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We characterize the coherent dynamics of a two-level quantum emitter driven by a pair of symmetrically-detuned phase-locked pulses. The promise of dichromatic excitation is to spectrally isolate the excitation laser from the quantum…

Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…

Atomic and Molecular Clusters · Physics 2009-03-31 Z. P. Wang , P. M. Dinh , P. -G. Reinhard , E. Suraud , F. S. Zhang

We study theoretically the effect of the giant resonance in Xe on the phase difference between the consecutive high order resonantly-enhanced harmonics and calculate the duration of the attosecond pulses produced by these harmonics. For…

Atomic Physics · Physics 2016-12-28 V. V. Strelkov

The use of bichromatic counter-rotating laser field is known to generate high-order harmonics with non-zero ellipticity. By combining such laser field with a plasmonic-enhanced spatially inhomogeneous field, we propose a way to influence…

We present a model for quasi-phase matching (QPM) in high-order harmonic generation (HHG). Using a one-dimensional description, we analyze the time-dependent, ultrafast wave-vector balance to calculate the on-axis harmonic output versus…

We predict high-order harmonics in which the polarization within the spectral bandwidth of each harmonic varies continuously and significantly. For example, the interaction of counter-rotating circularly-polarized bichromatic drivers having…

Optics · Physics 2014-10-24 Avner Fleischer , Ofer Kfir , Pavel Sidorenko , Oren Cohen

We study high-order harmonic generation (HHG) driven by seeded plasmonic-enhanced fields. On one hand, plasmonic-enhanced fields have shown a great potential to extend the HHG cutoff, an instrumental pre-requisite for the generation of…

Atomic Physics · Physics 2018-12-12 Irfana N. Ansari , M. S. Mrudul , Marcelo F. Ciappina , Maciej Lewenstein , Gopal Dixit

We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneities of the local electric field and the confinement of the electron motion…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , Srdjan S. Acimovic , T. Shaaran , J. Biegert , R. Quidant , M. Lewenstein

High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…

The bi-circular scheme for high harmonic generation, which combines two counter-rotating circular fields with frequency ratio 2:1, has recently permitted to generate high harmonics with essentially circular polarization, opening the way for…

Based on the dual-chirped optical parametric amplification and type-I BiB$_3$O$_6$(BiBO) crystals, the generation of $>$100 mJ, 10.4 fs, 10 Hz, carrier-to-envelope phase (CEP)-stable laser pulses, which are centered at 1.7 $\mu$m, is…

We report calculations of the high-order harmonic spectra of few-atomic clusters of two noble gases, helium and krypton, subjected to laser pulses of intensities above $10^{13}$ W/cm\textsuperscript{2}. We employ a fully \textit{ab intio}…

Chemical Physics · Physics 2023-12-05 Aleksander P. Woźniak , Robert Moszyński

We investigate a two-level atom in the field of a strong laser pulse. The resulting time-dependent polarization is the source of a radiation the frequency components of which are essentially harmonics of the driving field's carrier…

Quantum Physics · Physics 2016-09-13 Ákos Gombkötő , Attila Czirják , Sándor Varró , Péter Földi

The order of high harmonics emitted by an atom in an intense laser field is limited by the so-called cutoff frequency. Solving the time-dependent Schr\"odinger equation, we show that this frequency can be increased considerably by a…

Atomic Physics · Physics 2016-09-08 Carla Figueira de Morisson Faria , Jan-Michael Rost

We theoretically study the scaling with the driving wavelength of the high-order harmonic generation (HHG) under the simultaneous irradiation of an extreme ultraviolet (XUV) pulse. Surprisingly, when the cutoff energy and ionization yield…

Atomic Physics · Physics 2009-03-26 Kenichi L. Ishikawa , Eiji J. Takahashi , Katsumi Midorikawa

Wavelength scaling law for the yield of high-order harmonic emission is theoretically examined for excited state atoms which are optically prepared by simultaneously exposing to an extreme ultraviolet pulse at the resonant wavelength and an…

Atomic Physics · Physics 2015-05-13 Jing Chen , Ya Cheng , Zhizhan Xu

We produce oriented rotational wave packets in CO and measure their characteristics via high harmonic generation. The wavepacket is created using an intense, femtosecond laser pulse and its second harmonic. A delayed 800 nm pulse probes the…

High-order harmonic generation is investigated for H$_2^+$ and D$_2^+$ with and without Born-Oppenheimer approximation by numerical solution of full dimensional electronic time-dependent Schr\"{o}dinger equation under 4-cycle intense laser…

Atomic Physics · Physics 2014-10-22 Hamed Ahmadi , Ali Maghari , Hassan Sabzyan , Ali Reza Niknam , Mohsen Vafaee

High harmonic generation (HHG) is a crucial technology for compact, high-brightness extreme ultraviolet (XUV) and soft X-ray sources, which are key to advancing both fundamental and applied sciences. The availability of advanced driving…

Optics · Physics 2025-10-07 Robert Klas , Martin Gebhardt , Jan Rothhardt , Jens Limpert

We investigate high-order harmonic generation in ZnO driven by linearly polarized multi-color pulses. It is shown that the intensities of the harmonics in the plateau region can be enhanced by two to three orders of magnitude when driven by…

Computational Physics · Physics 2020-03-25 Xiaohong Song , Shidong Yang , Ruixin Zuo , Torsten Meier , Weifeng Yang