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High field mangetization, field-dependent specific heat measurements, and zero field inelastic magnetic neutron scattering have been used to explore the magnetic properties of copper pyrazine dinitrate (Cu(C4H4N2)(NO3)2). The material is an…

Strongly Correlated Electrons · Physics 2009-10-31 P. R. Hammar , M. B. Stone , Daniel H. Reich , C. Broholm , P. J. Gibson , M. M. Turnbull , C. P. Landee , M. Oshikawa

The effective spin-1/2 antiferromagnetic Heisenberg-Ising chain materials, ACo$_2$V$_2$O$_8$, A = Sr, Ba, are a rich source of exotic fundamental phenomena and have been investigated for their model magnetic properties both in zero and…

Strongly Correlated Electrons · Physics 2023-09-29 K. Puzniak , C. Aguilar-Maldonado , R. Feyerherm , K. Prokeš , A. T. M. N. Islam , Y. Skourski , L. Keller , B. Lake

The effect of orbital degrees of freedom on the exchange interactions in the spin-1 quasi-one-dimensional antiferromagnet CaV2O4 is systematically studied. For this purpose a realistic low-energy model with the parameters derived from the…

Materials Science · Physics 2015-06-23 Z. V. Pchelkina , I. V. Solovyev

We report the successful growth of high-quality single crystals of \ACVO, a quasi-one-dimensional zigzag chain compound containing Co$^{2+}$ ions, using the optical floating zone method. The crystal growth was stabilized under high-pressure…

Strongly Correlated Electrons · Physics 2025-08-15 Anzar Ali , Guratinder Kaur , Arvind Maurya , Isha , Kathrin Küster , Ulrich Starke , Pascal Puphal , Arvind Kumar Yogi , Masahiko Isobe

Inelastic neutron scattering measurements demonstrate that the magnetic interactions in antiferromagnetic LaFeAsO are two-dimensional. Spin wave velocities within the Fe layer and the magnitude of the spin gap are similar to the…

We report on the crystal structure and magnetic behavior of the spin-1/2 compound AgVOAsO4. Magnetic susceptibility, high-field magnetization, and electron spin resonance measurements identify AgVOAsO4 as a gapped quantum magnet with a spin…

NMR, muSR, magnetization and specific heat measurements in Li(2)VOSiO(4) powders and single crystals are reported. Specific heat and magnetization measurements evidence that Li(2)VOSiO(4) is a frustrated two-dimensional S=1/2 Heisenberg…

Strongly Correlated Electrons · Physics 2009-11-07 R. Melzi , S. Aldrovandi , F. Tedoldi , P. Carretta , P. Millet , F. Mila

We present a comprehensive experimental and ab-initio study of the $S=1/2$ Mo$^{5+}$ system, KMoOP$_2$O$_7$, and show that it realizes the $S = 1/2$ Heisenberg chain antiferromagnet model. Powder neutron diffraction reveals that…

Ni2SiO4, Liebenbergite, is an example of a quasi-one-dimensional magnet made up of frustrated corner sharing triangles of Ni2+ (S = 1) ions that propagate parallel to the b axis. Ni2SiO4 is isostructural with olivine, a common mineral of…

Strongly Correlated Electrons · Physics 2009-07-10 R H Colman , T Fennell , C Ritter , G Lau , R J Cava , A S Wills

Magnetism in the orthorhombic metal CaFe$_4$As$_3$ was examined through neutron diffraction for powder and single crystalline samples. Incommensurate (${\bm q}_{\rm m}\approx (0.37-0.39)\times{\bm b}^{\ast}$) and predominantly…

Elastic and inelastic neutron scattering were used to study the ordered phase of the quasi-one-dimensional spin-1/2 antiferromagnet ${\rm BaCu_{2}Si_{2}O_{7}}$. The previously proposed model for the low-temperature magnetic structure was…

Strongly Correlated Electrons · Physics 2016-08-15 M. Kenzelmann , A. Zheludev , S. Raymond , E. Ressouche , T. Masuda , P. Böni , K. Kakurai , I. Tsukada , K. Uchinokura , R. Coldea

Based on density functional theory band structure calculations, quantum Monte-Carlo simulations, and high-field magnetization measurements, we address the microscopic magnetic model of BaAg2Cu[VO4]2 that was recently proposed as a spin-1/2…

Materials Science · Physics 2012-06-19 Alexander A. Tsirlin , Angela Moeller , B. Lorenz , Yu. Skourski , H. Rosner

Experimental results on magnetic resonance (ESR) and magnetic susceptibility are given for single crystalline (VO)$_2$P$_2$O$_{7}$. The crystal growth procedure is briefly discussed. The susceptibility is interpreted numerically using a…

Condensed Matter · Physics 2009-10-30 A. V. Prokofiev , F. Büllesfeld , W. Assmus , H. Schwenk , D. Wichert , U. Löw , B. Lüthi

We study electronic and magnetic properties of the quasi-one-dimensional spin-1/2 magnet Ba3Cu3Sc4O12 with a distinct orthogonal connectivity of CuO4 plaquettes. An effective low-energy model taking into account spin-orbit coupling was…

Strongly Correlated Electrons · Physics 2016-09-14 D. I. Badrtdinov , O. S. Volkova , A. A. Tsirlin , I. V. Solovyev , A. N. Vasiliev , V. V. Mazurenko

Our experimental (neutron diffraction, M\"ossbauer spectroscopy, magnetic susceptibility, specific heat) and numerical studies on the evolution of short- and long-range magnetic order in $\gamma_{\rm II}$-Li\(_2\)FeSiO\(_4\) suggest a…

Strongly Correlated Electrons · Physics 2025-01-20 W. Hergett , N. Bouldi , M. Jonak , C. Neef , C. Ritter , M. Abdel-Hafiez , F. Seewald , H. -H. Klauss , M. W. -Haverkort , R. Klingeler

We investigate magnetic excitations in the frustrated zigzag spin-1/2 chain compound $\beta$-TeVO$_4$ by inelastic neutron scattering. In the magnetically ordered ground state, the excitation spectrum exhibits coexisting magnon dispersion,…

Strongly Correlated Electrons · Physics 2018-09-10 M. Pregelj , O. Zaharko , U. Stuhr , A. Zorko , H. Berger , A. Prokofiev , D. Arčon

The low-temperature electron spin resonance (ESR) spectra and the static magnetization data obtained for the stoichiometric single crystals of $\beta$-Na$_{0.33}$V$_2$O$_5$ indicate that this quasi-one-dimensional mixed valence (V4+/V5+)…

Strongly Correlated Electrons · Physics 2009-10-31 A. N. Vasil'ev , V. I. Marchenko , A. I. Smirnov , S. S. Sosin , H. Yamada , Y. Ueda

The magnetic correlations in the quasi-two dimensional spin-1/2 square-lattice system Zn2VO(PO4)2 have been investigated by neutron diffraction technique. A long-range antiferromagnetic (AFM) ordering below 3.75 K (TN) has been observed…

Materials Science · Physics 2015-05-19 S. M. Yusuf , A. K. Bera , N. S. Kini , I. Mirebeau , S. Petit

The title quasi-1D copper oxides (0=< x =<0.4) were investigated by neutron diffraction and magnetic susceptibility studies. Polyhedral CuO4 units in the compounds were found to comprise linear-chains at inter-chain distance of…

Superconductivity · Physics 2009-11-07 K. Yamaura , Q. Huang , E. Takayama-Muromachi

We present a joint experimental and computational study of the recently synthesized spin 1/2 system silver-copper-orthovanadate AgCuVO4 [A. M\"oller and J. Jainski, Z. Anorg. Allg. Chem. 634, 1669 (2008)] exhibiting chains of trans…

Strongly Correlated Electrons · Physics 2009-10-12 A. Möller , M. Schmitt , W. Schnelle , T. Förster , H. Rosner