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We have investigated the magnetic and dielectric properties of orthorhombic Eu$_{1-y}$Y$_y$MnO$_3$ ($0\leq y\leq 0.6$) single crystals without the presence of the 4$f$ magnetic moments of the rare-earth ions. In $y\geq 0.2$, the…

Strongly Correlated Electrons · Physics 2015-05-28 Mitsuru Akaki , Masaaki Hitomi , Mizuaki Ehara , Daisuke Akahoshi , Hideki Kuwahara

A ferroelectric is a material with a polar structure whose polarity can be reversed by applying an electric field. In metals, the itinerant electrons tend to screen electrostatic forces between ions, helping to explain why polar metals are…

We have recently reported that the Haldane spin-chain system, Er2BaNiO5, undergoing antiferromagnetic order below 32 K, is characterized by the onset of ferroelectricity near 60K due to magnetoelectric coupling induced by short-range…

Strongly Correlated Electrons · Physics 2015-06-22 Tathamay Basu , Kiran Singh , N. Mohapatra , E. V. Sampathkumaran

We present a detailed study of complex dielectric constant and ferroelectric polarization in multiferroic LiCuVO4 as function of temperature and external magnetic field. In zero external magnetic field, spiral spin order with an ab helix…

Strongly Correlated Electrons · Physics 2008-04-15 F. Schrettle , S. Krohns , P. Lunkenheimer , J. Hemberger , N. Büttgen , H. -A. Krug von Nidda , A. V. Prokofiev , A. Loidl

Perovskite metal-organic frameworks (MOFs) have recently emerged as potential candidates for multiferroicity. However, the compounds synthesized so far possess only weak ferromagnetism and low polarization. Additionally, the very low…

Materials Science · Physics 2018-01-24 Paresh Chandra Rout , Varadharajan Srinivasan

The polycrystalline co-doped samples of Sm0.5Y0.5Fe0.58Mn0.42O3 were prepared by solid-state reaction route and its various physical properties with their correlations have been investigated. The dc magnetization measurements on the sample…

The magnetic, dielectric and structural properties of type-I multiferroic KNiPO$_4$ have been investigated by neutron powder diffraction, magnetization, dielectric and high temperature synchrotron-XRD measurements. Below the N\'{e}el…

Strongly Correlated Electrons · Physics 2022-07-15 Alexandre Pages , Jian-Rui Soh , Marjaneh Jafari Fesharaki , Henrik M. Ronnow , Hossein Ahmadvand

The perovskite TbFe$_{0.5}$Cr$_{0.5}$O$_3$ shows two anomalies in the magnetic susceptibility at $T_N$ = 257K and $T_{SR}$ = 190K which are respectively, the antiferromagnetic and spin reorientation transition that occur in the Fe/Cr…

Multiferroicity in LiCu2O2 single crystals is studied using resonant soft x-ray magnetic scattering, hard x-ray diffraction, heat capacity, magnetic susceptibility, and electrical polarization. Two magnetic transitions are found at 24.6 K…

In multiferroic BiFeO$_3$ a cycloidal antiferromagnetic structure is coupled to a large electric polarization at room temperature, giving rise to magnetoelectric functionality that may be exploited in novel multiferroic-based devices. In…

Strongly Correlated Electrons · Physics 2017-03-08 R. D. Johnson , P. A. McClarty , D. D. Khalyavin , P. Manuel , P. Svedlindh , C. S. Knee

Multiferroics with coupling between ferroelectricity and magnetism have been pursued for decades. However, their magnetoelectric performances remain limited due to the common trade-off between ferroelectricity and magnetism. Here, a family…

Materials Science · Physics 2022-11-23 Churen Gui , Jun Chen , Shuai Dong

Composite multiferroics are materials exhibiting the interplay of ferroelectricity, magnetism, and strong electron correlations. Typical example --- magnetic nano grains embedded in a ferroelectric matrix. Coupling of ferroelectric and…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 O. G. Udalov , N. M. Chtchelkatchev , I. S. Beloborodov

BiFeO$_3$ is the most famous multiferroic material, but it has no strong spontaneous magnetization due to its antiferromagnetism. Here we show that giant ferroelectric polarization and strong spontaneous magnetization can be both realized…

Materials Science · Physics 2019-06-13 Peng Chen , Bang-Gui Liu

Dielectric and magnetic properties of Eu0.5Ba0.25Sr0.25TiO3 are investigated between 10 K and 300 K in the frequency range from 10 Hz to 100 THz. A peak in permittivity revealed near 130 K and observed ferroelectric hysteresis loops prove…

Materials Science · Physics 2012-10-12 Veronica Goian , Stanislav Kamba , Premysl Vanek , Maxim Savinov , Christelle Kadlec , Jan Prokleska

We report the observation of para - antiferromagnetic transition at ~ 50 K in lithium iron phosphate, LiFePO4 through DC magnetization and M\"ossbauer spectroscopy. The Ferrous ion Fe2+ (3d6, 5D) in LiFePO4 exhibits relaxation effects with…

Materials Science · Physics 2015-06-04 Y. Sundarayya , C. Bansal , C. S. Sunandana , Ajay Kumar Mishra , Richard A. Brand , Horst Hahn

We have studied the thermodynamic properties of a multiferroic that couples ferromagnetic and ferroelectric order. Some of the results are independent of the form of the free energy. We calculate the temperature dependence of the electric,…

Materials Science · Physics 2011-01-31 G. R. Boyd , P. Kumar , S. R. Phillpot

We report a phenomenological magneto-structural model based on competing free-energy terms that couple either polar or chiral distortions in cubic quadruple perovskites, depending on the global direction of magnetic moments. The model…

Materials Science · Physics 2024-03-05 M. Tardieux , E. Stylianidis , D. Behr , R. Liu , K. Yamaura , D. D. Khalyavin , D. R. Bowler , A. A. Belik , R. D. Johnson

We have investigated dielectric properties in a series of crystals of $R$MnO$_{3}$ ($R$ is a rare earth ion) under magnetic fields and quasihydrostatic pressure. We have found that ferroelectric phase appeared in GdMnO$_3$ crystal below…

Strongly Correlated Electrons · Physics 2009-11-10 H. Kuwahara , K. Noda , J. Nagayama , S. Nakamura

The magnetic properties of polycrystaline La0.5Ba0.5CoO2.5+d (d = 0.44 and 0.485) where investigated using muon spin relaxation and bulk magnetization experiments. Below a Curie temperature of T_C = 160 K and 180 K, respectively, a magnetic…

Strongly Correlated Electrons · Physics 2011-11-23 M. Stingaciu , H. Luetkens , Y. G. Pashkevich , E. Pomjakushina , K. Conder , H. -H. Klauss

Neutron diffraction studies have been carried out on a single crystal of oxygen-deficient perovskite NdBaCo2O5 in the temperature range of 7-370 K. There have been observed, with decreasing temperature T, two magnetic transitions…

Strongly Correlated Electrons · Physics 2009-11-10 Minoru Soda , Yukio Yasui , Masafumi Ito , Satoshi Iikubo , Masatoshi Sato , Kazuhisa Kakurai