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Spin relaxometry using fluorescent nanodiamonds (FNDs) has been applied successfully to sense numerous paramagnetic target molecules such as free radicals and metalloproteins. However, despite their high sensitivity, T1 spin relaxation…

Mesoscale and Nanoscale Physics · Physics 2026-02-23 Trent Ralph , Erin S. Grant , Lianne Lay , Sepehr Ahmadi , David A. Simpson

Currently, the primary applications of fluorescent nanodiamonds (FNDs) are in the area of biosensing, by using photoluminescence or spin properties of colour centres, mainly represented by the Nitrogen Vacancy (NV) point defect. The…

Mesoscale and Nanoscale Physics · Physics 2026-05-19 Jeroen Prooth , Michael Petrov , Alevtina Shmakova , Michal Gulka , Petr Cigler , Jan D'Haen , Hans-Gerd Boyen , Milos Nesladek

Probing electrical and magnetic properties in aqueous environments remains a frontier challenge in nanoscale sensing. Our inability to do so with quantitative accuracy imposes severe limitations, for example, on our understanding of the…

Fluorescent nanodiamonds (FNDs) relaxometry holds promising future for advancement of high spatiotemporal resolution metabolic imaging technology. In this study, we demonstrate a simultaneous integration of spatial position tracking with…

Biological Physics · Physics 2025-12-23 Jia Su , Linyu Zeng , Pengyu Chen , Zenghao Kong , Fazhan Shi

Understanding and controlling fluorescent nanodiamonds (FNDs) with optically read qubits is a key focus of research, as they show high potential for detecting electric and magnetic fields, temperature, and other physico-chemical quantities…

The nitrogen-vacancy (NV) center in diamond is a powerful and versatile quantum sensor for diverse quantities. In particular, relaxometry (or T1), allows to detect magnetic noise at the nanoscale. While increasing the number of NV centers…

The nitrogen-vacancy (NV) centers in nanodiamonds can be utilized as low-cost, highly versatile quantum sensors for studying surface properties in condensed matter physics through the application of relaxometry protocols. For such…

Mesoscale and Nanoscale Physics · Physics 2025-09-03 Izidor Benedičič , Yuri Tanuma , Žiga Gosar , Bastien Anézo , Mariusz Mrózek , Adam Wojciechowski , Denis Arčon

Optically accessible spin-active nanomaterials are promising as quantum nanosensors for probing biological samples. However, achieving bioimaging-level brightness and high-quality spin properties for these materials is challenging and…

Spin relaxometry based on quantum spin systems has developed as a valuable tool in medical and condensed matter systems, offering the advantage of operating without the need for external DC or RF fields. Spin relaxometry with…

Quantum Physics · Physics 2026-05-08 Ella P. Walsh , Sepehr Ahmadi , Alexander J. Healey , David A. Simpson , Liam T. Hall

We report an experimental study of the longitudinal relaxation time ($T_1$) of the electron spin associated with single nitrogen-vacancy (NV) defects hosted in nanodiamonds (ND). We first show that $T_1$ decreases over three orders of…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 J. -P. Tetienne , T. Hingant , L. Rondin , A. Cavailles , L. Mayer , G. Dantelle , T. Gacoin , J. Wrachtrup , J. -F. Roch , V. Jacques

We demonstrate a wide-band all-optical method of nanoscale magnetic resonance (MR) spectroscopy under ambient conditions. Our method relies on cross-relaxation between a probe spin, the electronic spin of a nitrogen-vacancy centre in…

Fluorescent nanodiamonds (fNDs) containing Nitrogen Vacancy (NV) centres are promising candidates for quantum sensing in biological environments. However, to date, there has been little progress made to combine the sensing capabilities of…

Applied Physics · Physics 2018-12-06 J. C. Price , S. J. Levett , V. Radu , D. A. Simpson , A. Mogas Barcons , C. F. Adams , M. L. Mather

We demonstrate fluorescence thermometry techniques with sensitivities approaching 10 mK Hz^(-1/2) based on the spin-dependent photoluminescence of nitrogen vacancy (NV) centers in diamond. These techniques use dynamical decoupling protocols…

Mesoscale and Nanoscale Physics · Physics 2013-05-24 David M. Toyli , Charles F. de las Casas , David J. Christle , Viatcheslav V. Dobrovitski , David D. Awschalom

Nanodiamonds (NDs) hosting nitrogen-vacancy (NV) centers are promising for applications of quantum sensing. Long spin relaxation times ($T_1$ and $T_2$) are critical for high sensitivity in quantum applications. It has been shown that…

Mesoscale and Nanoscale Physics · Physics 2020-08-11 Zaili Peng , Jax Dallas , Susumu Takahashi

Biocompatible nanoscale probes for sensitive detection of paramagnetic species and molecules associated with their (bio)chemical transformations would provide a desirable tool for a better understanding of cellular redox processes. Here, we…

To study the magnetic dynamics of superparamagnetic nanoparticles we use scanning probe relaxometry and dephasing of the nitrogen-vacancy (NV) center in diamond, characterizing the spin-noise of a single 10-nm magnetite particle.…

We report the experimental study of the temperature-dependence of the longitudinal spin relaxation time $T_1$ of single Nitrogen-Vacancy (NV) centers hosted in nanodiamonds. To determine the relaxation mechanisms at stake, measurements of…

Mesoscale and Nanoscale Physics · Physics 2020-11-04 Timothée de Guillebon , Baptiste Vindolet , Jean-François Roch , Vincent Jacques , Loïc Rondin

Magnetic resonance detection is one of the most important tools used in life-sciences today. However, as the technique detects the magnetization of large ensembles of spins it is fundamentally limited in spatial resolution to mesoscopic…

A single spin quantum sensor can quantitatively detect and image fluctuating electromagnetic fields via their effect on the sensor spin's relaxation time, thus revealing important information about the target solid-state or molecular…

Quantum Physics · Physics 2022-08-25 Zhiran Zhang , Maxime Joos , Dolev Bluvstein , Yuanqi Lyu , Ania C. Bleszynski Jayich

The negatively charged nitrogen-vacancy centre (NV$^-$) in diamond has been utilized in a wide variety of sensing applications. The centre's long spin coherence and relaxation times ($T_2^*$, $T_2$ and $T_1$) at room temperature are crucial…

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