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Circular dichroism, arising from interactions with light fields of opposite spin angular momentum, has become a fundamental tool for molecular characterization. Meanwhile, helical dichroism (HD) - the dichroic response to vortex beams…

Circular dichroism (CD) induced by spin angular momentum of light is vital to investigate the chirality of microscopic objects such as molecules, proteins and metamaterials. However, orbital angular momentum (OAM) of light failed to…

Circular dichroism (CD) caused by the response of a chiral object to circularly polarized light has been well established, and the strong CD of plasmonic meta-molecules has also become of interest in recent years; however, their response if…

Optics · Physics 2020-09-30 Yangzhe Guo , Guodong Zhu , Wanlu Bian , Bin Dong , Yurui Fang

Helical dichroism (HD) is a proposed method for the resolution of molecular chirality, employing the orbital angular momentum (OAM) of light. Going beyond the conventional assumptions about HD, this work proposes a rigid theoretical…

Atomic Physics · Physics 2026-01-09 Mateja Hrast , Georgios M. Koutentakis , Mikhail Maslov , Mikhail Lemeshko

Chirality is a structural property of molecules lacking mirror symmetry that has strong implications in diverse fields, ranging from life to materials sciences. Established spectroscopic methods that are sensitive to chirality, such as…

Investigating chiral light-matter interactions is essential for advancing applications in sensing, imaging, and pharmaceutical development. However, the chiroptical response in natural chiral molecules and subwavelength chiral structures is…

Acoustic helical dichroism (HD) arises from the interaction between vortex beams carrying orbital angular momentum (OAM) and chiral media, yet such chiral sound-matter interactions are typically weak. Here, we employ quasi-bound states in…

Applied Physics · Physics 2025-12-02 Qing Tong , Tong Fu , Yuqiong Cheng , Shubo Wang

We present a system consisting of two stacked chiral plasmonic nanoelements, so-called triskelia, that exhibits a high degree of circular dichroism. The optical modes arising from the interactions between the two elements are the main…

Identifying and imaging spin textures of ever more complex magnetic structures has become a major challenge in the past decade, especially at ultrashort timescales. Most of current approaches are based on the analysis of their polarization…

Optics · Physics 2020-05-26 Thierry Ruchon , Mauro Fanciulli

Circular dichroism and helical dichroism are intriguing chiroptical phenomena with broad applications in optical sensing and imaging. Here, we generalize one of the phenomena-helical dichroism-to acoustics. We show that a one-dimensional…

Applied Physics · Physics 2022-03-22 Qing Tong , Shubo Wang

Chiral light-matter interactions have traditionally been understood in terms of electric-magnetic dipolar interference driven by light with spin angular momentum. Here, we show that optical chirality can also originate from the orbital…

Optics · Physics 2025-08-13 Shun Hashiyada , An'an Wu , Yoshito Y. Tanaka

The plasmon resonances (modes) of a metal nanostructure can be defined as a dipole, a quadrupole, or high-order modes depending on the surface charge distribution induced by the incident field. In a non-symmetrical environment or clusters,…

Whether or not chiral interaction exists between the optical orbital angular momentum (OAM) and a chiral molecule remains unanswered. So far, such an interaction has not been observed experimentally. Here we present a T-matrix method to…

Optics · Physics 2018-01-01 Tong Wu , Rongyao Wang , Xiangdong Zhang

The controlled fabrication and chiroptical characterization of microscale chiral structures remain central challenges in photonics, sensing, and metamaterial engineering. Here we demonstrate an accessible, low-cost platform that combines…

Optics · Physics 2026-05-07 Jing Xu , Rik Strobbe , Yovan de Coene , Renaud A. L. Vallée , Koen Clays

We report observation of electron helical dichroism on a material with chiral structure. In analogy with circular dichroism, a common technique for molecular structural fingerprinting, we use a nanofabricated forked diffraction grating to…

Materials Science · Physics 2015-07-08 Tyler R. Harvey , Jordan S. Pierce , Jordan J. Chess , Benjamin J. McMorran

Chirality is a highly important topic in modern chemistry, given the dramatically different pharmacological effects that enantiomers can have on the body. Chirality of natural molecules can be controlled by reconfiguration of molecular…

Optics · Physics 2018-03-21 Xiaoyang Duan , Simon Kamin , Florian Sterl , Harald Giessen , Na Liu

We present a rigorous finite element method to calculate circular dichroism (CD) in various systems consisting of nanostructures and oriented chiral molecules with electric quadrupole transitions. The interaction between oriented molecule…

Optics · Physics 2017-12-27 Weixuan Zhang , Tong Wu , Rongyao Wang , Xiangdong Zhang

Circular dichroism is the differential rate of absorption of right- and left-handed circularly polarized light by chiral particles. Optical vortices which convey orbital angular momentum (OAM) possess a chirality associated with the…

Optics · Physics 2021-05-26 Kayn A. Forbes , Garth A. Jones

We present a systematic investigation of the optical response to circularly polarized illumination in twisted stacked plasmonic nanostructures. The system consissts in two identical, parallel gold triskelia centrally aligned and rotated at…

We present the classical electromagnetic theory framework of reflection of a light beam carrying Orbital Angular Momentum (OAM) by an in-plane magnetic structure with generic symmetry. Depending on the magnetization symmetry, we find a…

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