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We report on the experimental characterization of the second-order susceptibility in MoSe$_2$/WS$_2$ heterobilayers, including their hidden complex phases. To this end, we developed a heterodyne-detection scheme for second-harmonic…

Materials Science · Physics 2025-12-10 Zeyuan Zhu , Taejun Yoo , Kanchan Shaikh , Amalya C. Johnson , Qiuyang Li , Fang Liu , Hui Deng , Yuki Kobayashi

Magnetic two-dimensional (2D) semiconductors have attracted a lot of attention because modern preparation techniques are capable of providing single crystal films of these materials with precise control of thickness down to the single-layer…

Atomic monolayers represent a novel class of materials to study localized and free excitons in two dimensions and to engineer optoelectronic devices based on their significant optical response. Here, we investigate the role of the substrate…

Mesoscale and Nanoscale Physics · Physics 2017-07-21 Oliver Iff , Yu-Ming He , Nils Lundt , Sebastian Stoll , Vasilij Baumann , Sven Höfling , Christian Schneider

The performance of state-of-the-art superconducting quantum devices is currently limited by microwave dielectric losses at different surfaces and interfaces. {\alpha}-tantalum is a superconductor that has proven effective in reducing…

In this letter we report on the synthesis of monolayers of MoS$_2$ via chemical vapor deposition directly on thin films of Al$_2$O$_3$ grown by spatial atomic layer deposition. The synthesized monolayers are characterized by atomic force…

We investigated the electronic structure of monolayer VTe2 grown on bilayer graphene by angle-resolved photoemission spectroscopy (ARPES). We found that monolayer VTe2 takes the octahedral 1T structure in contrast to the monoclinic one in…

Incorporating a monolayer of WS$_2$ via interface engineering enhances the overall physical properties of a FAPbI3 perovskite based heterostructure. FAPbI$_3$/WS$_2$/TiO$_2$/ITO and FAPbI$_3$/TiO$_2$/ITO heterostructures were analyzed by…

The self-assembled monolayers of alkane thiolates on Ag (111) surfaces and nanoparticles are studied using molecular dynamics. Reactive force fields allow simulations of very large systems such as nanoparticles of 10 nm. Stable (sqrt(7) X…

Chemical Physics · Physics 2024-01-11 Adam Lahouari , Jean-Philip Piquemal , Johannes Richardi

We present a new double-layer design for 2D surface superlattice systems in GaAs-AlGaAs heterostructures. Unlike previous studies, our device (1) uses an in-situ gate, which allows very short period superlattice in high mobility, shallow…

Mesoscale and Nanoscale Physics · Physics 2024-03-13 D. Q. Wang , D. Reuter , A. D. Wieck , A. R. Hamilton , O. Klochan

We report a characterization of surfaces of the dichalcogenide TaSe$_2$ using scanning tunneling microscopy and spectroscopy (STM/S) at 150 mK. When the top layer has the 2H structure and the layer immediately below the 1T structure, we…

We perform ab initio calculations of hydrogen-based tunneling defects in alumina to identify deleterious two-level systems (TLS) in superconducting qubits. The defects analyzed include bulk hydrogenated Al vacancies, bulk hydrogen…

Materials Science · Physics 2013-10-23 Aaron M. Holder , Kevin D. Osborn , C. J. Lobb , Charles B. Musgrave

Transition metal dichalcogenides such as MoS$_2$ represent promising candidates for building blocks of ultra-thin nanophotonic devices. For such applications, vertically-oriented MoS$_2$ (v-MoS$_2$) nanosheets could be advantageous as…

Materials Science · Physics 2020-01-29 M. Bolhuis , J. Hernandez-Rueda , S. E. van Heijst , M. Tinoco Rivas , L. Kuipers , S. Conesa-Boj

Titanium dioxide (TiO$_2$) plays a central role in the study of artificial photosynthesis, owing to its ability to perform photocatalytic water splitting. Despite over four decades of intense research efforts in this area, there is still…

Materials Science · Physics 2016-07-28 Christopher E. Patrick , Feliciano Giustino

The superconducting (SC) phase diagram in uranium ditelluride is explored under magnetic fields ($H$) along the hard magnetic b-axis using a high-quality single crystal with $T_{\rm c} = 2.1$ K. Simultaneous electrical resistivity and AC…

Superconductivity · Physics 2023-05-18 H. Sakai , Y. Tokiwa , P. Opletal , M. Kimata , S. Awaji , T. Sasaki , D. Aoki , S. Kambe , Y. Tokunaga , Y. Haga

The conditions whereby epitaxy is achieved are commonly believed to be mostly governed by misfit strain. We report on a systematic investigation of growth and interface structure of single crystalline tungsten thin films on two different…

Individual atomic defects in 2D materials impact their macroscopic functionality. Correlating the interplay is challenging, however, intelligent hyperspectral scanning tunneling spectroscopy (STS) mapping provides a feasible solution to…

Lower thermal stability due to thinning often leads to unprecedented hidden phases in low-dimensional materials. Such hidden phases can coexist or compete with preexisting electronic phases. We investigate hidden phases observed in…

Materials Science · Physics 2023-02-09 Wooin Yang , Dowook Kim , Hyoung Kug Kim , Tae-Hwan Kim

Group-10 transition metal dichalcogenides (TMDs) are rising in prominence within the highly innovative field of 2D materials. While PtS2 has been investigated for potential electronic applications, due to its high charge-carrier mobility…

Colloidal materials of tin(II) sulfide (SnS), as a layered semiconductor with a narrow band gap, are emerging as a potential alternative to the more toxic metal chalcogenides (PbS, PbSe, CdS, CdSe) for various applications such as…

The structure of titanium films on \alpha - Al2O3(0001) surfaces at room temperature was investigated through in situ reflection high energy electron diffraction (RHEED). The \alpha-phase of titanium was observed to grow with the Ti(0001)…

Materials Science · Physics 2007-05-23 E. Sondergard , O. Kerjan , C. Barreteau , J. Jupille
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