Related papers: Large Amplitude Oscillatory Shear Study of a Collo…
Colloidal gels form through the sol-gel transition of attractive particle suspensions, where local aggregation leads to a space-spanning network with solid-like properties. Their microstructure and mechanical properties are highly sensitive…
We provide the first characterization of the nonlinear and time dependent rheologic response of viscoelastic bottom-up holographic models. More precisely, we perform oscillatory shear tests in holographic massive gravity theories with…
We examine microstructural and mechanical changes which occur during oscillatory shear flow and reformation after flow cessation of an intermediate volume fraction colloidal gel using rheometry and Brownian Dynamics (BD) simulations. A…
We report on the response of a yield stress material, namely a colloidal gel made of attractive carbon black particles, submitted to large amplitude oscillatory shear stress (LAOStress). At a constant stress amplitude well below its…
Many metastable complex fluids such as colloidal glasses and gels show distinct nonlinear viscoelasticity with increasing oscillatory-strain amplitude; the storage modulus decreases monotonically as the strain amplitude increases whereas…
Soft particulate gels can reversibly yield when sufficient deformation is applied, and the characteristics of this transition can be enhanced or limited by designing hybrid hydrogel composites. While the microscopic dynamics and macroscopic…
Using a combination of theory, experiment and simulation we investigate the nonlinear response of dense colloidal suspensions to large amplitude oscillatory shear flow. The time-dependent stress response is calculated using a recently…
In this work we study onset of nonlinear rheological behavior of a colloidal dispersion of a synthetic hectorite clay, Laponite, at the critical gel state while undergoing sol-gel transition. When subjected to step strain in the nonlinear…
We report direct measurements of spatially resolved surface stresses of a dense suspension during large amplitude oscillatory shear (LAOS) in the discontinuous shear thickening regime using boundary stress microscopy. Consistent with…
We introduce a comprehensive scheme to physically quantify both viscous and elastic rheological nonlinearities simultaneously, using an imposed large amplitude oscillatory shear (LAOS) strain. The new framework naturally lends a physical…
Large Amplitude Oscillatory Shear (LAOS) is a key technique for characterizing nonlinear viscoelasticity in a wide range of materials. Most research to date has focused on the shear stress response to an oscillatory strain input. However,…
We investigate theoretically shear banding in large amplitude oscillatory shear (LAOS) of polymers and wormlike micelles. In LAOStrain we find banding at low frequencies and sufficiently high strain rate amplitudes in fluids for which the…
The evolution of viscoelastic properties near the sol-gel transition is studied by performing oscillatory rheological measurements on two different types of systems: a colloidal dispersion and a thermo-responsive polymer solution under…
Variable-amplitude oscillatory shear tests are emerging as powerful tools to investigate and quantify the nonlinear rheology of amorphous solids, complex fluids and biological materials. Quite a few recent experimental and atomistic…
In a recent work, Wyss, {\it et.al.} [Phys. Rev. Lett., {\bf 98}, 238303 (2007)] have noted a property of `soft solids' under oscillatory shear, the so-called strain-rate frequency superposition (SRFS). We extend this study to the case of…
This study presents an experimental framework for large amplitude oscillatory extension (LAOE) to investigate nonlinear material properties of complex fluids. Using a microfluidic optimized shape cross-slot extensional rheometer, we…
We report measurements of the frequency-dependent shear moduli of aging colloidal systems that evolve from a purely low-viscosity liquid to a predominantly elastic glass or gel. Using microrheology, we measure the local complex shear…
Fatigue refers to the changes in material properties caused by repeatedly applied loads. It has been widely studied for, e.g., construction materials, but much less has been done on soft materials. Here, we characterize the fatigue dynamics…
We consider a model dense colloidal dispersion at the glass transition, and investigate the connection between equilibrium stress fluctuations, seen in linear shear moduli, and the shear stresses under strong flow conditions far from…
The large amplitude oscillatory shear (LAOS) has been extensively studied for understanding the rheological responses of yield stress fluids. However, the employed methodology for determining the yield stress remains uncertain albeit the…