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We introduce a matrix-product state based method to efficiently obtain dynamical response functions for two-dimensional microscopic Hamiltonians, which we apply to different phases of the Kitaev-Heisenberg model. We find significant broad…

Strongly Correlated Electrons · Physics 2017-10-18 Matthias Gohlke , Ruben Verresen , Roderich Moessner , Frank Pollmann

We study the non-equilibrium dynamics of dipoles confined in multiple stacked two-dimensional layers realising a long-range interacting quantum spin 1/2 XXZ model. We demonstrate that strong in-plane XXX interactions can protect a manifold…

Quantum Physics · Physics 2023-08-07 Thomas Bilitewski , Ana Maria Rey

As a nuclear spin model of scalable quantum register, the one-dimensional chain of the magnetic atoms with nuclear spins 1/2 substituting the basic atoms in the plate of nuclear spin free easy-axis 3D antiferromagnet is considered. It is…

Quantum Physics · Physics 2008-12-02 A. A. Kokin , V. A. Kokin

Recent interest in monolayer materials motivated a search for two-dimensional ferromagnets with sizable spin-orbit coupling. Magnetic anisotropy of exchange Hamiltonian, induced by spin-orbit coupling, may not only stabilize long-range…

Strongly Correlated Electrons · Physics 2025-08-08 Kaushal K. Kesharpu , Pavel A. Maksimov

We present a systematic derivation of effective lattice spin Hamiltonians derived from a rotationally invariant multi-orbital Hubbard model including a term ensuring Hund's rule coupling. The Hamiltonians are derived down-folding the…

Mesoscale and Nanoscale Physics · Physics 2020-01-29 Markus Hoffmann , Stefan Blügel

By means of density functional theory (DFT) calculations (with and without inclusion of spin-orbit (SO) coupling) we present a detailed study of the electronic structure and corresponding microscopic Hamiltonian parameters of Na2IrO3. In…

Strongly Correlated Electrons · Physics 2014-01-31 Kateryna Foyevtsova , Harald O. Jeschke , I. I. Mazin , D. I. Khomskii , Roser Valenti

We derive and study a spin one-half Hamiltonian on a honeycomb lattice describing the exchange interactions between Ir$^{4+}$ ions in a family of layered iridates $A_2$IrO$_3$ ($A$=Li,Na). Depending on the microscopic parameters, the…

Strongly Correlated Electrons · Physics 2014-11-20 Jiri Chaloupka , George Jackeli , Giniyat Khaliullin

An extension of the Heisenberg Hamiltonian is discussed, that allows to go beyond the standard bilinear spin Hamiltonian taking into account various contributions due to multispin interactions having both chiral and non-chiral character.…

Materials Science · Physics 2020-05-06 S. Mankovsky , S. Polesya , H. Ebert

Motivated by recent reports of a quantum disordered ground state in the triangular lattice compound NaRuO$_2$, we derive a $j_{\rm eff}=1/2$ magnetic model for this system by means of first-principles calculations. The pseudospin…

Motivated by recent neutron and x-ray observations in V$_2$O$_3$, we derive the effective Hamiltonian in the strong coupling limit of an Hubbard model with three degenerate t_{2g} states containing two electrons coupled to spin S = 1, and…

Strongly Correlated Electrons · Physics 2025-04-14 S. Di Matteo , N. B. Perkins , C. R. Natoli

Recently there has been a renewed interest in properties of the higher-spin Kitaev models, especially their low-dimensional analogues with additional interactions. These quasi-1D systems exhibit rich phase diagrams with symmetry-protected…

Strongly Correlated Electrons · Physics 2022-04-12 Jacob S. Gordon , Hae-Young Kee

Metastable states with surprising properties abound in Hilbert space. We study unfrustrated isotropic spin-\half Heisenberg models in honeycomb lattice and find emergence of \textit{metastable Kitaev spin liquids having a 2-spin nematic…

Strongly Correlated Electrons · Physics 2023-09-14 Ganapathy Baskaran

In the quest for materials hosting Kitaev spin liquids, much of the efforts have been focused on the fourth- and fifth-row transition metal compounds, which are spin-orbit coupling assisted Mott insulators. Here, we study the structural and…

Strongly Correlated Electrons · Physics 2022-12-20 Shishir Kumar Pandey , Ji Feng

Understanding magnetoelectric coupling in emerging van der Waals multiferroics is crucial for developing atomically thin spintronic devices. Here, we present a comprehensive first-principles investigation of magnetoelectric coupling in…

Materials Science · Physics 2026-03-06 Hui-Shi Yu , Xiao-Sheng Ni , Kun Cao

We performed inelastic neutron scattering experiments on single crystal samples of a linear magnetoelectric material Mn$_{3}$Ta$_{2}$O$_{8}$, which exhibits a collinear antiferromagnetic order, to reveal the spin dynamics. Numerous modes…

Strongly Correlated Electrons · Physics 2025-04-08 Hodaka Kikuchi , SHunsuke Hasegawa , Shinichiro Asai , Tao Hong , Kenta Kimura , Tsuyoshi Kimura , Shinichi Itoh , Takatsugu Masuda

We report a comprehensive inelastic neutron scattering study of the hybrid molecule-based multiferroic compound (ND4)2FeCl5D2O in the zero-field incommensurate cycloidal phase and the high-field quasi-collinear phase. The spontaneous…

Recently considerable excitement has arisen due to the experimental observation of a field-induced spin liquid phase in the compound $\alpha$-RuCl$_3$. However, the nature of this putative spin liquid phase and the relevant microscopic…

Strongly Correlated Electrons · Physics 2019-10-23 Yi-Fan Jiang , Thomas P. Devereaux , Hong-Chen Jiang

We explore the phase diagram of the Kitaev-Heisenberg model with nearest neighbor interactions on the honeycomb lattice using the exact diagonalization of finite systems combined with the cluster mean field approximation, and supplemented…

Strongly Correlated Electrons · Physics 2017-02-01 Dorota Gotfryd , Juraj Rusnačko , Krzysztof Wohlfeld , George Jackeli , Jiří Chaloupka , Andrzej M. Oleś

Nearly two decades ago, Alexei Kitaev proposed a model for spin-$1/2$ particles with bond-directional interactions on a two-dimensional honeycomb lattice which had the potential to host a quantum spin-liquid ground state. This work…

Materials Science · Physics 2022-01-19 Faranak Bahrami , Mykola Abramchuk , Oleg I. Lebedev , Fazel Tafti

The tetrameric Ni(II) spin cluster Ni4Mo12 has been studied by INS. The data were analyzed extensively in terms of a very general spin Hamiltonian, which includes antiferromagnetic Heisenberg interactions, biquadratic 2-spin and 3-spin…

Mesoscale and Nanoscale Physics · Physics 2010-06-11 J. Nehrkorn , M. Höck , M. Brüger , H. Mutka , J. Schnack , O. Waldmann