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Complex absorbing potentials (CAPs) are artificial potentials added to electronic Hamiltonians to make the wave function of metastable electronic states square-integrable. This makes electronic-structure theory of resonances comparable to…

Chemical Physics · Physics 2023-12-27 Jerryman A. Gyamfi , Thomas-C. Jagau

The complex absorbing potential (CAP) technique is one of the commonly used Non-Hermitian quantum mechanics approaches for characterizing electronic resonances. CAP combined with various electronic structure methods has shown promising…

Chemical Physics · Physics 2025-03-11 Soubhik Mondal , Ksenia B. Bravaya

The Complex Absorbing Potential (CAP) method is widely used to compute resonances in Quantum Chemistry, both for nonrelativistic and relativistic Hamiltonians. In the semiclassical limit $\hbar \to 0$ we consider resonances near the real…

Analysis of PDEs · Mathematics 2013-10-08 J. Kungsman , M. Melgaard

Electronic resonances are metastable states that can decay by electron loss. They are ubiquitous across various fields of science, such as chemistry, physics, and biology. However, current theoretical and computational models for resonances…

Chemical Physics · Physics 2025-04-15 Yann Damour , Anthony Scemama , Fábris Kossoski , Pierre-François Loos

The complex absorbing potential (CAP) formalism has been successfully employed in various wavefunction-based methods to study electronic resonance states. In contrast, Green's function-based methods are widely used to compute ionization…

Chemical Physics · Physics 2026-05-20 Loris Burth , Fábris Kossoski , Pierre-François Loos

We study the Complex Absorbing Potential (CAP) Method in computing quantum resonances of width $c(h) = O(h^N)$, $N\gg1$. We show that up to $h^{-M}\sqrt{c(h)} +\Oh$ error, $M\gg1$, resonances are perturbed eigenvalues of the CAP Hamiltonian…

Mathematical Physics · Physics 2007-05-23 Plamen Stefanov

We show that the complex absorbing potential (CAP) method for computing scattering resonances applies to the case of exponentially decaying potentials. That means that the eigenvalues of $-\Delta + V - i\epsilon x^2$, $|V(x)|\leq C…

Spectral Theory · Mathematics 2021-03-17 Haoren Xiong

The conditions for optimal reflection-free complex-absorbing potentials (CAPs) are discussed. It is shown that the CAPs as derived from the smooth-exterior-scaling transformation of the Hamiltonian,[J. Phys. B. 31, 1431 (1998)], serve as…

Quantum Physics · Physics 2009-11-11 Oded Shemer , Daria Brisker , Nimrod Moiseyev

Electronic resonances are metastable states with finite lifetimes, encountered in processes such as photodetachment, electron transmission, and Auger decay. Resonances appear in Hermitian quantum mechanics as increased density of states in…

Chemical Physics · Physics 2025-11-10 Cansu Utku , Garrette Pauley Paran , Thomas-C. Jagau

Based on the complex absorbing potential (CAP) method, a Lorentzian expansion scheme is developed to express the self-energy. The CAP-based Lorentzian expansion of self-energy is employed to solve efficiently the Liouville-von Neumann…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Hang Xie , Yanho Kwok , Feng Jiang , Xiao Zheng , GuanHua Chen

We show that the complex absorbing potential (CAP) method for computing scattering resonances applies to an abstractly defined class of black box perturbations of the Laplacian in $\mathbb{R}^n$ which can be analytically extended from…

Mathematical Physics · Physics 2022-03-09 Haoren Xiong

We introduce a stochastic framework based on complex absorbing potentials (CAPs) to investigate exciton transport in large molecular aggregates. Within this approach, CAPs act as non-Hermitian reservoirs and sinks that enable effective…

Chemical Physics · Physics 2026-05-19 Dimitri Bazile , Justin Caram , Chern Chuang , Daniel Neuhauser

Complex eigenvalues, resonances, play an important role in large variety of fields in physics and chemistry. For example, in cold molecular collision experiments and electron scattering experiments, autoionizing and pre-dissociative…

Quantum Physics · Physics 2016-09-28 Arie Landau , Idan Haritan , Petra Ruth Kaprálová-Žďánská , Nimrod Moiseyev

Installation of capacitors in distribution networks is one of the most used procedure to compensate reactive power generated by loads and, consequently, to reduce technical losses. So, the problem consists in identifying the optimal…

Optimization and Control · Mathematics 2017-02-01 André R. Goncalves , Celso Cavelucci , Christiano Lyra Filho , Fernando J. Von Zuben

The superposition of atomic potentials (SAP) approach has recently been shown to be a simple and efficient way to initialize electronic structure calculations [S. Lehtola, J. Chem. Theory Comput. 15, 1593 (2019)]. Here, we study the…

Computational Physics · Physics 2020-04-13 Susi Lehtola , Lucas Visscher , Eberhard Engel

Non-Hermitian systems have recently shown new possibilities to manipulate wave scattering by exploiting loss, yet coherent perfect absorption at an exceptional point (CPA EP) remains elusive in acoustics. Here we demonstrate it based on a…

Applied Physics · Physics 2025-06-06 Yi-Fei Xia , Zi-Xiang Xu , Yu-Ting Yan , An Chen , Jing Yang , Bin Liang , Jian-Chun Cheng , Johan Christensen

Objective: In cochlear implant users with residual acoustic hearing, compound action potentials (CAPs) can be evoked by acoustic (aCAP) or electric (eCAP) stimulation and recorded through the electrodes of the implant. We propose a novel…

Medical Physics · Physics 2024-10-28 Daniel Kipping , Yixuan Zhang , Waldo Nogueira

In electronic structure calculations the optimized effective potential (OEP) is a method that treats exchange interactions exactly using a local potential within density-functional theory (DFT). We present a method using density functional…

Materials Science · Physics 2013-01-24 Tom W. Hollins , Stewart J. Clark , Keith Refson , Nikitas I. Gidopoulos

We present the theory for the evaluation of non-adiabatic couplings (NACs) involving resonance states within the complex absorbing potential equation-of-motion coupled-cluster (CAP-EOM-CC) framework implemented within the singles and…

We characterize the resonances of Stark Hamiltonians by the complex absorbing potential method. Namely, we prove that the Stark resonances are the limit points of complex eigenvalues of the Stark Hamiltonian with a quadratic complex…

Mathematical Physics · Physics 2024-02-06 Kentaro Kameoka
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