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We develop a microscopic theory describing a quantum impurity whose rotational degree of freedom is coupled to a many-particle bath. We approach the problem by introducing the concept of an 'angulon' - a quantum rotor dressed by a quantum…

Quantum Gases · Physics 2015-05-27 Richard Schmidt , Mikhail Lemeshko

Recently it was shown that an impurity exchanging orbital angular momentum with a surrounding bath can be described in terms of the angulon quasiparticle [Phys. Rev. Lett. 118, 095301 (2017)]. The angulon consists of a quantum rotor dressed…

Quantum Gases · Physics 2017-08-11 Giacomo Bighin , Mikhail Lemeshko

The formation of angulon, stemming from the rotor (molecule or impurity) rotating in the quantum many-body field, adds a new member in the quasiparticle's family and has aroused intensively interests in multiple research fields. However,…

Mesoscale and Nanoscale Physics · Physics 2023-05-08 Yi-Yan Liu , Yu Cui , Xiao-Zhe Zhang , Ran-Bo Yang , Zhi-Qing Li , Zi-Wu Wang

Understanding the behavior of molecules interacting with superfluid helium represents a formidable challenge and, in general, requires approaches relying on large-scale numerical simulations. Here we demonstrate that experimental data…

Chemical Physics · Physics 2017-03-08 Mikhail Lemeshko

In several settings of physics and chemistry one has to deal with molecules interacting with some kind of an external environment, be it a gas, a solution, or a crystal surface. Understanding molecular processes in the presence of such a…

Quantum Gases · Physics 2017-04-06 Mikhail Lemeshko , Richard Schmidt

Problems involving quantum impurities, in which one or a few particles are interacting with a macroscopic environment, represent a pervasive paradigm, spanning across atomic, molecular, and condensed-matter physics. In this paper we…

Mesoscale and Nanoscale Physics · Physics 2019-01-31 Xiang Li , Giacomo Bighin , Enderalp Yakaboylu , Mikhail Lemeshko

Inspired by the possibility to experimentally manipulate and enhance chemical reactivity in helium nanodroplets, we investigate the effective interaction and the resulting correlations between two diatomic molecules immersed in a bath of…

Mesoscale and Nanoscale Physics · Physics 2025-05-08 Xiang Li , Enderalp Yakaboylu , Giacomo Bighin , Richard Schmidt , Mikhail Lemeshko , Andreas Deuchert

We investigate the in- and out-of-equilibrium phenomena of a rotational impurity -- specifically, a linear molecule -- coupled to a nonconventional environment, a helium nanodroplet. By employing a Lee-Low-Pines-like transformation combined…

Quantum Gases · Physics 2025-04-23 Wei Zhang , Zhongda Zeng , Tao Shi

Recently it was shown that a molecule rotating in a quantum solvent can be described in terms of the `angulon' quasiparticle [Phys. Rev. Lett. 118, 095301 (2017)]. Here we extend the angulon theory to the case of molecules possessing an…

Chemical Physics · Physics 2018-03-16 Wojciech Rzadkowski , Mikhail Lemeshko

Impurity motion in a many-body environment has been a central issue in the field of low-temperature physics for decades. In bosonic quantum fluids, the onset of a drag force experienced by point-like objects is due to collective environment…

Quantum Gases · Physics 2025-03-19 Alberto Cappellaro , Giacomo Bighin , Igor Cherepanov , Mikhail Lemeshko

Recently it was shown that molecules rotating in superfluid helium can be described in terms of the angulon quasiparticles (Phys. Rev. Lett. 118, 095301 (2017)). Here we demonstrate that in the experimentally realized regime the angulon can…

Quantum Gases · Physics 2017-12-13 Enderalp Yakaboylu , Andreas Deuchert , Mikhail Lemeshko

The formation of vortices is usually considered to be the main mechanism of angular momentum disposal in superfluids. Recently, it was predicted that a superfluid can acquire angular momentum via an alternative, microscopic route -- namely,…

Chemical Physics · Physics 2017-08-16 Igor N. Cherepanov , Mikhail Lemeshko

The existence of a self-localization transition in the polaron problem has been under an active debate ever since Landau suggested it 83 years ago. Here we reveal the self-localization transition for the rotational analogue of the polaron…

Quantum Gases · Physics 2017-03-13 Xiang Li , Robert Seiringer , Mikhail Lemeshko

During the last 70 years, the quantum theory of angular momentum has been successfully applied to describing the properties of nuclei, atoms, and molecules, their interactions with each other as well as with external fields. Due to the…

Quantum Gases · Physics 2016-02-17 Richard Schmidt , Mikhail Lemeshko

We study a quantum impurity possessing both translational and internal rotational degrees of freedom interacting with a bosonic bath. Such a system corresponds to a `rotating polaron', which can be used to model, e.g., a rotating molecule…

The elementary excitations of a fractional quantum Hall liquid are quasiparticles or quasiholes which are neither bosons nor fermions, but so-called anyons. Here we study impurity particles immersed in a quantum Hall liquid which bind to…

Mesoscale and Nanoscale Physics · Physics 2020-09-30 Tobias Graß , Bruno Juliá-Díaz , Niccolò Baldelli , Utso Bhattacharya , Maciej Lewenstein

We study a linear rotor in a bosonic bath within the angulon formalism. Our focus is on systems where isotropic or anisotropic impurity-boson interactions support a shallow bound state. To study the fate of the angulon in the vicinity of…

We use laser-induced rotation of single molecules embedded in superfluid helium nanodroplets to reveal angular momentum dynamics and transfer in a controlled setting, under far-from-equilibrium conditions. As an unexpected result, we…

We study a polar molecule immersed into a superfluid environment, such as a helium nanodroplet or a Bose-Einstein condensate, in the presence of an intense electrostatic field. We show that coupling of the molecular pendular motion, induced…

Atomic Physics · Physics 2016-09-30 E. S. Redchenko , Mikhail Lemeshko

The quantum rotor represents, after the harmonic oscillator, the next obvious quantum system to study the complementary pair of variables: the angular momentum and the unitary shift operator in angular momentum. Proper quantification of…

Quantum Physics · Physics 2024-08-13 Ladislav Mišta , Matouš Mišta , Zdeněk Hradil
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