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Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…

Mid-infrared high-resolution spectroscopy has proven an invaluable tool for the study of the structure and dynamics of molecules in the gas phase. The advent of frequency combs advances the frontiers of precise molecular spectroscopy. Here…

Optics · Physics 2019-02-28 Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué

Dual-comb spectroscopy utilizes two sets of comb lines with slightly different comb-tooth-spacings, and optical spectral information is acquired by measuring the radio-frequency beat notes between the sets of comb lines. It holds the…

Optics · Physics 2016-09-13 Xin Zhao , Guoqing Hu , Bofeng Zhao , Cui Li , Yingling Pan , Ya Liu , Takeshi Yasui , Zheng Zheng

Ultrafast optical frequency combs allow for both high spectral and temporal resolution in molecular spectroscopy and have become a powerful tool in many areas of chemistry and physics. Ultrafast lasers and frequency combs generated from…

Optics · Physics 2024-05-08 Jie Zhan , Nicholas D. Cooper , Melanie A. R. Reber

Spectroscopy has attracted much attention in molecular detection, biomolecular identification, and chemical analysis for providing accurate measurement. However, it is almost unable to distinguish different sources with overlapped…

Instrumentation and Detectors · Physics 2020-05-12 Ting Qing , Shupeng Li , Yijie Fang , Xiaohu Tang , Lihan Wang , Meihui Cao , Xinyu Li , Shilong Pan

We radically simplify coherently averaged dual-comb spectroscopy by introducing a real-time self-correction system: a radio frequency system-on-chip computes each incoming dual-comb interferogram's phase, frequency, and arrival time;…

Integrated femtosecond pulse and frequency comb sources are critical components for a wide range of applications. The leading approaches for on-chip pulse generation rely on mode locking inside microresonator with either third-order…

Repetition-rate-scanned lasers are practical in accordion frequency comb generation that serves as a variable gearbox connecting optical and radio wave domains. Rapid and wide-range scanned repetition rate can benefit versatile purposes,…

We report the generation of spectrally-tailored supercontinuum using Fourier-domain pulse shaping of femtosecond pulses injected into a highly nonlinear fiber controlled by a genetic algorithm. User-selectable spectral enhancement is…

Dual comb spectroscopy (DCS) is a powerful technique for broadband spectroscopy with high precision and fast data acquisition. High-frequency resolution requires long data acquisition times, limiting the temporal resolution in time-resolved…

Optics · Physics 2022-12-06 Sutapa Ghosh , Gadi Eisenstein

Dual-comb spectroscopy is extended to the visible spectral range with a set-up based on two frequency-doubled femtosecond ytterbium-doped fiber lasers. The dense rovibronic spectrum of iodine around 19240 cm-1 is recorded within 12 ms at…

Fourier-transform spectroscopy is an indispensable tool for analyzing chemical samples in scientific research as well as chemical and pharmaceutical industries. Recently, its measurement speed, sensitivity, and precision have been shown to…

Optics · Physics 2025-05-06 Takuro Ideguchi , Tasuku Nakamura , Yohei Kobayashi , Keisuke Goda

Optical frequency combs are laser sources which are capable of generating discrete, equal-spaced and highly coherent comb modes. Optical frequency comb technique provides a significant bridge to transfer the stability between optical…

Optics · Physics 2022-04-14 Haochen Tian

We have performed sub-Doppler spectroscopy on the narrow intercombination line of cold calcium atoms using the amplified output of a femtosecond laser frequency comb. Injection locking of a 657-nm diode laser with a femtosecond comb allows…

Atomic Physics · Physics 2010-03-19 T. M. Fortier , Y. Le Coq , J. E. Stalnaker , D. Ortega , S. A. Diddams , C. W. Oates , L. Hollberg

Improvements to dual-comb interferometers will benefit precision spectroscopy and sensing, distance metrology, tomography, telecommunications etc. A specific requirement of such interferometers is to enforce mutual coherence between the two…

Optics · Physics 2018-08-10 Zaijun Chen , Ming Yan , Theodor W. Hänsch , Nathalie Picqué

The major development recently undergone by quantum cascade lasers has effectively extended frequency comb emission to longer-wavelength spectral regions, i.e. the mid and far infrared. Unlike classical pulsed frequency combs, their…

Dual-comb lasers from which asynchronous ultrashort pulses can be simultaneously generated have recently become an interesting research subject. They could be an intriguing alternative to the current dual-laser optical-frequency-comb source…

Optics · Physics 2016-09-13 Ya Liu , Xin Zhao , Guoqing Hu , Cui Li , Bofeng Zhao , Zheng Zheng

Mid-infrared femtosecond optical frequency combs were produced by difference frequency generation of the spectral components of a near-infrared comb in a 3-mm-long MgO:PPLN crystal. We observe strong pump depletion and 9.3 dB parametric…

An optical fast-scan delay exploiting the near-collinear interaction between a train of ultrashort optical pulses and an acoustic wave propagating in a birefringent crystal is introduced. In combination with a femtosecond Er:fiber laser,…

Instrumentation and Detectors · Physics 2018-07-16 Olaf Schubert , Max Eisele , Vincent Crozatier , Nicolas Forget , Daniel Kaplan , Rupert Huber

A phase-stabilized femtosecond laser comb is directly used for high-resolution spectroscopy and absolute optical frequency measurements of one- and two-photon transitions in laser-cooled \rb atoms. Absolute atomic transition frequencies,…

Atomic Physics · Physics 2009-11-11 Adela Marian , Matthew C. Stowe , Daniel Felinto , Jun Ye