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We present an experimental investigation of the Rydberg 23 P$_{1/2}$ state of laser-cooled $^{40}$Ca$^+$ ions in a radiofrequency ion trap. Using micromotion sideband spectroscopy on a narrow quadrupole transition, the oscillating electric…

Direct frequency comb spectroscopy of trapped ions is demonstated for the first time. It is shown that the 4s^2S_(1/2)-4p^2P_(3/2) transition in calcium ions can be excited directly with a frequency comb laser that is upconverted to 393 nm.…

Atomic Physics · Physics 2009-06-08 A. L. Wolf , S. A. van den Berg , W. Ubachs , K. S. E. Eikema

We present absolute-frequency measurements for the transitions from the 6s$_{1/2}$ ground state of $^{133}$Cs to $n$p$_{1/2}$ and $n$p$_{3/2}$ Rydberg states. The transition frequencies are determined by one-photon UV spectroscopy in…

We demonstrate excitation of a single trapped cold $^{40}$Ca$^+$ ion to Rydberg levels by laser radiation in the vacuum-ultraviolet at 122 nm wavelength. Observed resonances are identified as 3d$^2$D$_{3/2}$ to 51 F, 52 F and…

Quantum Physics · Physics 2015-10-28 T. Feldker , P. Bachor , M. Stappel , D. Kolbe , R. Gerritsma , J. Walz , F. Schmidt-Kaler

We present new measurements of quantum defects and core polarizabilities in cesium ($^{133}$Cs), based on transition frequency measurements between Rydberg states ($14 \leq n \leq 38$) obtained through terahertz (THz) and radio-frequency…

Atomic Physics · Physics 2025-06-03 Gianluca Allinson , Lucy A. Downes , Kevin J. Weatherill , C. Stuart Adams

We demonstrate a single-photon Rydberg excitation spectroscopy of cesium (Cs) atoms in a room-temperature vapor cell. Cs atoms are excited directly from 6S1/2 ground state to nP3/2 (n = 70 - 100) Rydberg states with a 318.6 nm ultraviolet…

Atomic Physics · Physics 2017-10-11 Jieying Wang , Jiandong Bai , Jun He , Junmin Wang

At TRIUMF's off-line laser ion source test stand, stepwise resonant laser ionization spectroscopy of chromium (Cr) was carried out, to find an efficient ionization scheme suitable for titanium sapphire (Ti:Sa) laser systems. With three…

Atomic Physics · Physics 2025-04-23 Romina Schulz , Ruohong Li , Julius Wessolek , Maryam Mostamand , Peter Kunz , Jens Lassen

A complete set of spectroscopic data is indispensable when using Rydberg states of trapped ions for quantum information processing. We carried out Rydberg series spectroscopy for $nS_{1/2}$ states with $38 \leq n \leq 65$ and for $nD_{5/2}$…

Atomic Physics · Physics 2022-08-25 Justas Andrijauskas , Jonas Vogel , Arezoo Mokhberi , Ferdinand Schmidt-Kaler

We present an innovative frequency comb methodology utilizing pulsed lasers for Rydberg atoms and implement it for electric field measurement. It achieves the Rydberg state population of multi-velocity group atoms through the two-photon…

Atomic Physics · Physics 2025-07-14 Ke Di , Chenglin Ye , Yijie Du , Yu Liu , Feng Gao , Jiajia Du , Jun He

We apply direct frequency-comb spectroscopy, in combination with precision cw spectroscopy, to measure the ${\rm 4s4p} ^3P_1 \to {\rm 4s5s} ^3S_1$ transition frequency in cold calcium atoms. A 657 nm ultrastable cw laser was used to excite…

Atomic Physics · Physics 2010-03-25 J. E. Stalnaker , Y. Le Coq , T. M. Fortier , S. A. Diddams , C. W. Oates , L. Hollberg

High accuracy frequency metrology on the 4s 2S1/2 - 4p 2P1/2 transition in calcium ions is performed using laser cooled and crystallized ions in a linear Paul trap. Calibration is performed with a frequency comb laser, resulting in a…

Atomic Physics · Physics 2009-11-13 A. L. Wolf , S. A. van den Berg , C. Gohle , E. J. Salumbides , W. Ubachs , K. S. E. Eikema

We present studies of resonance-enhanced photo-ionization for isotope-selective loading of Ca+ into a Paul trap. The 4s^2 ^1S_0 <-> 4s4p ^1P_1 transition of neutral calcium is driven by a 423nm laser and the atoms are photo-ionized by a…

We theoretically study multiphoton ionization of the Ca atom irradiated by the second (photon energy 3.1 eV) and third (photon energy 4.65 eV) harmonics of Ti:sapphire laser pulses (photon energy 1.55 eV). Because of the dense energy level…

Atomic Physics · Physics 2013-03-07 Gabriela Buica , Takashi Nakajima

We calculated the electronic interaction associated with the exchange of an electron between an atom of calcium excited to a Rydberg state ($n\sim 10-15$) and another, neighbouring calcium atom in its ground state. In this range the Rydberg…

Atomic Physics · Physics 2026-05-06 Alisée Bouillon , Matthieu Génévriez

This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to…

We present a versatile laser system which provides more than 1.5W of narrowband light, tunable in the range from 455-463 nm. It consists of a commercial Titanium-Sapphire laser which is frequency doubled using resonant cavity second…

We report on the observation and numerical calculation of ionization spectra of highly Stark-shifted Rydberg states of rubidium beyond the classical ionization threshold. In the numerical calculations, a complex absorbing potential (CAP)…

We demonstrate the ability to load, cool and detect singly-charged calcium ions in a surface electrode trap using only visible and infrared lasers for the trapped-ion control. As opposed to the standard methods of cooling using…

Atomic Physics · Physics 2017-07-27 F. Lindenfelser , M. Marinelli , V. Negnevitsky , S. Ragg , J. P. Home

We present Rydberg-state electromagnetically-induced-transparency (EIT) measurements examining the effects of laser polarization, magnetic fields, laser intensities, and the optical density of the thermal $^{87}$Rb medium. Two…

Atomic Physics · Physics 2022-01-11 Hsuan-Jui Su , Jia-You Liou , I-Chun Lin , Yi-Hsin Chen

We report the measurement of absolute excitation frequencies of 87Rb to nS and nD Rydberg states. The Rydberg transition frequencies are obtained by observing electromagnetically induced transparency on a rubidium vapor cell. The accuracy…

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