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We demonstrate one-dimensional Doppler cooling of a beam of buffer-gas cooled Barium monofluoride (BaF) molecules. The dependences of the cooling efficiency with the laser detuning, the bias filed and the laser intensity are carefully…

Atomic Physics · Physics 2022-03-23 Yuhe Zhang , Zixuan Zeng , Qian Liang , Wenhao Bu , Bo Yan

Cryogenic buffer gas cells have been a workhorse for the cooling of molecules in the last decades. The straightforward sympathetic cooling principle makes them applicable to a huge variety of different species. Notwithstanding this success,…

Chemical Physics · Physics 2020-08-26 Thomas Gantner , Manuel Koller , Xing Wu , Gerhard Rempe , Martin Zeppenfeld

Buffer gas cooling with a $^4$He gas is used to perform laser-absorption spectroscopy of the $^{12}$C$_2$H$_2$ ($\nu_1+\nu_3$) band at cryogenic temperatures. Doppler thermometry is first carried out to extract translational temperatures…

Instrumentation and Methods for Astrophysics · Physics 2015-06-23 L. Santamaria , V. Di Sarno , I. Ricciardi , M. De Rosa , S. Mosca , G. Santambrogio , P. Maddaloni , P. De Natale

We demonstrate Doppler-free saturated absorption spectroscopy of cold molecular radicals formed by laser ablation inside a cryogenic buffer gas cell. By lowering the temperature, congested regions of the spectrum can be simplified, and by…

We demonstrate optical cycling and sub-Doppler laser cooling of a cryogenic buffer-gas beam of calcium monohydride (CaH) molecules. We measure vibrational branching ratios for laser cooling transitions for both excited electronic states A…

Atomic Physics · Physics 2022-08-24 S. F. Vázquez-Carson , Q. Sun , J. Dai , D. Mitra , T. Zelevinsky

We report an experimental investigation on the Doppler-free saturated absorption spectroscopy of buffer-gas-cooled Barium monofluoride (BaF) molecules in a 4~K cryogenic cell. The obtained spectra with a resolution of 19~MHz, much smaller…

Atomic Physics · Physics 2023-02-14 Wenhao Bu , Yuhe Zhang , Qian Liang , Tao Chen , Bo Yan

We present a combined experimental and theoretical study of beam formation from a cryogenic buffer gas cell. Atoms and molecules are loaded into the cell by laser ablation of a target, and are cooled and swept out of the cell by a flow of…

Atomic Physics · Physics 2017-09-13 N. E. Bulleid , S. M. Skoff , R. J. Hendricks , B. E. Sauer , E. A. Hinds , M. R. Tarbutt

We present a comprehensive characterization of cold molecular beams from a cryogenic buffer-gas cell, providing an insight into the physics of buffer-gas cooling. Cold molecular beams are extracted from a cryogenic cell by electrostatic…

Chemical Physics · Physics 2018-12-04 X. Wu , T. Gantner , M. Zeppenfeld , S. Chervenkov , G. Rempe

We reported a detailed experimental study of the cold collision of Barium monofluoride (BaF) with buffer gas and the high-resolution spectroscopy relevant with direct laser cooling. BaF molecules are efficiently produced with laser ablation…

Atomic Physics · Physics 2017-03-22 Wenhao Bu , Tao Chen , Guitao Lv , Bo Yan

We demonstrate buffer gas cooling of carbon atoms to cryogenic temperatures. By employing pulsed two-photon excitation followed by vacuum ultraviolet fluorescence detection, we measured the arrival time distribution of the ablated carbon…

Atomic Physics · Physics 2024-07-15 Takashi Sakamoto , Kohei Suzuki , Kosuke Yoshioka

We demonstrate that buffer-gas cooling combined with laser ablation can be used to create coherent optical media with high optical depth and low Doppler broadening that offers metastable states with low collisional and motional decoherence.…

We study laser cooling of atomic gases by collisional redistribution of fluorescence. In a high pressure buffer gas regime, frequent collisions perturb the energy levels of alkali atoms, which allows for the absorption of a far red detuned…

We theoretically study prospects and limitations of a new route towards macroscopic scale laser refrigeration based on exciplex-mediated frequency up-conversion in gas filled hollow-core fibres. Using proven quantum optical rate equations…

Quantum Physics · Physics 2019-10-23 Christian Sommer , Nicolas Y. Joly , Helmut Ritsch , Claudiu Genes

A cryogenic buffer gas beam, an electrostatic hexapole lens, and 2D transverse Doppler laser cooling are combined to produce a bright beam of barium monofluoride ($^{138}$Ba$^{19}$F) molecules. Experimental results and trajectory…

A novel two-stage helium buffer gas cooled beam source is introduced. The properties of the molecular beams produced from this source are investigated theoretically using the CaF as a test molecule. The gas-phase molecules are first…

Atomic Physics · Physics 2020-04-14 Vijay Singh

Many predictions of Doppler cooling theory of two-level atoms have never been verified in a three-dimensional geometry, including the celebrated minimum achievable temperature $\hbar \Gamma/2 k_B$, where $\Gamma$ is the transition…

Barium monohydride (BaH) is an attractive candidate for extending laser cooling and trapping techniques to diatomic hydrides. The apparatus and high-resolution optical spectroscopy presented here demonstrate progress toward this goal. A…

Atomic Physics · Physics 2017-08-08 G. Z. Iwata , R. L. McNally , T. Zelevinsky

For experiments that require a quantum system to be in the ultra-cold regime, laser cooling is an essential tool. While techniques for laser cooling ions and neutral atoms have been refined and temperatures below the Doppler limit have been…

Atomic Physics · Physics 2024-10-31 Caleb Heuvel-Horwitz , S. F. Yelin

Employing a two-stage cryogenic buffer gas cell, we produce a cold, hydrodynamically extracted beam of calcium monohydride molecules with a near effusive velocity distribution. Beam dynamics, thermalization and slowing are studied using…

Atomic Physics · Physics 2017-09-13 Hsin-I Lu , Julia Rasmussen , Matthew J. Wright , Dave Patterson , John M. Doyle

The ability to cool atoms below the Doppler limit -- the minimum temperature reachable by Doppler cooling -- has been essential to most experiments with quantum degenerate gases, optical lattices and atomic fountains, among many other…

Atomic Physics · Physics 2018-01-17 S. Truppe , H. J. Williams , M. Hambach , L. Caldwell , N. J. Fitch , E. A. Hinds , B. E. Sauer , M. R. Tarbutt
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