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Related papers: Density anomaly in water-alcohol mixtures: minimum…

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We study the change in the temperature of maximum density (TMD) of a water-like solvent when small amounts of solute are added to the mixture. The water is modeled as a two length scales potential, which is known to exhibit water-like…

Soft Condensed Matter · Physics 2022-09-14 Marco Antônio Habitzreuter , Marcia C. Barbosa

We perform an extensive computational study of binary mixtures of water and short-chain alcohols resorting to two-scale potential models to account for the singularities of hydrogen bonded liquids. Water molecules are represented by a well…

Soft Condensed Matter · Physics 2017-04-26 A. P. Furlan , E. Lomba , M. C. Barbosa

We address the investigation of the solvation properties of the minimal orientational model for water, originally proposed by Bell and Lavis. The model presents two liquid phases separated by a critical line. The difference between the two…

Statistical Mechanics · Physics 2015-06-05 Marcia M. Szortyka , Carlos E. Fiore , Marcia C. Barbosa , Vera B. Henriques

After melting, at ambient pressure, the density of water continues to increase with temperature until it reaches a maximum around 4 {\deg}C. For nearly a century, this phenomenon has been qualitatively attributed to a mixture of ordered and…

Chemical Physics · Physics 2026-03-31 Yizhi Song , Renxi Liu , Chunyi Zhang , Yifan Li , Biswajit Santra , Mohan Chen , Michael L. Klein , Xifan Wu

Short-chain alcohols at high dilution are among the very few solutes that enhance the anomalous behavior of water, in particular the value of the temperature of maximum density. This peculiar feature, first discovered experimentally in the…

Soft Condensed Matter · Physics 2021-07-28 Murilo S. Marques , Enrique Lomba , Eva G. Noya , D. González-Salgado , Marcia C. Barbosa

In this paper we investigate the solubility of a hard - sphere gas in a solvent modeled as an associating lattice gas (ALG). The solution phase diagram for solute at 5% is compared with the phase diagram of the original solute free model.…

Statistical Mechanics · Physics 2012-05-10 Marcia M. Szortyka , Maurício Girardi , Vera B. Henriques , Marcia C. Barbosa

We use molecular dynamics simulations in two dimensions to investigate the possibility that a core-softened potential can reproduce static and dynamic anomalies found experimentally in liquid water: (i) the increase in specific volume upon…

Soft Condensed Matter · Physics 2009-10-31 A. Scala , M. Reza Sadr-Lahijany , N. Giovambattista , S. V. Buldyrev , H. E. Stanley

We investigate a lattice-fluid model of water, defined on a 3-dimensional body-centered cubic lattice. Model molecules possess a tetrahedral symmetry, with four equivalent bonding arms. The model is similar to the one proposed by Roberts…

Soft Condensed Matter · Physics 2016-08-31 M. Pretti , C. Buzano

Using molecular dynamic simulations we study a waterlike model confined between two fixed hydrophobic plates. The system is tested for density, diffusion and structural anomalous behavior and compared with the bulk results. Within the range…

Chemical Physics · Physics 2013-03-06 Leandro Batirolla Krott , Marcia Cristina Bernardes Barbosa

Very recently the effect of equisized charged hard sphere solutes in a mixture with core-softened fluid model on the structural and thermodynamic anomalies of the system has been explored in detail by using Monte Carlo simulations and…

Soft Condensed Matter · Physics 2013-12-18 B. Hribar-Lee , O. Pizio

Using Monte Carlo simulations a lattice gas model with only repulsive interactions was checked for the presence of anomalies. We show that this system exhibits the density (temperature of maximum density - TMD) and diffusion anomalies as…

Statistical Mechanics · Physics 2016-11-25 Andressa A. Bertolazzo , Marcia C. Barbosa

The so-called thermodynamic anomalies of water form an integral part of the peculiar behaviour of this both important and ubiquitous molecule. In this paper our aim is to establish whether the recently proposed TIP4P/2005 model is capable…

We report Monte Carlo results for the fluid structure of a system of dimeric particles interacting via a core-softened potential. More specifically, dimers interact through a repulsive pair potential of inverse-power form, modified in such…

Soft Condensed Matter · Physics 2016-03-08 Gianmarco Munaò , Franz Saija

Methanol is an amphiphilic solute whose aqueous solutions exhibit distinctive physical properties. The volume change upon mixing, for example, is negative across the entire composition range, indicating strong association. We explore the…

Soft Condensed Matter · Physics 2015-06-03 Zhiqiang Su , Sergey V. Buldyrev , Pablo G. Debenedetti , Peter J. Rossky , H. Eugene Stanley

We have studied the composition dependence of density of liquid water-DMSO mixtures at different temperatures by using the isobaric-isothermal (NPT) molecular dynamics computer simulations. The non-polarizable semi-flexible, P1 and P2…

Soft Condensed Matter · Physics 2023-01-05 M. Aguilar , H. Dominguez , O. Pizio

We study the effects of two kinds of interactions in tube-like polymers and demonstrate that they result in the formation of secondary motifs. The first has an entropic origin and is a measure of the effective space available to the…

Statistical Mechanics · Physics 2009-11-13 Chiara Poletto , Achille Giacometti , Antonio Trovato , Jayanth R. Banavar , Amos Maritan

In this work, we discuss the connection between the anomalies of the thermodynamic properties, experimentally observed in tertiary butyl alcohol (TBA) and water solutions, and the molecular clustering in these solutions, as revealed by…

Soft Condensed Matter · Physics 2013-08-19 Deepa Subramanian , Jeffery B. Klauda , Jan Leys , Mikhail A. Anisimov

The thermodynamic liquid-state anomalies and associated structural changes of the Stillinger-Weber family of liquids are mapped out as a function of the degree of tetrahedrality of the interaction potential, focusing in particular on…

Soft Condensed Matter · Physics 2011-09-09 Waldemar Hujo , B. Shadrack Jabes , Varun K. Rana , Charusita Chakravarty , Valeria Molinero

In this contribution we review a series of simple one dimensional lattice models that with an appropriate choice of parameters can account for various anomalous features of the behaviour of complex systems such as water. In particular, we…

Statistical Mechanics · Physics 2015-03-13 Enrique Lomba

Water is a complex structured liquid of hydrogen-bonded molecules that displays a surprising array of unusual properties, also known as water anomalies, the most famous being the density maximum at about $4^\circ$C. The origin of these…

Soft Condensed Matter · Physics 2015-06-16 John Russo , Hajime Tanaka
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