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In this work, we systematically investigate for the first time the nature of stress correlations in soft colloidal gel materials which support tensile and compressive forces as well as finite rolling torque, as a function of system…

Soft Condensed Matter · Physics 2023-08-09 Divas Singh Dagur , Chandana Mondal , Saikat Roy

Dispersed colloidal particles within a suspension can aggregate and spontaneously self-organize into a robust, percolating structure known as a gel. These network-like structures are prevalent in nature and play a critical role in many…

Soft Condensed Matter · Physics 2025-04-29 David Richard , Mehdi Bouzid

The compressive yield stress of particle gels shows a highly nonlinear dependence on the packing fraction. We have studied continuous compression processes, and discussed the packing fraction dependence with the particle scale…

Soft Condensed Matter · Physics 2013-11-22 Ryohei Seto , Robert Botet , Martine Meireles , Günter K. Auernhammer , Bernard Cabane

Colloidal dispersions are prized as model systems to understand basic properties of materials, and are central to a wide range of industries from cosmetics to foods to agrichemicals. Among the key developments in using colloids to address…

Soft Condensed Matter · Physics 2022-06-22 Jun Dong , Francesco Turci , Robert L. Jack , Malcolm A. Faers , C. Patrick Royall

We investigate the spatial correlations of microscopic stresses in soft particulate gels, using 2D and 3D numerical simulations. We use a recently developed theoretical framework predicting the analytical form of stress-stress correlations…

Soft Condensed Matter · Physics 2023-03-29 H. A. Vinutha , Fabiola Diaz Ruiz , Xiaoming Mao , Bulbul Chakraborty , Emanuela Del Gado

We exploit the controlled drying of millimeter-sized gel beads to investigate isotropic compression of colloidal fractal gels. Using a custom dynamic light scattering setup, we demonstrate that stresses imposed by drying on the bead surface…

Soft Condensed Matter · Physics 2026-01-22 M. Milani , E. Cavalletti , V. Ruzzi , A. Martinelli , P. Dieudonne-George , C. Ligoure , T. Phou , L. Cipelletti , L. Ramos

We use numerical simulations and an athermal quasi-static shear protocol to investigate the yielding of a model colloidal gel. Under increasing deformation, the elastic regime is followed by a significant stiffening before yielding takes…

Soft Condensed Matter · Physics 2015-06-22 Jader Colombo , Emanuela Del Gado

Soft particulate gels include materials we can eat, squeeze, or 3D print. From foods to bio-inks to cement hydrates, these gels are composed of a small amount of particulate matter (proteins, polymers, colloidal particles, or agglomerates…

Colloidal gel networks are disordered elastic solids that can form even in extremely dilute particle suspensions. With interaction strengths comparable to the thermal energy, their stress-bearing network can locally restructure via breaking…

Soft Condensed Matter · Physics 2014-06-18 Jader Colombo , Asaph Widmer-Cooper , Emanuela Del Gado

A liquid droplet resting on a soft gel substrate can deform that substrate to the point of material failure, whereby fractures develop on the gel surface that propagate outwards from the contact-line in a starburst pattern. In this paper,…

Soft Condensed Matter · Physics 2015-06-17 Joshua B. Bostwick , Karen E. Daniels

We examine the network of forces to be expected in a static assembly of hard, frictionless spherical beads of random sizes, such as a colloidal glass. Such an assembly is minimally connected: the ratio of constraint equations to contact…

Soft Condensed Matter · Physics 2009-10-31 Alexei V. Tkachenko , Thomas A. Witten

The behavior of microgels near surfaces and their adsorption is studied by simple scaling theory. Two different types of microgels can be studied, i.e., fractal type microgels and randomly crosslinked polymer chains. In the first case the…

Soft Condensed Matter · Physics 2009-10-31 Thomas A. Vilgis , Michael Stapper

Theoretical treatments of frictional granular matter often assume that it is legitimate to invoke classical elastic theory to describe its coarse-grained mechanical properties. Here we show, based on experiments and numerical simulations,…

Soft Condensed Matter · Physics 2021-02-24 Anaël Lemaître , Chandana Mondal , Itamar Procaccia , Saikat Roy , Yinqiao Wang , Jie Zhang

Many organisms have an elastic skeleton that consists of a closed shell of epithelial cells that is filled with fluid, and can actively regulate both elastic forces in the shell and hydrostatic pressure inside it. In this work we introduce…

Soft Condensed Matter · Physics 2023-10-13 Ajoy Maji , Yitzhak Rabin

Highly-deformable materials, from synthetic hydrogels to biological tissues, are becoming increasingly important from both fundamental and practical perspectives. Their mechanical behaviors, in particular the dynamics of crack propagation…

Materials Science · Physics 2015-06-09 Tamar Goldman Boué , Roi Harpaz , Jay Fineberg , Eran Bouchbinder

The consolidation of suspended particulate matter under external forces such as pressure or gravity is of widespread interest. In this work, we derive a constitutive relation to describe the deformation of a {\it two-dimensional} strongly…

Soft Condensed Matter · Physics 2014-02-26 Saikat Roy , Mahesh S Tirumkudulu

Microgels are soft colloidal particles that, when dispersed in a solvent, swell and deswell in response to changes in environmental conditions, such as temperature, concentration, and $p$H. Using Monte Carlo simulation, we model bulk…

Soft Condensed Matter · Physics 2016-11-10 Matthew Urich , Alan R. Denton

Colloidal gels consist of percolating networks of interconnected arms. Their mechanical properties depend on the individual arms, and on their collective behaviour. We use numerical simulations to pull on a single arm, built from a model…

Soft Condensed Matter · Physics 2023-01-31 Kristian Thijssen , T. B. Liverpool , C. Patrick Royall , Robert L. Jack

Hydrogels have had a profound impact in the fields of tissue engineering, drug delivery, and materials science as a whole. Due to the network architecture of these materials, imbibement with water often results in uniform swelling and…

Physically assembled gels have promising applications in many fields because of their tunable mechanical properties. Here, we report the mechanical properties as a function of polymer volume fraction ($\phi$) for a physical gel system…

Soft Condensed Matter · Physics 2020-03-31 Satish Mishra , Rosa Maria Badani Prado , Santanu Kundu
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