Related papers: Non-resonant Coherent Amplitude Transfer in Attose…
We study the nonlinear optical response of argon to a four-wave-mixing pulse sequence consisting of an extreme ultraviolet pulse, an overlapping collinear IR and an non-collinear delayed IR pulses. Absorption of an extreme ultraviolet and…
Ultracold Rb atoms were used to demonstrate non-degenerate four-wave mixing through a Rydberg state. Continuous 5S-5P-nD two-photon excitation to the Rydberg state was combined with an nD-6P tuned laser in a phase matched geometry. The…
Attosecond noncollinear four wave mixing spectroscopy with one attosecond extreme ultraviolet (XUV) pulse and two few-cycle near-infrared (NIR) pulses was used to measure the autoionization decay lifetimes of inner valence electronic…
In this study we analyze the transmission spectrum of a thin plate of Cuprous Oxide in the range of the absorption of the yellow exciton states with the coherent transfer matrix method. We demonstrate that, in contrast to the usual analysis…
A coherent vibrational wavepacket is launched and manipulated in the symmetric stretch (a$_1$) mode of CBr$_4$, by impulsive stimulated Raman scattering from non-resonant 400 nm laser pump pulses with various peak intensities on the order…
We report our measurements of the absolute transition frequencies of 5P_3/2,F = 3 to nS and nD Rydberg states of 87Rb with high principal quantum numbers in a wide range of values (n = 45-124). The measurements were performed using Rydberg…
We report the measurement of absolute excitation frequencies of 87Rb to nS and nD Rydberg states. The Rydberg transition frequencies are obtained by observing electromagnetically induced transparency on a rubidium vapor cell. The accuracy…
Rydberg atom-based radio frequency electromagnetic field sensors are drawing wide-spread interest because of their unique properties, such as small size, dielectric construction, and self-calibration. These photonic sensors use lasers to…
We present measurements on pulsed four-wave mixing involving a Rydberg state in an atomic vapor cell. The excitation to the Rydberg state is conducted by a pulsed two-photon excitation on the nanosecond timescale that is combined with a…
We experimentally investigate the nonlinear transmission spectrum of coherent light fields propagating through a Rydberg EIT medium with strong atomic interactions. In contrast to previous investigations, which have largely focused on…
We report on time-resolved pulsed four-wave mixing (FWM) signals in a thermal Rubidium vapor involving a Rydberg state. We observe FWM signals with dephasing times up to 7 ns, strongly dependent on the excitation bandwidth to the Rydberg…
Attosecond charge migration is a periodic evolution of the charge density of a molecule on a time scale defined by the energy intervals between the electronic states involved. Here, we report the observation of charge migration in neutral…
Pulsed laser excitation of a dense ultracold Cs vapor has been used to study the pairwise interactions between Cs atoms excited to $n$p$_{3/2}$ Rydberg states of principal quantum numbers in the range $n=22-36$. Molecular resonances were…
We report on the observation, characterization, and control of the electron dynamics in ionized argon atoms. We utilized an intense mid-infrared (MIR) pulse to create a coherent superposition of the spin-orbit split ground state of the ion.…
We realize a coherent transfer between a laser-accessible low-angular-momentum Rydberg state and the circular Rydberg level with maximal angular momentum. This transfer is induced by a radiofrequency field with a high-purity $\sigma^+$…
In recent years the interest in studying interactions of Rydberg atoms or ensembles thereof with optical and microwave frequency fields has steadily increased, both in the context of basic research and for potential applications in quantum…
Multi-photon dressing and interference in atomic systems is a key to several cutting edge technologies like Rydberg atom radio frequency sensors, clocks and magnetometers because it enables the engineering of atomic properties. Rydberg atom…
Exact and asymptotic lineshape expressions are derived from the semi-classical density matrix representation describing a set of closed three-level atomic or molecular states including decoherences, relaxation rates and light-shifts. An…
Coupling by the resonant dipole-dipole energy transfer between cold cesium Rydberg atoms is investigated using time-resolved narrow-band de-excitation spectroscopy. This technique combines the advantage of efficient Rydberg excitation with…
We propose a new technique to fully characterize the temporal structure of extreme ultraviolet pulses by ionizing a bound coherent electronic wavepacket. The populated energy levels make it possible to interfere different spectral…