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Related papers: Enantiomer detection via Quantum Otto cycle

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Sculpting sub-cycle temporal structures of optical waveforms allows one to image and even control electronic clouds in atoms, molecules and solids. Here we show how the transverse spin component arising upon spatial confinement of such…

Optics · Physics 2020-11-17 David Ayuso , Andres Ordonez , Misha Ivanov , Olga Smirnova

State-selective enantiomeric excess is realized using microwave-driven coherent population transfer. The method selectively promotes either R or S molecules to a higher rotational state by phase-controlled microwave pulses that drive…

Chemical Physics · Physics 2017-03-23 Sandra Eibenberger , John Doyle , David Patterson

We propose employing a quantum heat engine as a sensitive probe for thermal baths. In particular, we study a single-atom Otto engine operating in an open thermodynamic cycle. Owing to its cyclic nature, the engine is capable of translating…

Quantum Physics · Physics 2020-05-15 Amikam Levy , Moritz Göb , Bo Deng , Kilian Singer , E. Torrontegui , Daqing Wang

Optical forces can be chiral when they exhibit opposite signs for the two enantiomeric versions of a chiral molecule or particle. Such forces could be eventually used to separate enantiomers, which could find application in numerous…

We propose and experimentally demonstrate that a Mach-Zehnder interferometer composed of polarized beam splitters and a pentaprism in the place of one of the mirrors works as a linear optical quantum controlled-NOT (CNOT) gate. To perform…

Quantum Physics · Physics 2018-07-18 J. H. Lopes , W. C. Soares , B. L. Bernardo , D. P. Caetano , Askery Canabarro

We present a practical roadmap to achieve optical cycling and laser cooling of asymmetric top molecules (ATMs). Our theoretical analysis describes how reduced molecular symmetry, as compared to diatomic and symmetric non-linear molecules,…

Atomic Physics · Physics 2020-08-05 Benjamin L. Augenbraun , John M. Doyle , Tanya Zelevinsky , Ivan Kozyryev

Geometrical chirality is a universal property encountered on very different length scales ranging from geometrical shapes of living organisms to protein and DNA molecules. Interaction of chiral matter with chiral light - that is,…

Coherent interconversion between optical and mechanical excitations in an optomechanical cavity can be used to engineer a quantum heat engine. This heat engine is based on an Otto cycle between a cold photonic reservoir and a hot phononic…

Quantum Physics · Physics 2014-08-14 Keye Zhang , Francesco Bariani , Pierre Meystre

A quantum Otto engine based on a three-dimensional harmonic oscillator is proposed. One of the modes of this oscillator functions as the working fluid, while the other two play the role of baths. The coupling between the working fluid and…

Quantum Physics · Physics 2023-12-07 Aleksandr Rodin

The principle that heat spontaneously flows from higher temperature to lower temperature is a cornerstone of classical thermodynamics, often assumed to be independent of the sequence of interactions. While this holds true for macroscopic…

The measurement of circular dichroism (CD) has widely been exploited to distinguish the different enantiomers of chiral structures. It has been applied to natural materials (e.g. molecules) as well as to artificial materials (e.g.…

We present a comprehensive theoretical investigation about the operational regions of quantum systems, specifically examining their roles as working media functioning between two thermal reservoirs in Quantum Thermal Machines (QTMs). This…

Quantum Physics · Physics 2025-07-03 Aline D. Lucio , Cleverson Filgueiras , Moises Rojas

Enantiomer-specific state transfer (ESST), which involves transferring enantiomers with different handedness of a chiral molecule into different-energy internal states, is a challenging yet significant task. Previous ESST methods are based…

Quantum Physics · Physics 2024-10-30 Fen Zou , Yong Li , Peng Zhang

Based on the four-level double-$\Delta$ model composed of two degenerated (left- and right-handed) chiral ground states and two achiral excited states, we propose a purely optical method for enantio-conversion of chiral mixture. By choosing…

Optics · Physics 2020-08-05 Chong Ye , Quansheng Zhang , Yu-Yuan Chen , Yong Li

Is it possible to infer the time evolving quantum state of a multichromophoric system from a sequence of two-dimensional electronic spectra (2D-ES) as a function of waiting time? Here we provide a positive answer for a tractable model…

Quantum Physics · Physics 2015-05-27 Joel Yuen-Zhou , Alán Aspuru-Guzik

The reactor antineutrino anomaly, discovered in 2011, means a noticeable difference between the observed rate of inverse beta decays and the expected (theoretical) rate of such processes based on the measurement of the spectra of electrons…

High Energy Physics - Phenomenology · Physics 2025-04-16 L. M. Slad

Metasurfaces are believed as one of the best candidates in nano-optical devices, attributed to the key feasible modulation features of phase, polarization, and local field enhancement by structural designing. However, current methods of…

Optics · Physics 2022-02-22 Renchao Jin , Lin Deng , Lili Tang , Yue Cao , Yongmin Liu , Zheng-Gao Dong

X-ray as well as electron diffraction are powerful tools for structure determination of molecules. Studies on randomly oriented molecules in the gas-phase address cases in which molecular crystals cannot be generated or the interaction-free…

Enantioselective photochemistry provides access to unique molecular structures and functions, with deep implications for fundamental science and industrial applications. Current methods for highly enantioselective photochemistry critically…

Chemical Physics · Physics 2025-03-07 Andrés Ordóñez , Patricia Vindel-Zandbergen , David Ayuso

A quantum thermal machine is an open quantum system coupled to hot and cold thermal baths. Thus, its dynamics can be well understood using the concepts and tools from non-Hermitian quantum systems. A hallmark of non-Hermiticity is the…

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