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The accurate incorporation of nuclear quantum effects in large-scale molecular dynamics (MD) simulations remains a significant challenge. Recently, we combined constrained nuclear-electronic orbital (CNEO) theory with classical MD and…

Chemical Physics · Physics 2023-01-11 Zehua Chen , Yang Yang

Quantum simulation holds the promise of improving the atomic simulations used at EDF to anticipate the ageing of materials of interest. One simulator in particular seems well suited to modeling interacting electrons: the Rydberg atoms…

Quantum Physics · Physics 2024-06-21 Antoine Michel

We propose a framework for simulating the real-time dynamics of quantum field theories (QFTs) using continuous-variable quantum computing (CVQC). Focusing on ($1+1$)-dimensional $\varphi^4$ scalar field theory, the approach employs the…

Quantum Physics · Physics 2025-09-03 Steven Abel , Michael Spannowsky , Simon Williams

We present here the first-principles dynamical CPA (coherent potential approximation) combined with the tight-binding LMTO LDA+U method towards quantitative calculations of the electronic structure and magnetism at finite temperatures in…

Strongly Correlated Electrons · Physics 2015-05-14 Y. Kakehashi , T. Tamashiro , M. A. R. Patoary , T. Nakamura

The quantum many-body problem in condensed phases is often simplified using a quasiparticle description, such as effective mass theory for electron motion in a periodic solid. These approaches are often the basis for understanding many…

Statistical Mechanics · Physics 2020-10-28 Richard C. Remsing , Jefferson E. Bates

QCD at finite temperature and density is becoming increasingly important for various experimental programmes, ranging from heavy ion physics to astro-particle physics. The non-perturbative nature of non-abelian quantum field theories at…

High Energy Physics - Lattice · Physics 2009-11-02 Owe Philipsen

Solid-state molecular qubits with open-shell ground states have great potential for addressability, scalability, and tunability, but understanding the fundamental limits of quantum coherence in these systems is challenging due to the…

Quantum Physics · Physics 2026-04-01 Katy Aruachan , Sanoj Raj , Yamil J. Colón , Daniel Aravena , Felipe Herrera

We present a comprehensive end-to-end framework for simulating the real-time dynamics of chemical systems on a fault-tolerant quantum computer, incorporating both electronic and nuclear quantum degrees of freedom. An all-particle simulation…

Atomistic spin dynamics (ASD) is a standard tool to model the magnetization dynamics of a variety of materials. The fundamental dynamical model underlying ASD is entirely classical. In this paper, we present two approaches to effectively…

Materials Science · Physics 2024-07-01 Marco Berritta , Stefano Scali , Federico Cerisola , Janet Anders

A quantum unitary evolution alternated with measurements is simulated by a bubble filled with fictitious particles called amplitude quanta that move chaotically and can be transformed by the simple rules that look like chemical reactions. A…

Quantum Physics · Physics 2016-09-08 Yuri Ozhigov

Quantum criticality is a fundamental organizing principle for studying strongly correlated systems. Nevertheless, understanding quantum critical dynamics at nonzero temperatures is a major challenge of condensed matter physics due to the…

Strongly Correlated Electrons · Physics 2018-06-19 Jianda Wu , Wang Yang , Congjun Wu , Qimiao Si

The problem of simulating the thermal behavior of quantum systems remains a central open challenge in quantum computing. Unlike well-established quantum algorithms for unitary dynamics, \emph{provably efficient} algorithms for preparing…

Quantum Physics · Physics 2026-05-14 Dominik Hahn , Ryan Sweke , Abhinav Deshpande , Oles Shtanko

We introduce a quantum information theory-inspired method to improve the characterization of many-body Hamiltonians on near-term quantum devices. We design a new class of similarity transformations that, when applied as a preprocessing…

Quantum Physics · Physics 2024-07-24 Andi Gu , Hong-Ye Hu , Di Luo , Taylor L. Patti , Nicholas C. Rubin , Susanne F. Yelin

Path integral molecular dynamics simulations, combined with an ab initio evaluation of interactions using electronic structure theory, incorporate the quantum mechanical nature of both the electrons and nuclei, which are essential to…

Chemical Physics · Physics 2016-02-15 Ondrej Marsalek , Thomas E. Markland

We investigate whether making the friction spatially dependent on the reaction coordinate introduces quantum effects into the thermal reaction rates for dissipative reactions. Quantum rates are calculated using the numerically exact…

The fundamental question of how to best simulate quantum systems using conventional computational resources lies at the forefront of condensed matter and quantum computation. It impacts both our understanding of quantum materials and our…

Strongly Correlated Electrons · Physics 2021-09-29 Juan Carrasquilla , Di Luo , Felipe Pérez , Ashley Milsted , Bryan K. Clark , Maksims Volkovs , Leandro Aolita

We present a detailed description of semi-quantum molecular dynamics simulation of stochastic dynamics of a system of interacting particles. Within this approach, the dynamics of the system is described with the use of classical Newtonian…

Computational Physics · Physics 2015-06-03 Alexander V. Savin , Yuriy A. Kosevich , Andres Cantarero

The quantum loop and dimer models are archetypal correlated systems with local constraints. With natural foundations in statistical mechanics, they are of direct relevance to various important physical concepts and systems, such as…

Strongly Correlated Electrons · Physics 2025-11-26 Xiaoxue Ran , Sylvain Capponi , Junchen Rong , Fabien Alet , Zi Yang Meng

We present a holographic quantum simulation algorithm to variationally prepare thermal states of $d$-dimensional interacting quantum many-body systems, using only enough hardware qubits to represent a ($d$-1)-dimensional cross-section. This…

Quantum Physics · Physics 2022-10-17 Yuxuan Zhang , Shahin Jahanbani , Daoheng Niu , Reza Haghshenas , Andrew C. Potter

It is widely anticipated that a large-scale quantum computer will offer an evermore accurate simulation of nature, opening the floodgates for exciting scientific breakthroughs and technological innovations. Here, we show a complete,…

Quantum Physics · Physics 2022-01-27 Angus Kan , Yunseong Nam