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In this work, optimized size distribution and optical properties in colloidal synthesis of gold nanoparticles (GNPs) were obtained using a proposed ultrasonic Tuerkevich-Frens method. The effect of three ultrasound (20 kHz) irradiation…
We develop a quantitative description of giant asymmetry in reflectance, recently observed in semicontinuous metal films. The developed scaling-theory based technique reproduces the spectral properties of semicontinuous composites, as well…
Deep subwavelength integration of high-definition plasmonic nanostructures is of key importance for the development of future optical nanocircuitry for high-speed communication, quantum computation and lab-on-a-chip applications. So far the…
We present a full-wave analytical solution for the problem of second-harmonic generation from spherical nanoparticles. The sources of the second-harmonic radiation are represented through an effective nonlinear polarization. The solution is…
Luminescence constitutes a unique source of insight into hot carrier processes in metals, including those in plasmonic nanostructures used for sensing and energy applications. However, being weak in nature, metal luminescence remains poorly…
Self-assembled Plasmonic Nanoparticle Networks (PNN) composed of chains of 12-nm diameter crystalline gold nanoparticles exhibit a longitudinally coupled plasmon mode cen- tered at 700 nm. We have exploited this longitudinal absorption band…
We investigate the angle-resolved photoelectron spectra from laser-assisted photoionization for helium and neon atoms using an \textit{ab initio} method based on time-dependent surface flux and configuration interaction singles. We find…
Mie theory is the classical problem for modeling of light scattering by spherical particles. In this paper, we perform a spherical harmonic analysis of its solution for the induced fields to reveal the physics underlying the resonant…
Particle plasmons in metal nanoparticles have primarily been investigated through the use of local optical response approximations. However, as nanoparticle size approaches the average distance of electrons to the metal surface, mesoscopic…
We report a comprehensive study of aqueous halide adsorption on nanoparticles of gold and palladium that addresses several limitations hampering the use of atomistic modeling as a tool for understanding and improving wet-chemical synthesis…
Transient absorption spectroscopy is routinely used to study the electron dynamics in plasmonic gold nanoparticles. Typically, the transient absorption bleach is analyzed as measure for the electron temperature. However, the implicitly…
Energetic or "hot" electrons and holes generated from the decay of localized surface plasmons in metallic nanoparticles have great potential for applications in photocatalysis, photovoltaics, and sensing. Here, we study the generation of…
Gravitational lensing of luminous matter that surrounds a black hole or some other sufficiently compact object produces an infinite sequence of images. Besides the direct (or primary) image, it comprises demagnified and deformed replicas of…
Electronic excitations in metallic nanoparticles in the optical regime that have been of great importance in surface enhanced spectroscopy and emerging applications of molecular plasmonics, due to control and confinement of electromagnetic…
We study experimentally the transmission of light through a square lattice of nanoholes perforated in a optically-thick gold film. We observe that the periodicity of the structure enhances the light transmission for specific wavelengths,…
Subwavelength aperture arrays in thin metal films can enable enhanced transmission of light and matter (atom) waves. The phenomenon relies on resonant excitation and interference of the plasmon or matter waves on the metal surface. We show…
Plasmonic waveguides are a promising platform for integrated nanophotonic circuits and nanoscale quantum optics. Their use is however often hampered by the limited propagation length of the guided surface plasmon modes. A detailed…
Atomic diffraction through double slits and transmission gratings is well described in terms of the associated de Broglie waves and classical wave optics. However, for weakly bound and relatively large systems, such as the He_2 dimer, this…
Low-frequency Raman scattering spectra are presented for gold nanocrystals with diameters 3.5 and 13 nm. The frequencies of the Raman peaks but also their number are shown to vary with the nanocrystal size. These results are analyzed using…
The optical absorption properties of graphene wrapped dielectric particles have been investigated by using Mie scattering theory and exact multi-scattering method. It is shown that subwavelength strong absorption in infrared spectra can…