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Below its N\'eel temperature, the frustrated magnet CdCr$_2$O$_4$ exhibits an antiferromagnetic spin-spiral ground state. Such states can give rise to a sizable magnetoelectric coupling. In this report, we measure the electric polarization…

Materials Science · Physics 2020-07-15 L. Rossi , D. Brüning , H. Ueda , Y. Skourski , T. Lorenz , B. Bryant

We show influence of electric field and magnetic flux on spin entanglement in an artificial triangular molecule build of coherently coupled quantum dots. In a subspace of doublet states an explicit relation of concurrence with spin…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Jukub Luczak , Bogdan R. Bulka

Spin-orbit coupling introduces chirality into electronic structure. This can have profound effects on the magnetization induced by orbital motion of electrons. Here we derive a formula for the orbital magnetization of interacting electrons…

Strongly Correlated Electrons · Physics 2014-09-23 R. Nourafkan , G. Kotliar , A. -M. S. Tremblay

Ferromagnet-ferroelectric-metal superlattices are proposed to realize the large room-temperature magnetoelectric effect. Spin dependent electron screening is the fundamental mechanism at the microscopic level. We also predict an electric…

Mesoscale and Nanoscale Physics · Physics 2009-12-16 Tianyi Cai , Sheng Ju , Jaekwang Lee , Na Sai , Alexander A. Demkov , Qian Niu , Zhenya Li , Junren Shi , Enge Wang

The magnetization reversal in a single molecular magnet (SMM) weakly coupled to an electrode with spin-dependent splitting of chemical potentials (spin bias) is theoretically investigated by means of the rate equation. A microscopic…

Mesoscale and Nanoscale Physics · Physics 2009-05-14 Hai-Zhou Lu , Bin Zhou , Shun-Qing Shen

The magneto-electric (ME) coupling on spin-wave resonances in single-crystal Cu2OSeO3 was studied by a novel technique using electron spin resonance combined with electric field modulation. An external electric field E induces a magnetic…

Strongly Correlated Electrons · Physics 2015-06-04 A. Maisuradze , A. Shengelaya , H. Berger , D. M. Djokić , H. Keller

Spin-dependent electric dipole operators are investigated group-theoretically for the emergence of an electric dipole induced by a single spin or by two spins, where the spin dependences are completely classified up to the quadratic order.…

Strongly Correlated Electrons · Physics 2017-02-09 Masashige Matsumoto , Kosuke Chimata , Mikito Koga

Electron spins in single molecules are a promising platform for quantum information processing. However, their practical implementation as qubits requires reliable control at the single-entity level, including an efficient state…

In single molecular magnets, chiral vibrations carrying vibrational angular momentum ($\hat{L}^{\text{vib}}$) emerge due to the splitting of a doubly degenerate vibrational mode. Here, we identify a new type of effective spin-vibrational…

Mesoscale and Nanoscale Physics · Physics 2025-05-19 Aman Ullah , Sergey A. Varganov , Yafis Barlas

We have performed high resolution neutron diffraction and inelastic neutron scattering experiments in the frustrated multiferroic hexagonal compounds RMnO3 (R=Ho, Yb, Sc, Y), which provide evidence of a strong magneto-elastic coupling in…

Strongly Correlated Electrons · Physics 2009-06-01 X. Fabreges , S. Petit , I. Mirebeau , S. Pailhes , L. Pinsard , A. Forget , M. T. Fernandez-Diaz , F. Porcher

The molecular electric dipole, quadrupole and octupole moments of a selected set of 21 spin-compensated molecules are determined employing the extended version of the Piris natural orbital functional 6 (PNOF6), using the triple-$\zeta$…

Chemical Physics · Physics 2016-08-11 Ion Mitxelena , Mario Piris

An accurate description of the two-electron density, crucial for magnetic coupling in spin systems, provides in general a major challenge for density functional theory calculations. It affects, e.g., the calculated zero-field splitting…

Quantum Physics · Physics 2020-05-06 Timur Biktagirov , Wolf Gero Schmidt , Uwe Gerstmann

Spin tunneling in molecular magnets controlled by dipole-dipole interactions (DDI) in the disordered state has been considered numerically on the basis of the microscopic model using the quantum mean-field approximation. In the actual case…

Statistical Mechanics · Physics 2014-01-07 D. A. Garanin

A key to building functional devices on the basis of single molecule magnets in the framework of molecular electronics is the ability to deposit and study these molecules on a surface, because the structural, electronic and magnetic…

Mesoscale and Nanoscale Physics · Physics 2016-01-26 Judith Donner , Jan-Philipp Broschinski , Bastian Feldscher , Anja Stammler , Hartmut Bögge , Thorsten Glaser , Daniel Wegner

Spin tunneling in molecular magnets has attracted much attention, however theoretical considerations of this phenomenon up to now have not taken into account the many-spin nature of molecular magnets. We present, to our knowledge, the first…

Materials Science · Physics 2009-10-31 M. Al-Saqer , V. V. Dobrovitski , B. N. Harmon , M. I. Katsnelson

We describe a simple scheme for the implementation and control of effective spin-spin interactions in self-assembled crystals of cold polar molecules. In our scheme spin states are encoded in two long-lived rotational states of the…

Quantum Physics · Physics 2015-05-30 Y. L. Zhou , M. Ortner , P. Rabl

Magnetic excitations are important quantum phenomena in magnetic systems and have been widely studied in individual magnetic atoms and molecules as well as their assembled structures over the past few decades. Using scanning tunneling…

Electric field control of magnetism is the key to many next generation spintronics applications1. Ferroelectric control of spin polarization2,3 followed by the electrically driven repeatable magnetization reversal in the absence of applied…

Materials Science · Physics 2016-01-14 Gaurav Vats , Ashok Kumar , Ram S. Katiyar , Nora Ortega

We propose a general protocol for on-demand generation of robust entangled states of nuclear and/or electron spins of ultracold $^1\Sigma$ and $^2\Sigma$ polar molecules using electric dipolar interactions. By encoding a spin-1/2 degree of…

Quantum Physics · Physics 2023-04-10 Timur V. Tscherbul , Jun Ye , Ana Maria Rey

Embedding a magnetic electroactive molecule in a three-terminal junction allows for the fast and local electric field control of magnetic properties desirable in spintronic devices and quantum gates. Here, we provide an example of this…