Related papers: Optical Activity of Solids from First Principles
Material anisotropy and chirality produce polarization-dependent light-matter interactions. Absorption leads to linear and circular dichroism, whereas elastic forward scattering produces linear and circular birefringence. Here we highlight…
We present two concepts of deformable mirror to compensate for first order optical aberrations. Deformation systems are designed using both elasticity theory and Finite Element Analysis in order to minimize the number of actuators. Starting…
There is current interest in developing photoactive materials that deform on illumination and can thus be used for photomechanical actuation. This is attractive since it can be affected at a distance, different frequencies can be used to…
A nonadiabatic scheme for the description of the coupled electron and nuclear motions in the ozone molecule was proposed recently. An initial coherent nonstationary state was prepared as a superposition of the ground state and the excited…
The nonrelativistic energies of the homonuclear ion T$_2^+$ are calculated for the ground state using the Lagrange-mesh method as was done for the isotopomers H$_2^+$ and D$_2^+$ ({\it J. Phys. B: At. Mol. Opt. Phys.} {\bf 45} 065101 and…
A method for evaluating finite trigonometric summations is applied to a system of N coupled oscillators under acceleration. Initial motion of the nth particle is shown to be of the order ${{T}^{2n+2}}$ for small time T and the end particle…
Four crystal classes are optically active yet not chiral (non-enantiomorphic). Corresponding Bragg diffraction patterns calculated for circularly polarized (helical) x-rays tuned to an atomic resonance prove that angular anisotropy in the…
The dynamic electric dipole polarizability function for the magnesium atom is formed by assembling the atomic electric dipole oscillator strength distribution from combinations of theoretical and experimental data for resonance oscillator…
Spheroidal fluid droplets immersed in another fluid and thermally fluctuating in the shape are considered. The polarizability of the droplet is evaluated up to the second order in the fluctuation amplitudes and also the previous first-order…
Accessing the ballistic regime of single particles in liquids remains an experimental challenge that shrouds our understanding of the particle-liquid interactions on exceedingly short time scales. We demonstrate the ballistic measurements…
The optical properties of nanoparticle clusters vary with the spatial arrangement of the constituent particles, but also the overall orientation of the cluster with respect to the incident light. This is particularly important in the…
The general formalism of the multipolar expansion of electrostatic interactions is applied to the calculation the potential energy between an excited atom (without fine structure) and a ground state diatomic molecule at large separations.…
In the mathematical modeling of nematic liquid crystals, a practical and physically reliable $\mathbf{Q}$-tensor model can be derived from Onsager's molecular model with the Bingham closure. However, this procedure leads to a singular…
In two meson photoproduction off a nucleon, for the case in which two of the three final state hadrons are products of the decay of an intermediate resonance, general expressions for its decay distribution and for polarization observables…
We study quantum dissipative effects due to the accelerated motion of a single, imperfect, zero-width mirror. It is assumed that the microscopic degrees of freedom on the mirror are confined to it, like in plasma or graphene sheets.…
Optical properties of materials related to light absorption and scattering are explained by the excitation of electrons. The Bethe-Salpeter equation is the state-of-the-art approach to describe these processes from first principles (ab…
We present all the periodic Green function dyadics that enter a description of a 2d array of emitters at the level that includes the electric dipole, magnetic dipole and electric quadrupole moment of each emitter. We find a concise analytic…
The light trajectory in the gravitational field of one body at rest with monopole and quadrupole structure is determined in the second post-Newtonian (2PN) approximation. The terms in the geodesic equation for light rays are separated into…
The light propagation in plasma medium around stationary gravitating objects is studied in the geometrical optics limit. Static metrics with quadrupole moments are considered, however, the main attention is paid to the stationary…
The dielectric properties of molecules or nanostructures are usually modified in a complex manner, when assembled into a condensed phase. We propose a first-principles method to compute polarizabilities of sub-entities of solids and…