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Angle-resolved photoemission spectroscopy (ARPES) is a powerful probe of electron correlations in two-dimensional layered materials. In this Letter we demonstrate that ARPES can be used to probe the onset of exciton condensation in…

Strongly Correlated Electrons · Physics 2013-02-25 Stefan Rist , A. A. Varlamov , A. H. MacDonald , Rosario Fazio , Marco Polini

A velocity-map-imaging spectrometer is demonstrated to characterize the normalized transverse emittance of photoemitted electron bunches. The two-dimensional (2D) projected velocity distribution images of photoemitted electrons are recorded…

X-ray photoelectron diffraction is a powerful tool for determining the structure of clean and adsorbate-covered surfaces. Extending the technique into the ultrafast time domain will open the door to studies as diverse as the direct…

A deep understanding of molecular photo-transformations is challenging because of the complex interaction between the configurations of electrons and nuclei. An initial optical excitation dissipates energy into electronic and structural…

We perform numerical simulations for photoionization of the argon atom when exposed to a combined field of an infrared laser (abbreviated IR) and its 13th harmonic (H13) by solving the Time-Dependent Schr\"odinger Equation (TDSE)], noting…

Atomic Physics · Physics 2022-08-26 Soumia Chqondi , Souhaila Chaddou , Abdelkader Makhoute

We demonstrate a simple and robust high-resolution ghost spectroscopy approach for x-ray and extreme ultraviolet absorption spectroscopy at free-electron laser sources. Our approach requires an on-line spectrometer before the sample and a…

The toolbox for imaging molecules is well-equipped today. Some techniques visualize the geometrical structure, others the electron density or electron orbitals. Molecules are many-body systems for which the correlation between the…

We report on the design and performance of a velocity map imaging (VMI) spectrometer optimized for experiments using high-intensity extreme ultraviolet (XUV) sources such as laser-driven high-order harmonic generation (HHG) sources and…

Image subtraction in astronomy is a tool for transient object discovery such as asteroids, extra-solar planets and supernovae. To match point spread functions (PSFs) between images of the same field taken at different times a convolution…

Instrumentation and Methods for Astrophysics · Physics 2013-05-30 Steven Hartung , Hemant Shukla , J. Patrick Miller , Carlton Pennypacker

This paper discusses the reconstruction of partially sampled spectrum-images to accelerate the acquisition in scanning transmission electron microscopy (STEM). The problem of image reconstruction has been widely considered in the literature…

Image and Video Processing · Electrical Eng. & Systems 2020-02-05 Etienne Monier , Thomas Oberlin , Nathalie Brun , Xiaoyan Li , Marcel Tencé , Nicolas Dobigeon

In this paper, a simple method is proposed to extend the photon energy range of a soft x-ray self-seeding free-electron laser (FEL). A normal monochromator is first applied to purify the FEL spectrum and provide a coherent seeding signal.…

Accelerator Physics · Physics 2017-04-05 Kaiqing Zhang , Zheng Qi , Chao Feng , Haixiao Deng , Dong Wang , Zhentang Zhao

X-ray free-electron lasers (FEL) deliver ultrabright X-ray pulses, but not the sequences of phase-coherent pulses required for time-domain interferometry and control of quantum states. For conventional split-and-delay schemes to produce…

Accelerator Physics · Physics 2022-02-11 S. Reiche , G. Knopp , B. Pedrini , E. Prat , G. Aeppli , S. Gerber

We present a time-dependent density-functional method able to describe the photoelectron spectrum of atoms and molecules when excited by laser pulses. This computationally feasible scheme is based on a geometrical partitioning that…

Atomic Physics · Physics 2012-06-28 U. De Giovannini , D. Varsano , M. A. L. Marques , H. Appel , E. K. U. Gross , A. Rubio

Photoelectron interferometry with femto- and atto-second light pulses is a powerful probe of the fast electron wavepacket dynamics, albeit it has practical limitations on the energy resolution. We show that one can simultaneously obtain…

Atomic Physics · Physics 2022-02-24 A. Plunkett , M. A. Alarcon , J. K. Wood , C. H. Greene , A. Sandhu

We obtained the spectral function of the graphite H point using high resolution angle resolved photoelectron spectroscopy (ARPES). The extracted width of the spectral function (inverse of the photo-hole lifetime) near the H point is…

We present a novel remote gas detection and identification technique based on correlation spectroscopy with a piezoelectric tunable fibre-optic Fabry-P\'erot filter. We show that the spectral correlation amplitude between the filter…

Instrumentation and Methods for Astrophysics · Physics 2021-11-24 Ross Cheriton , Adam Densmore , Suresh Sivanandam , Ernst De Mooij , Pavel Cheben , Dan-Xia Xu , Jens H. Schmid , Siegfried Janz

We reflect on the prospect of exploiting the recoil associated with absorption and emission of photons to perform spectroscopy of a single molecular ion. For this recoil to be detectable, the molecular ion is sympathetically cooled by a…

Imaging structures at the molecular level is a fast developing interdisciplinary research field that spans across the boundaries of physics and chemistry. High spatial resolution images of molecules can be obtained with photons or ultrafast…

Atomic Physics · Physics 2016-09-01 R. Puthumpally-Joseph , J. Viau-Trudel , M. Peters , T. T. Nguyen-Dang , O. Atabek , E. Charron

We show that the recently proposed ionic microscope set-up [Kollath et.al, PRA, \textbf{76}, 063602 (2007)] could be adapted to measure the \textit {local single-particle energy distribution} of a degenerate Fermi gas \textit{in situ} with…

Strongly Correlated Electrons · Physics 2009-11-13 Y. Sherkunov , B. Muzykantskii , N. d'Ambrumenil , B. D Simons