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The interplay of polarization and magnetism in materials with light can create rich nonlinear magneto-optical (NLMO) effects, and the recent discovery of two-dimensional (2D) van der Waals magnets provides remarkable control over NLMO…

Materials Science · Physics 2024-04-30 Dezhao Wu , Meng Ye , Haowei Chen , Yong Xu , Wenhui Duan

Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…

Mesoscale and Nanoscale Physics · Physics 2020-07-03 E. A. Stepanov , S. V. Semin , C. R. Woods , M. Vandelli , A. V. Kimel , K. S. Novoselov , M. I. Katsnelson

Optical second harmonic generation (SHG) has been measured for the first time in reflection from the nanometer-thick films (6 to 40 nm) of the topological insulator Bi2Se3 using 1.51 eV (820 nm) Ti:Sapphire laser photons and revealed a…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Yuri D. Glinka , Sercan Babakiray , Trent A. Johnson , Mikel B. Holcomb , David Lederman

Second harmonic generation (SHG) is a fundamental nonlinear optical phenomenon widely used both for experimental probes of materials and for application to optical devices. Even-order nonlinear optical responses including SHG generally…

Mesoscale and Nanoscale Physics · Physics 2021-10-13 Kazuaki Takasan , Takahiro Morimoto , Joseph Orenstein , Joel E. Moore

Second-order nonlinear optical materials enable frequency doubling of light (second-harmonic generation, SHG), which is essential for optoelectronic applications ranging from materials characterization to quantum technologies. However,…

Materials Science · Physics 2026-03-25 Aubrey G. J. Nyiri , Michael J. Waters , James M. Rondinelli

Spectroscopy of the centrosymmetric magnetic semiconductors EuTe and EuSe reveals spin-induced optical second harmonic generation (SHG) in the band gap vicinity at 2.1-2.4eV. The magnetic field and temperature dependence demonstrates that…

The notion of spontaneous symmetry breaking has been used to describe phase transitions in a variety of physical systems. In crystalline solids, the breaking of certain symmetries, such as mirror symmetry, is difficult to detect…

Materials Science · Physics 2020-07-01 Bryan T. Fichera , Anshul Kogar , Linda Ye , Bilal Gökce , Alfred Zong , Joseph G. Checkelsky , Nuh Gedik

Second-harmonic generation (SHG) is a fundamental nonlinear optical process widely used in photonics; however, it is strictly forbidden in the bulk of centrosymmetric materials due to their inversion symmetry. Nevertheless, applying an…

We have studied on optical second harmonic generations (SHGs) from atomically thin MoTe2 flakes with 2H and 1T' phases. From 2H-MoTe2 samples with odd (even) numbers of layers, strong (negligible) SHGs are observed due to the…

Optics · Physics 2018-05-25 Yu Song , Ruijuan Tian , Jiulong Yang , Rui Yin , Jianlin Zhao , Xuetao Gan

We study the second harmonic generation (SHG) in a suspension of small spherical particles confined within a slab, assuming undepleted pump and applying (i) single scattering approximation and (ii) diffusion approximation. In the case (i),…

Optics · Physics 2007-05-23 E. V. Makeev , S. E. Skipetrov

Second-harmonic generation (SHG) has emerged as a promising tool for detecting electronic and magnetic structures in noncentrosymmetric materials, but 100$\%$ spin-polarized SHG has not been reported. In this work, we demonstrate nearly…

Materials Science · Physics 2023-09-06 Y. Q. Liu , M. S. Si , G. P. Zhang

We demonstrate phase-matched second-harmonic generation (SHG) from three-dimensional metamaterials consisting of stacked metasurfaces. To achieve phase matching, we utilize a novel mechanism based on phase engineering of the metasurfaces at…

Optical second harmonic generation is a second-order nonlinear process that combines two photons of a given frequency into a third photon at twice the frequency. Due to the symmetry constraints, it is widely used as a sensitive probe to…

We present an analytical theory of second harmonic generation (SHG) in hybrid structures combining a nonlinear 2D crystal with a dielectric metasurface waveguide. The theory describes the excitation spectrum and enhancement of SHG at both…

Optics · Physics 2025-11-07 Egor S. Vyatkin , Sergey A. Tarasenko

Spectroscopic magnetization induced optical Second Harmonic Generation (MSHG) measurements from a clean Ni(110) surface reveal strong resonance effects near 2.7 eV that can be attributed to the presence of an empty surface state. The good…

Materials Science · Physics 2009-10-31 K. J. Veenstra , A. V. Petukhov , E. Jurdik , Th. Rasing

The anisotropic dispersion and inherent nonlinearity of magnetostatic spin waves in thin films and confined structures provide unique opportunities for implementation in next-generation magnonic devices for data and signal processing. A…

Materials Science · Physics 2026-05-19 Stephanie R. Lake , Marc Eger , Philipp Geyer , Rouven Dreyer , Seth W. Kurfman , Georg Schmidt

The generation process of second harmonic (SH) radiation from holes periodically arranged on a metal surface is investigated. Three main modulating factors affecting the optical response are identified: the near-field distribution at the…

Mesoscale and Nanoscale Physics · Physics 2015-01-08 Sergio G. Rodrigo , V. Laliena , L. Martín-Moreno

The half-Heusler compound GdBiPt orders antiferromagnetically around $T_\mathrm{N}=8.5$ K which implies breaking the time reversal symmetry as well as the translational symmetry. This combination preserves the global symmetry. Here, we used…

Materials Science · Physics 2024-10-02 Simon Daneau , Richard Leonelli , Andrea D. Bianchi

The origin of the second harmonic generation (SHG) from plasmonic structures remains a subject of debate. Here, we investigate SHG from gold plasmonic nanostructures by scanning nanostructures at the single-particle level to acquire…

Integrating 2D materials onto on-chip photonic devices holds significant potential for nonlinear frequency conversion across various applications. The lack of inversion symmetry in monolayers of transition metal dichalcogenides (TMDs),…

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