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A computational study of the electron paramagnetic resonance (EPR) $g$-tensors and hyperfine tensors in Mg and Zn doped $\beta$-Ga$_2$O$_3$ is presented. While Mg has been found previously to prefer the octahedral site, we find here that Zn…

Materials Science · Physics 2019-05-16 Dmitry Skachkov , Walter R. L. Lambrecht

A computational study of the Electron Paramagnetic Resonance (EPR) $g$-tensors and hyperfine tensors of Li and Ga vacancies in LiGaO$_2$ is presented. Density Functinal Theory (DFT) calculations are carried out of the Ga and Li vacancies…

Materials Science · Physics 2020-04-22 Dmitry Skachkov , Walter Lambrecht , Klichchupong Dabsamut , Adisak Boonchun

A theory for the reliable prediction of the EPR g-tensor for paramagnetic defects in solids is presented. It is based on density functional theory and on the gauge including projector augmented wave (GIPAW) approach to the calculation of…

Materials Science · Physics 2009-11-07 Chris J. Pickard , Francesco Mauri

We present a state interaction spin-orbit coupling method to calculate electron paramagnetic resonance (EPR) $g$-tensors from density matrix renormalization group wavefunctions. We apply the technique to compute $g$-tensors for the…

Chemical Physics · Physics 2018-07-17 Elvira R. Sayfutyarova , Garnet K. -L. Chan

This paper presents first principles calculations of paramagnetic cubic CrN$_x$ with the aim to provide deeper insight into recently published transmission electron microscopy-based study on this material. Among several types of point…

Materials Science · Physics 2014-10-14 David Holec , Liangcai Zhou , Zaoli Zhang , Paul H. Mayrhofer

A combined experimental/theoretical study of the EPR in irradiated $\beta$-Ga$_2$O$_3$ is presented. Four EPR spectra, two $S=1/2$ and two $S=1$, are observed after high-energy proton or electron irradiation. One of the S=1/2 spectra (EPR1)…

In the present Ph.D. Thesis we report an experimental investigation on the effects of gamma- and beta-ray irradiation and of subsequent thermal treatment on many types of a-SiO2 materials, differing in the production methods, OH- and…

Other Condensed Matter · Physics 2007-11-27 G. Buscarino

Calculations of formation energies and charge transition levels of defects routinely rely on density functional theory (DFT) for describing the electronic structure. Since bulk band gaps of semiconductors and insulators are not well…

Materials Science · Physics 2012-04-19 Audrius Alkauskas , Alfredo Pasquarello

X- and Q-band electron paramagnetic resonance (EPR) study is reported on the SrTiO3 single crystals doped with 0.5-at.% MnO. EPR spectra originating from the S = 2 ground state of Mn3+ ions are shown to belong to the three distinct types of…

Materials Science · Physics 2015-06-03 D. V. Azamat , A. Dejneka , J. Lancok , V. A. Trepakov , L. Jastrabik , A. G. Badalyan

The electron paramagnetic resonance (EPR) parameters ($g$ factors $g_{i}$ and the hyperfine structure constants ${{A}}_{{i}}$, ${i} = {x}, {y}, {z}$) are interpreted by using the perturbation formulae for a $3{d}^{9}$ ion in rhombically…

Materials Science · Physics 2015-12-25 Ch. -Y. Li , L. -B. Chen , J. -J. Mao , X. -M. Zheng

Proton irradiation of both n-type and semi-insulating bulk samples of \b{eta}-Ga2O3 leads to the formation of one paramagnetic defect with spin S=1/2, monoclinic point symmetry, a g-tensor with principal values of gb=2.0313, gc=2.0079, ga*=…

Experiments of Electron Spin Resonance (ESR) were performed on Co$% ^{2+}$ substituting Zn$^{2+}$ or Mg$^{2+}$ in powder samples of Zn$_2$(OH)PO$_4$ and Mg$_2$(OH)AsO$_4$. The observed resonances are described with a theoretical model that…

Materials Science · Physics 2009-11-07 M. E. Foglio , M. C dos Santos , G. E. Barberis , J. M. Rojo , J. L. Mesa , L. Lezama , T. Rojo

Electron paramagnetic resonance (EPR) is a valuable tool for physics, chemistry, biology and medicine, providing complementary spectroscopic information to NMR. It has long been known that EPR at high magnetic fields offers greater spectral…

We report Electron Paramagnetic Resonance measurements on single crystalline and powder samples of Nd_0.5Ca_0.5MnO_3 across the charge-ordering transition at T_co=240 K down to the antiferromagnetic ordering transition at T_N = 140 K. The…

Strongly Correlated Electrons · Physics 2021-05-26 Janhavi P. Joshi , Rajeev Gupta , A. K. Sood , S. V. Bhat , A. R. Raju , C. N. R. Rao

We report on low temperature photoluminescence (PL) and EPR study of bulk polycrystalline ZnO . Variation of peak position of donor bound exciton transition (D1XA) and FXAn=1-1LO with pump intensity show red shift and blue shift…

Materials Science · Physics 2012-02-29 Sanjiv Kumar Tiwari

Mn2+ ion doping is used as an electron paramagnetic resonance (EPR) probe to investigate the influence of low-coordination structural defects such as step edges at the surface of terraced (001) MgO nanoparticles on the electronic…

Mesoscale and Nanoscale Physics · Physics 2016-05-24 Peter V. Pikhitsa , Sukbyung Chae , Seungha Shin , Mansoo Choi

We present an electron paramagnetic resonance (EPR) study of ErSc2N@C80 fullerene in which there are two Er3+ sites corresponding to two different configurations of the ErSc2N cluster inside the C80 cage. For each configuration, the EPR…

Although the role of the electron paramagnetic resonance (EPR) g-tensor and hyperfine coupling tensor in the EPR effective spin Hamiltonian is discussed extensively in many textbooks, certain aspects of the theory are missing. In this text…

Quantum Physics · Physics 2023-05-12 Stanislav Komorovsky

The electron paramagnetic resonance (EPR) g factors g_x, g_y and g_z of the orthorhombic Cu^{2+}(1) site in fresh PrBa_{2}Cu_{3}O_{6+x} powders are theoretically investigated using the perturbation formulas of the g factors for a 3d^9 ion…

Materials Science · Physics 2012-10-09 M. Q. Kuang , S. Y. Wu , B. T. Song , X. F. Hu

Point defects in Ga- and Al-doped ZnO thin films are studied by means of first principles electronic structure calculations. Candidate defects are identified to explain recently observed differences in electrical and spectroscopical…

Materials Science · Physics 2016-10-06 E. Menéndez-Proupin , P. Palacios , P. Wahnón
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