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We find that, for sufficiently strong mid-IR fields, transitions between different conduction bands play an important role in the generation of high-order harmonics in a dielectric. The transitions make a significant contribution to the…

Other Condensed Matter · Physics 2015-06-22 Peter G. Hawkins , Misha Yu. Ivanov , Vladislav S. Yakovlev

The observation of non-perturbative harmonic emission in solids from ultrashort laser pulses [1] sparked a wave of studies [2,3] as a probe of charge carrier dynamics in solids under strong fields and a route to extreme ultraviolet (XUV)…

Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. In atomic gases, high-harmonic radiation…

With a combination of numerical methods, including quantum Monte Carlo, exact diagonalization, and a simplified dynamical mean-field model, we consider the attosecond charge dynamics of electrons induced by strong-field laser pulses in…

Strongly Correlated Electrons · Physics 2021-10-08 Christopher Orthodoxou , Amelle Zaïr , George H. Booth

Ultrafast all-optical control of light emission is a central goal of extreme nonlinear optics, with implications for compact short-wavelength sources, petahertz optoelectronics, and label-free superresolution microscopy. High-harmonic…

At the core of attosecond science lies the ability to generate laser pulses of sub-femtosecond duration. In tabletop devices the process relies on high-harmonic generation, where a major challenge is to obtain high yields and high cutoff…

Atomic Physics · Physics 2014-11-05 J. Solanpää , J. A. Budagosky , N. I. Shvetsov-Shilovski , A. Castro , A. Rubio , E. Räsänen

We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…

We apply the theory of high-order harmonic generation by low-frequency laser fields in the strong field approximation to the study of the spatial and temporal coherence properties of the harmonics. We discuss the role of dynamically induced…

Quantum Physics · Physics 2007-05-23 Pascal Salières , Anne L'Huillier , Philippe Antoine , Maciej Lewenstein

It is shown that electron backscattering can enhance high-harmonic generation in periodic systems with broken translational symmetry. Paradigmatically, we derive for a finite chain of atoms the harmonic cutoff due to electrons backscattered…

Atomic Physics · Physics 2022-04-13 Chuan Yu , Ulf Saalmann , Jan M. Rost

We consider several aspects of high-order harmonic generation in solids: the effects of elastic and inelastic scattering; varying pulse characteristics; and inclusion of material-specific parameters through a realistic band structure. We…

Other Condensed Matter · Physics 2013-02-07 A. F. Kemper , B. Moritz , J. K. Freericks , T. P. Devereaux

We investigate the electron quantum path interference effects during high harmonic generation in atomic gas medium driven by ultrashort chirped laser pulses. To achieve that, we identify and vary the different experimentally relevant…

High harmonic spectra generated in condensed matter carry the fingerprints of sub-cycle electronic motion and the energy structure of the studied system. Here we show that tailoring the waveform of mid-infrared driving light by using a…

We study the generation of high harmonic radiation by Bloch electrons in a model transparent solid driven by a strong mid-infrared laser field. We solve the single-electron time-dependent Schr\"odinger equation (TDSE) using a velocity-gauge…

Atomic Physics · Physics 2015-05-20 Mengxi Wu , Shambhu Ghimire , David A. Reis , Kenneth J. Schafer , Mette B. Gaarde

We present a study of high-order-harmonic generation (HHG) assisted by extreme ultraviolet (XUV) attosecond pulses, which can lead to the excitation of inner-shell electrons and the generation of a second HHG plateau. With the treatment of…

Atomic Physics · Physics 2017-10-30 Jhih-An You , Jan Marcus Dahlström , Nina Rohringer

Based on the multiband semiconductor Bloch equations a microscopic approach to high-harmonic generation in crystalline solids which is able to properly describe degenerate bands and band crossings is presented and analyzed. It is well-known…

Mesoscale and Nanoscale Physics · Physics 2021-02-10 Le Huu Thong , Cong Ngo , Huynh Thanh Duc , Xiaohong Song , Torsten Meier

We study numerically the Bloch electron wavepacket dynamics in periodic potentials to simulate laser-solid interactions. We introduce a new perspective in the coordinate space combined with the motion of the Bloch electron wavepackets…

Optics · Physics 2018-01-12 Tao-Yuan Du , Xiao-Huan Huang , Xue-Bin Bian

Using reflective cross-polarized 2D THz time-domain spectroscopy in the range of 1-12 THz, we follow the trajectory of the out-of-equilibrium electron population in the low-bandgap semiconductor InSb. The 2D THz spectra show a set of…

Strongly Correlated Electrons · Physics 2019-06-10 S. Houver , L. Huber , M. Savoini , E. Abreu , S. L. Johnson

High-harmonic generation in solids by intense laser pulses provides a fascinating platform for studying material properties and ultra-fast electron dynamics, where its coherent character is a central aspect. Using the semiconductor Bloch…

Mesoscale and Nanoscale Physics · Physics 2026-01-22 Wolfgang Hogger , Alexander Riedel , Debadrito Roy , Angelika Knothe , Cosimo Gorini , Juan-Diego Urbina , Klaus Richter

Using a high-frequency field superposed to a linearly polarized bichromatic laser field composed by a wave with frequency $\omega $ and a wave with frequency $2\omega $, we show it is possible to enhance the intensity of a group of high…

Atomic Physics · Physics 2009-11-06 C. Figueira de Morisson Faria , M. L. Du

We theoretically study high-harmonic generation (HHG) from solids driven by intense laser pulses using a one-dimensional model periodic crystal. By numerically solving the time-dependent Schr\"{o}dinger equation directly on a real-space…