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We develop a generalized Ginzburg-Landau theory for second harmonic generation (SHG) in magnets by expanding the free energy in terms of the order parameter in the magnetic phase and the susceptibility tensor in the corresponding…

Condensed Matter · Physics 2016-08-31 Debanand Sa , R. Valenti , C. Gros

We report on the experimental and theoretical investigation of magnetic-field-induced second harmonic generation (SHG) and two-photon absorption (TPA) of excited exciton states ($n \geq 3$) of the yellow series in Cu$_2$O. In this…

Mesoscale and Nanoscale Physics · Physics 2020-04-01 A. Farenbruch , J. Mund , D. Fröhlich , D. R. Yakovlev , M. Bayer , M. A. Semina , M. M. Glazov

We theoretically investigate the second harmonic generation (SHG) of topological insulator surface states in a perpendicular magnetic field. Our theory is based on the microscopic expression of the second-order magneto-optical conductivity…

Mesoscale and Nanoscale Physics · Physics 2024-11-27 Kainan Chang , Muhammad Zubair , Jin Luo Cheng , Wang-Kong Tse

A comprehensive analysis of optical second harmonic generation (SHG) on an incommensurate (IC) magnetically ordered state is presented using multiferroic MnWO4 as model compound. Two fundamentally different SHG contributions coupling to the…

Strongly Correlated Electrons · Physics 2012-08-08 D. Meier , N. Leo , G. Yuan , Th. Lottermoser , P. Becker , L. Bohaty , M. Fiebig

We study the effective second-harmonic generation (SHG) susceptibility in graded metallic films by invoking the local field effects exactly, and further numerically demonstrate that the graded metallic films can serve as a novel optical…

Optics · Physics 2009-11-10 J. P. Huang , K. W. Yu

Second harmonic generation (SHG) is a powerful optical tool for identifying non-centrosymmetric crystalline structures. Here, we analyze SHG in multilayer graphenes (MLG), with a focus on its dependence on the stacking order, encapsulation…

Mesoscale and Nanoscale Physics · Physics 2026-03-25 Patrick Johansen Sarsfield , Takaaki V. Joya , Takuto Kawakami , Mikito Koshino , Vladimir Fal'ko

Magnetic materials have been applied in a large variety of technologies, from data storage to quantum devices. The development of 2D materials has opened new arenas for magnetic compounds, even when classical theories discourage their…

Materials Science · Physics 2022-02-11 Carlos Mera Acosta , Elton Ogoshi , Jose Antonio Souza , Gustavo M. Dalpian

Although second harmonic generation (SHG) is a promising and widely used method recently for studying 2D magnetic materials, the quantitative analysis of the full SHG tensor is currently challenging. In this letter, we describe a…

Strongly Correlated Electrons · Physics 2026-02-04 Banasree S. Mou , Stephen M. Winter

Magnetism has witnessed remarkable progress in recent decades, largely driven by its potential for next-generation storage devices. However, the classification of magnetic orders, even for fundamental concepts such as ferromagnetism and…

Materials Science · Physics 2026-04-24 Yuntian Liu , Xiaobing Chen , Yutong Yu , Jesús Etxebarria , J. Manuel Perez-Mato , Qihang Liu

Using symmetry arguments we show how optical second harmonic generation (SHG) can be used to detect antiferromagnetism at surfaces and in thin films. Based on the group theoretical analysis of the nonlinear electric susceptibility we…

Condensed Matter · Physics 2007-05-23 A. Daehn , W. Huebner , K. H. Bennemann

We conduct a theoretical and numerical study on the second-harmonic (SH) optical response of a nano-structured metamaterial composed of a periodic array of inclusions. Both the inclusions and their surrounding matrix are made of…

Mesoscale and Nanoscale Physics · Physics 2019-03-13 Ulises R. Meza , Bernardo S. Mendoza , W. Luis Mochán

Second harmonic generation (SHG) is forbidden in centrosymmetric molecular materials. However, a signal is frequently observed from interfaces where the symmetry is broken. Whereas the effect can be phenomenologically accommodated, an ab…

Surfaces and interfaces of magnetic nanostructures can reveal rather interesting and unusual properties that differ substantially from those of bulky materials. Here we apply the surface-sensitive method of optical second harmonic…

Mesoscale and Nanoscale Physics · Physics 2018-12-13 T. V. Murzina , K. A. Lazareva , E. E. Shalygina , I. A. Kolmychek , E. A. Karashtin , N. S. Gusev , A. A. Fraerman

The recent discovery of two-dimensional (2D) magnets offers unique opportunities for the experimental exploration of low-dimensional magnetism4 and the magnetic proximity effects, and for the development of novel magnetoelectric,…

The effective second-harmonic generation (SHG) coefficient is a crucial data that quantifies the efficiency of transforming fundamental frequency light into its second harmonic. With the help of the symmetry of nonlinear optical…

Optimization and Control · Mathematics 2026-02-24 Die Xiao , Yisheng Song

The interplay between magnetism and light can create abundant optical phenomena. Here, we demonstrate the emergence of an unconventional magnetization-induced second-harmonic generation (MSHG) stemming from vector spin chirality, denoted as…

Materials Science · Physics 2025-04-08 Dezhao Wu , Yong Xu , Meng Ye , Wenhui Duan

A comparative experimental investigation of the dependence of second harmonic generation (SHG) on applied external voltage between the standard nematic liquid crystalline material and an analogue ferromagnetic nematic liquid crystalline…

Soft Condensed Matter · Physics 2019-09-30 Jure Brence , Luka Cmok , Nerea Sebastian , Alenka Mertelj , Darja Lisjak , Irena Drevensek-Olenik

We report on the optical second harmonic generation (SHG) on the 1S exciton-polariton resonance in bulk ZnSe that is subject to an external magnetic field applied perpendicular to the light wave vector $\mathbf k$ (Voigt geometry). For the…

Mesoscale and Nanoscale Physics · Physics 2025-07-18 J. Mund , D. R. Yakovlev , A. Farenbruch , N. V. Siverin , M. A. Semina , M. M. Glazov , E. L. Ivchenko , M. Bayer

We have developed a numerical method for calculating the second harmonic generation (SHG) generated by an anisotropic material whose optical properties present an arbitrary modulation in one dimension. The method is based on the Berreman…

Optics · Physics 2023-05-31 J. Ortega , C. L. Folcia , J. Etxebarria

Optical second-harmonic generation (SHG) is a nonlinear parametric process that doubles the frequency of incoming light. Only allowed in non-centrosymmetric materials, it has been widely used in frequency modulation of lasers, surface…

Materials Science · Physics 2021-01-05 Wontaek Kim , Je Yhoung Ahn , Juseung Oh , Ji Hoon Shim , Sunmin Ryu
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