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The loss of information about the relative phase between two quantum states, known as decoherence, strongly limits resolution in electron paramagnetic spectroscopy and hampers the use of molecules for quantum information processing. At low…

Quantum Physics · Physics 2025-04-28 Conor Ryan , Valerio Briganti , Cathal Hogan , Mark O'Neill , Alessandro Lunghi

We investigate the inelastic spin-flip rate for electrons in a quantum dot due to their contact hyperfine interaction with lattice nuclei. In contrast to other works, we obtain a spin-phonon coupling term from this interaction by taking…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Veniamin A. Abalmassov , Florian Marquardt

Nuclear spin relaxation is studied in n-GaAs thick layers and microcavity samples with different electron densities. We reveal that both in metallic samples where electrons are free and mobile, and in insulating samples, where electrons are…

We discuss the implications of a small indium content (3%) in a GaAs epilayer on the electron- and nuclear-spin relaxation due to enhanced quadrupolar effects induced by the strain. Using the weakly perturbative spin-noise spectroscopy, we…

Mesoscale and Nanoscale Physics · Physics 2022-07-27 C. Rittmann , M. Yu. Petrov , A. N. Kamenskii , K. V. Kavokin , A. Yu. Kuntsevich , Yu. P. Efimov , S. A. Eliseev , M. Bayer , A. Greilich

We have characterized spin-squeezed states produced at a temperature of $26^\circ{\mathrm C}$ on a Nuclear Magnetic Resonance (NMR) quadrupolar system. The implementation is carried out in an ensemble of $^{133}$Cs nuclei with spin $I=7/2$…

We develop a theory in order to describe the effect of relaxation in a condensed medium upon the quantum decay of a metastable liquid near the spinodal at low temperatures. We find that both the regime and the rate of quantum nucleation…

Statistical Mechanics · Physics 2009-11-10 S. N. Burmistrov , L. B. Dubovskii , Y. Okuda

We investigate the role of the nuclear spin quantum dynamics in hyperfine-induced spin relaxation of hopping carriers in organic semiconductors. The fast hopping regime with a small carrier spin precession during a waiting time between hops…

Mesoscale and Nanoscale Physics · Physics 2017-06-21 V. V. Mkhitaryan , V. V. Dobrovitski

Current typical methods to realize nuclear-nuclear quantum gates require a sequence of electronnuclear quantum gates by using dynamical decoupling techniques, which are implemented at low temperature because of short decoherence and…

Quantum Physics · Physics 2022-04-27 Jiawen Jiang , Q. Chen

Using the ab initio computed Potential Energy Surface (PES) for the electronic interaction of the MgH$^+$ ($^1\Sigma$) ion with the He($^1$S) atom, we calculate the relevant state-changing rotationally inelastic collision cross sections…

Atomic Physics · Physics 2020-10-28 L. González-Sánchez , R. Wester , F. A. Gianturco

Electrons in a two-dimensional semiconducting heterostructure interact with nuclear spins via the hyperfine interaction. Using a a Kondo lattice formulation of the electron-nuclear spin interaction, we show that the nuclear spin system…

Strongly Correlated Electrons · Physics 2015-06-25 Pascal Simon , Daniel Loss

Optically accessible solid state defect spins serve as a primary platform for quantum information processing, where precise control of the electron spin and ancillary nuclear spins is essential for operation. Using the nitrogen-vacancy (NV)…

Quantum Physics · Physics 2026-02-12 Gergő Thiering , Adam Gali

The prospects of sympathetic cooling of polar molecules with magnetically co-trapped alkali-metal atoms are generally considered poor due to strongly anisotropic atom-molecule interactions leading to large spin relaxation rates. Using…

Atomic Physics · Physics 2012-02-06 T. V. Tscherbul , J. Klos , A. A. Buchachenko

Modeling blocking temperature in molecular magnets has been a long standing problem in the field of molecular magnetism. We investigate this problem using a kinetic Monte Carlo (kMC) approach on an assembly of 100,000 short molecular…

Strongly Correlated Electrons · Physics 2021-06-23 Sumit Haldar , S. Ramasesha

We study the low-temperature dynamics of a shallow donor, e.g., $^{31}$P, impurity electron spin in silicon, interacting with the bath of nuclear spins of the $^{29}$Si isotope. For small applied magnetic fields, the electron spin…

Mesoscale and Nanoscale Physics · Physics 2010-09-22 Semion Saykin , Dima Mozyrsky , Vladimir Privman

We derived a simple reduced form from the exact solution of the mixed magnetic and quadrupolar nuclear spin--lattice relaxation function at the central transition line of a quadrupole-split NMR spectrum for the nuclear spin $I$ = 3/2. The…

Superconductivity · Physics 2024-11-27 Yutaka Itoh , Akihiro Ogawa , Seiji Adachi

Ultracold collisions between spin-polarized Na atoms and vibrationally excited Na_2 molecules are investigated theoretically, using both an inelastic formalism (neglecting atom exchange channels) and a reactive formalism (including atom…

Soft Condensed Matter · Physics 2009-11-07 Pavel Soldan , Marko T. Cvitas , Jeremy M. Hutson , Pascal Honvault , Jean-Michel Launay

We present an accurate quantum mechanical study of molecule-molecule collisions in the presence of a magnetic field. The work focusses on the analysis of elastic scattering and spin relaxation in collisions of O2(3Sigma_g) molecules at cold…

Atomic Physics · Physics 2012-02-06 T. V. Tscherbul , Yu. V. Suleimanov , V. Aquilanti , R. V. Krems

Elastic and spin-changing inelastic collision cross sections are presented for cold and ultracold magnetically trapped NH. The cross sections are obtained from coupled-channel scattering calculations as a function of energy and magnetic…

We calculate the proton and neutron spin contributions for nuclei using semi-empirical methods, as well as a novel hybrid \emph{ab initio}/semi-empirical method, for interpretation of experimental data. We demonstrate that core-polarisation…

High Energy Physics - Phenomenology · Physics 2015-03-10 Y. V. Stadnik , V. V. Flambaum

We use state- and time-resolved coherent Raman spectroscopy to study the rotational dynamics of oxygen molecules in ultra-high rotational states. While it is possible to reach rotational quantum numbers up to $N \approx 50$ by increasing…

Chemical Physics · Physics 2015-06-19 Alexander A. Milner , Aleksey Korobenko , Valery Milner