertically stacked van der Waals structures are promising platforms that enable layer engineering, opening new avenues for the quantum control of elementary excitations, including optically generated bound electron-hole pairs. Here we…

Mesoscale and Nanoscale Physics · Physics 2025-07-16 Alexandre R. Rocha , Rodrigo G. Amorim , Wanderlã L. Scopel , Cesar E. P. Villegas

Artificial moir\'e superlattices in 2d van der Waals heterostructure is a new venue for realizing and controlling correlated electronic phenomena. Recently, twisted bilayer WSe$_2$ emerged as a new robust moir\'e system hosting a correlated…

Strongly Correlated Electrons · Physics 2020-12-02 Zhen Bi , Liang Fu

Excitonic condensate has been long-sought within bulk indirect-gap semiconductors, quantum wells, and 2D material layers, all tried as carrying media. Here we propose intrinsically stable 2D semiconductor heterostructures with…

Mesoscale and Nanoscale Physics · Physics 2020-06-17 Sunny Gupta , Alex Kutana , Boris I. Yakobson

Van der Waals (vdW) materials, with their unique combination of electronic, optical, and magnetic properties, are emerging as promising platforms for exploring excitonic phenomena. Thus far, the choice of materials with exceptional…

Excitons in monolayer semiconductors have large optical transition dipole for strong coupling with light field. Interlayer excitons in heterobilayers, with layer separation of electron and hole components, feature large electric dipole that…

Mesoscale and Nanoscale Physics · Physics 2019-03-07 Wei-Ting Hsu , Bo-Han Lin , Li-Syuan Lu , Ming-Hao Lee , Ming-Wen Chu , Lain-Jong Li , Wang Yao , Wen-Hao Chang , Chih-Kang Shih

Identifying two-dimensional heterostructures with exceptional electronic and optical properties remains an active area of research in advanced optoelectronics. Here, we present a comprehensive first-principles investigation of the…

Van der Waals heterostructures usually formed using atomic thin transition metal dichalcogenides (TMDCs) with a direct bandgap in the near-infrared to the visible range are promising candidates for low-dimensional optoelectronic…

Mesoscale and Nanoscale Physics · Physics 2018-09-21 Guanghui Cheng , Baikui Li , Chunyu Zhao , Xin Yan , Hong Wang , Kei May Lau , Jiannong Wang

Throughout the years, strongly correlated coherent states of excitons have been the subject of intense theoretical and experimental studies. This topic has recently boomed due to new emerging quantum materials such as van der Waals (vdW)…

Mesoscale and Nanoscale Physics · Physics 2021-12-30 Igor V. Bondarev , Oleg L. Berman , Roman Ya. Kezerashvili , Yurii E. Lozovik

Excitons dominate the optics of atomically-thin transition metal dichalcogenides and 2D van der Waals heterostructures. Interlayer 2D excitons, with an electron and a hole residing in different layers, form rapidly in heterostructures…

Mesoscale and Nanoscale Physics · Physics 2021-04-20 M. G. Burdanova , M. Liu , M. Staniforth , Y. Zheng , R. Xiang , S. Chiashi , A. Anisimov , E. I. Kauppinen , S. Maruyama , J. Lloyd-Hughes

Bound electron-hole pairs in semiconductors known as excitons can form a coherent state at low temperatures akin to a BCS condensate. The resulting phase is known as the excitonic insulator and has superfluid properties. Here we…

Strongly Correlated Electrons · Physics 2025-06-06 L. Maisel Licerán , H. T. C. Stoof

Direct-gap materials hold promises for excitonic insulator. In contrast to indirect-gap materials, here the difficulty to distinguish from a Peierls charge density wave is circumvented. However, direct-gap materials still suffer from the…

Materials Science · Physics 2018-08-29 Zeyu Jiang , Yuanchang Li , Shengbai Zhang , Wenhui Duan

Van der Waals heterostructures formed by stacking two-dimensional atomic crystals are a unique platform for exploring new phenomena and functionalities. Interlayer excitons, bound states of spatially separated electron-hole pairs in van der…

Materials Science · Physics 2018-02-14 Zefang Wang , Yi-Hsin Chiu , Kevin Honz , Kin Fai Mak , Jie Shan

Recent theoretical and experimental studies suggest that van der Waals heterostructures with n- and p-doped bilayers of transition metal dichalcogenides are promising facilitators of exciton superfluidity. Exciton superfluidity in such…

Mesoscale and Nanoscale Physics · Physics 2023-08-10 Rune Højlund , Emil Grovn , Sahar Pakdel , Kristian S. Thygesen , Fredrik Nilsson

Strongly bound excitons and many-body interactions between them determine light-matter interactions in van der Waals (vdW) heterostructures of 2D semiconductors. Unlike fundamental particles, quasiparticles in condensed matter, such as…

Mesoscale and Nanoscale Physics · Physics 2022-08-12 Weijie Li , Zach Hadjri , Jin Zhang , Luka M. Devenica , Song Liu , James Hone , Kenji Watanabe , Takashi Taniguchi , Angel Rubio , Ajit Srivastava

Because of the reduced dielectric screening and enhanced Coulomb interactions, two-dimensional (2D) materials like phosphorene and transition metal dichalcogenides (TMDs) exhibit strong excitonic effects, resulting in fascinating…

Materials Science · Physics 2019-11-04 Xiaoyang Zheng , Xian Zhang

The existence of strongly bound excitons is one of the hallmarks of the newly discovered atomically thin semi-conductors. While it is understood that the large binding energy is mainly due to the weak dielectric screening in two dimensions…

Materials Science · Physics 2016-01-20 Simone Latini , Thomas Olsen , Kristian S. Thygesen

Our ability to efficiently detect and generate far-infrared (i.e., terahertz) radiation is vital in areas spanning from biomedical imaging to interstellar spectroscopy. Despite decades of intense research, bridging the terahertz gap between…

Materials Science · Physics 2023-07-24 Zhao Tang , Greis J. Cruz , Fanhao Jia , Yabei Wu , Weiyi Xia , Peihong Zhang

Ensembles of indirect or interlayer excitons (IXs) are intriguing systems to explore classical and quantum phases of interacting bosonic ensembles. IXs are composite bosons that feature enlarged lifetimes due to the reduced overlap of the…

We predict a new family of robust two-dimensional (2D) topological insulators in van der Waals heterostructures comprising graphene and chalcogenides BiTeX (X=Cl, Br and I). The layered structures of both constituent materials produce a…

Materials Science · Physics 2014-12-25 Liangzhi Kou , Shu-Chun Wu , Claudia Felser , Thomas Frauenheim , Changfeng Chen , Binghai Yan
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