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Polarization-dependent x-ray absorption spectroscopy at the B 1s edge of single-crystalline Mg(x)Al(1-x)B(2) reveals a strongly anisotropic electronic structure near the Fermi energy. Comparing spectra for superconducting compounds (x=0.9,…

The electronic structure of BaFe$_2X_3$ ($X$ = S and Se) and CsFe$_2$Se$_3$ in which two-leg ladders are formed by the Fe sites are studied by means of x-ray absorption and resonant inelastic x-ray scattering spectroscopy. The x-ray…

To extend the applicability of density functional theory for superconductors (SCDFT) to systems with significant particle-hole asymmetry, we construct a new exchange-correlation kernel entering the gap equation. We show that the kernel is…

Superconductivity · Physics 2013-07-22 Ryosuke Akashi , Ryotaro Arita

The electronic band structure of correlated Ca3Ru2O7 featuring an antiferromagnetic as well as a structural transition has been determined theoretically at high temperatures, which has led to the understanding of the remarkable properties…

Strongly Correlated Electrons · Physics 2018-01-30 Hui Xing , Libin Wen , Chenyi Shen , Jiaming He , Xinxin Cai , Jin Peng , Shun Wang , Mingliang Tian , Zhu-An Xu , Wei Ku , Zhiqiang Mao , Ying Liu

Metal halide perovskites have emerged as an exciting class of materials for applications in solar energy harvesting, optical devices, catalysis, and other photophysical applications. Many of the exciting properties of halide perovskites are…

Materials Science · Physics 2024-04-18 Colin M. Hylton-Farrington , Richard C. Remsing

The semimetal MoTe$_2$ is studied by spin- and angle- resolved photoemission spectroscopy to probe the detailed electronic structure underlying its broad range of response behavior. A novel spin-texture is uncovered in the bulk Fermi…

Multi-principal-element alloys, including high-entropy alloys, experience segregation or partially-ordering as they are cooled to lower temperatures. For Ti$_{0.25}$CrFeNiAl$_{x}$, experiments suggest a partially-ordered B2 phase, whereas…

Materials Science · Physics 2021-05-11 Prashant Singh , A. V. Smirnov , Aftab Alam , Duane D. Johnson

The electronic structure of Samarium (Sm) was calculated using the density functional theory combined with the single-site dynamical mean-field theory. In this work, we investigated the electronic properties of {\alpha}, \b{eta} and…

Strongly Correlated Electrons · Physics 2026-05-15 Shengsong Xu , Zhenfeng Ouyang , Li Huang , Zhong-Yi Lu

Stable structures of layered SnS and SnSe and their associated electronic and vibrational spectra are predicted using first-principles DFT calculations. The calculations show that both materials undergo a phase transformation upon thinning…

Materials Science · Physics 2019-06-04 Antoine Dewandre , Matthieu J. Verstraete , Nicole Grobert , Zeila Zanolli

We study the electronic properties of the $\textrm{Fe}\textrm{Se}_{1-x}\textrm{Te}_x$ system ($x=0$, 0.25, 0.5, 0.75, and 1) from the perspective of X-ray spectroscopy and density functional theory (DFT). The analysis performed on the…

Superconductivity · Physics 2014-11-10 I. Perez , J. A. Mcleod , R. J. Green , R. Escamilla , V. Ortiz , A. Moewes

The microscopic origin of the large negative thermal expansion of cubic scandium trifluorides (ScF3) is investigated by performing a set of anharmonic free-energy calculations based on density functional theory. We demonstrate that the…

Materials Science · Physics 2019-03-13 Yusuke Oba , Terumasa Tadano , Ryosuke Akashi , Shinji Tsuneyuki

Thin films of CdTe were deposited on glass substrates by thermal evaporation. From the XRD measurements itis found that the films are of zinc-blende-type structure. Transmittance, absorption, extinction, and refractive coefficients are…

Materials Science · Physics 2009-11-11 S. Lalitha , S. Zh. Karazhanov , P. Ravindran , S. Senthilarasu , R. Sathyamoorthy , J. Janabergenov

Using ab initio evolutionary structure prediction method in conjunction with density functional theory, we performed a systematic investigation on the structural transition of elemental scandium under pressure up to 250 GPa. Our prediction…

Materials Science · Physics 2019-01-09 Shengcai Zhu , Xiao-Zhi Yan , Scott Fredericks , Yan-Ling Li , Qiang Zhu

A theoretical investigation was conducted on Na-based fluoro-perovskites NaYF3 (Y = Sc, Ti) to examine their structural, optical, electronic, and mechanical characteristics for the first time. These cubic compounds exhibit structural…

The development of high-performance electron sources requires theoretical frameworks that accurately link the microscopic electronic properties of cathode materials to their macroscopic photoemission observables. Here, we present a…

Materials Science · Physics 2026-02-16 Richard Schier , Chen Wang , Jonas Dube , Julius Kühn , Alice Galdi , Thorsten Kamps , Caterina Cocchi

We present an accurate, first-principles study of the electronic structure and absorption spectrum of bulk copper within Density Functional Theory in the Local Density Approximation (DFT-LDA), including the study of intraband transitions.…

Materials Science · Physics 2009-11-07 Andrea Marini , Giovanni Onida , Rodolfo Del Sole

X-ray photoelectron spectroscopy, ultraviolet photoelectron spectroscopy and density functional theory calculations were used to study the electronic structure of three lanthanide scandates: GdScO3, TbScO3, and DyScO3. X-ray photoelectron…

Materials Science · Physics 2018-02-21 Christopher A. Mizzi , Pratik Koirala , Laurence D. Marks

The halide perovskites have truly emerged as efficient optoelectronic materials and show the promise of exhibiting nontrivial topological phases. Since the bandgap is the deterministic factor for these quantum phases, here we present a…

Materials Science · Physics 2021-03-31 Ravi Kashikar , Mayank Gupta , B. R. K. Nanda

We report an extensive study on the intrinsic bulk electronic structure of the high-temperature superconductor CeFeAsO0.89F0.11 and its parent compound CeFeAsO by soft and hard x-ray photoemission, x-ray absorption and soft-x-ray emission…

Silver fulminate (AgCNO) is a primary explosive, which exists in two polymorphic phases namely orthorhombic (\emph{Cmcm}) and trigonal (\emph{R$\bar{3}$}) forms at ambient conditions. In the present study, we have investigated the effect of…

Materials Science · Physics 2015-06-22 N. Yedukondalu , G. Vaitheeswaran